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Thin-walled tubular deployable composite boom (DCB) has gained significant attention due to its lightweight, simple structure and high packaging efficiency. The experimental and numerical simulation methods were employed in this paper to investigate the folding behavior of the DCB. Using T700/epoxy unidirectional reinforced prepreg as raw material, DCB specimens were prepared by the vacuum bag method. To complete the folding experiments of DCB specimens, a folding mechanism was designed and manufactured. Folding experiments of DCB specimens were conducted and folding moment versus rotational displacement curves were measured. In addition, a Finite Element Model (FEM) was established to predict the folding behavior of the DCB. Different failure criteria were considered in the numerical analysis, including the Tsai‐Hill criterion and maximum stress criterion. Prediction results using the FEM were compared with experimental results, and both sets of results were in good agreement. It is shown that the DCB can achieve the folding function without failure. The research results in this paper are of great significance to the practical engineering application of the DCB. [Display omitted] • Six tubular deployable composite boom specimens and a precise folding mechanism were designed and prepared. • Folding experiments were conducted to measure the folding moment and rotational displacement curves. • A finite element model for predicting the folding behavior of the tubular deployable composite boom was established. [ABSTRACT FROM AUTHOR]