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Usually, the temperature dependence of specific heats is neglected or the specific heats are frozen in interface computations for compressible two-material flows. In this paper, we present a practical interface treatment to faithfully capture the effect of high temperature on interface evolutions. A general technique for solving the Riemann problem equipped with a wide variety of equations of state (EOS) is established. In a unified framework for computing the interfacial states, it provides a convenient way to deal with the thermally perfect gas (PG) that considers the effect of temperature on specific heats. The algorithm of the complete and exact solution to Riemann problem with thermally PG is also designed in detail. Based on this technique, the modified ghost fluid method with an approximate Riemann solver is further extended to handle the interface of two-material flows involving thermally PG with chemical reactions. Several typical problems are selected to validate and test the present algorithm for the interaction between the thermally PG and other gases or liquids. The results indicate that the present algorithm enables an effective implementation for simulating various two-material multi-species flows with different types of EOS. As temperature increases, the behavior of the interfacial flows under the assumption of thermally PG EOS gradually differs from that under the assumption of calorically PG EOS. • Unified framework for simulating two-material multi-species flows. • Exact and approximate Riemann solvers for thermally perfect gases. • Modified ghost fluid method for high-temperature effects with chemical reactions. • Comparison of thermally/calorically perfect gases. [ABSTRACT FROM AUTHOR]