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Apart from Vaca Muerta's case history in Argentina, the unconventional exploration in South America is still underdeveloped, and one of the causes is the scarcity of geological studies. The present paper enlightens the embryonic unconventional exploration in the Sergipe-Alagoas Basin by introducing a seismic interpretation workflow to map thin shale layers and the natural fracture system, a challenge in unconventional reservoir explorations. Fracture and faults are critical elements in exploring ultra-low permeability shale oil/gas reservoirs. Identifying and locating these structures influence modeling fluid flow, hydraulics, and simulation models to improve horizontal well-drilling plans. The workflow comprises four main steps: data pre-conditioning, well-to-seismic tie, seismic spectral blueing (for frequency enhancement), and, finally, spectral decomposition and advanced fault attributes. The proposed workflow was applied to a seismic dataset from the onshore Brejo Grande oilfield focusing on the source rocks of the Coqueiro Seco Formation, the main unconventional reservoir candidate in the basin. That approach allowed mapping the lateral continuity, truncation, faults, and fractures in these thin shale layers previously below seismic resolution. The mapped structures belong to the complex natural fracture system with faults distributed to all trend directions. These faults are distributed along two zones with distinct fault densities with a possible sweet spot outline. • We present an interpretation workflow implemented to unconventional reservoirs. • The workflow combines seismic-resolution enhancing techniques and fault attributes. • As a result, thin-shale layers and fault zones were identified at Coqueiro Seco Fm. [ABSTRACT FROM AUTHOR]