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1. A three-dimensional metal–organic framework based on hexanuclear copper units with unsaturated CuII centers

Author

Zhang, Huan, Lu, Ying, Zhang, Zhi-ming, and Wang, En-bo

Subjects
*ORGANOCOPPER compounds, *CARBOXYLATES, *SOLUTION (Chemistry), *CARBOXYL group, *CHEMICAL reactions, *PHOTOCATALYSIS, *CHEMICAL decomposition, *RHODAMINE B
Abstract

Abstract: A new metal–organic framework based on hexanuclear copper units, Cu6(μ3-O)(μ3-OH)(pz)6(btc) (pz=pyrazolate, btc=1,3,5-benzenetricarboxylate) 1, has been prepared by the hydrothermal reaction of Cu2+ ions, Hpz and H3btc ligands in a methanolic solution. The hexanuclear copper building unit in 1 is composed of two triangular Cu3O(H)(pz)3 units bridged by carboxyl groups, in which each Cu center is coordinatively unsaturated with open coordination sites. The photocatalytic investigation indicates that compound 1 exhibits a higher photocatalytic activity for the degradation of Rhodamine B. [Copyright &y& Elsevier]

Published
2012
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