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Abstract: This paper is the second in a series of three papers aimed at understanding the emissions of vehicles in China by conducting on-board emission measurements. This paper focuses on light-duty gasoline vehicles. In this study, we measured 57 light-duty gasoline vehicles (LDGVs) in three Chinese mega-cites (Beijing, Guangzhou, and Shenzhen), covering Euro 0 through Euro IV technologies, and generated CO, HC, and NOx emission factors and deterioration rates for each vehicle technology. The results show that the vehicle emission standards have played a significant role in reducing vehicle emission levels in China. The vehicle emission factors are reduced by 47–81%, 53–64%, 46–71%, and 78–82% for each phase from Euro I to Euro IV. Euro 0 vehicles have a considerably high emission level, which is hundreds of times larger than that of Euro IV vehicles. Three old taxis and four other Euro I and Euro II LDGVs are also identified as super emitters with equivalent emission levels to Euro 0 vehicles. Of the measured fleet, 23% super emitters were estimated to contribute 50–80% to total emissions. Besides vehicle emission standards, measures for restricting super emitters are equally important to reduce vehicle emissions. This study is intended to improve the understanding of the vehicle emission levels in China, but some key issues such as emission deterioration rates are yet to be addressed with the presence of a sufficient amount of vehicle emission measurements. [Copyright &y& Elsevier]

Abstract: This paper aims to study the vehicular emissions trends in the Beijing–Tianjin–Hebei (BTH) region, located in northern China. The multiyear emission inventories of NO X , CO, VOC and PM10 from road vehicles in the period 1999–2010 were developed by the COPERT IV model. Results show that vehicular emissions of CO and VOC have decreased by annual average change rates (AACR) of −3.1% to −5.2% and −4.4% to −6.9% in the study area, respectively. However, due to the rapid development of freight traffic, emissions of NO X and PM10 have kept increasing in Tianjin and Hebei. Based on the vehicular emission inventories, trends of emission levels for vehicles with different standards, as well as the overall effects of implementing vehicular emission mitigation strategies were assessed. It is suggested that passenger cars (PC) with Euro 0 and Euro I standards, which were at higher emission level in the PC fleet, should be gradually eliminated. Although the increasing rates (IR) of emissions from PC were lower than those of the PC population, the sharp growth of PC population in recent years contributed to a remarkable increase of emissions, weakening the overall mitigation effect. Total vehicle population capacity and other mitigation measures should be studied in China in order to develop new and more effective vehicular emission control strategies. [Copyright &y& Elsevier]

Abstract: In order to further study the realization of carbon intensity target, find the key influencing factors of CO2 emissions, and explore the path of developing low-carbon economy, this paper empirically studied the influences of urbanization level, economic level, industry proportion, tertiary industry proportion, energy intensity and R&D output on CO2 emissions in Beijing using improved STIRPAT (stochastic impacts by regression on population, affluence and technology) model. The model is examined using partial least square regression. Results show that urbanization level, economic level and industry proportion positively influence the CO2 emissions, while tertiary industry proportion, energy intensity and R&D output negatively do. Urbanization level is the main driving factor of CO2 emissions, and tertiary industry proportion is the main inhibiting factor. In addition, along with the growth of per capita GDP, the increase of CO2 emissions does not follow the Environmental Kuznets Curve model. Based on these empirical findings and the specific circumstances of Beijing, we provide some policy recommendations on how to reduce carbon intensity. Beijing should pay more attention to tertiary industry and residential energy consumption for carbon emission reduction. It is necessary to establish a comprehensive evaluation index of social development. Investing more capital on carbon emission reduction science and technology, and promoting R&D output is also an efficient way to reduce CO2 emissions. [Copyright &y& Elsevier]

Abstract: To improve the air quality during the 2008 Beijing Olympic Games, the Beijing Municipal Government enforced a series of emission control measures. This provided a valuable case study to evaluate the effectiveness of these aggressive measures on mitigating air pollution and improving the atmospheric environment. In this paper, we report the first results of the chemical and Sr isotopic compositions of the rainwater in Beijing during the 2008 Olympic year. The ionic composition of samples show that Ca2+ and NH4 + were the dominant cations, accounting for about 76–97% of the total cations, and that SO4 2− and NO3 − were the major anions, accounting for 61–91% of the total anions measured. Using Na as the indicator of marine origin and Al as that of terrestrial inputs, the proportions of sea salt and terrestrial elements were estimated from elemental ratios. The calculated results indicate that the major chemical components were mainly of non-sea-salt origin. Good correlation between Ca2+ and Sr2+ (R 2 =0.85) in rainwater samples indicates the potential of Sr as a provenance tracer for Ca. Sr2+ concentrations in rainwater samples ranged from 0.01 to 2.87μmoll−1, with 87Sr/86Sr ratios from 0.7092 to 0.7109. All of the samples had a 87Sr/86Sr ratio higher than that of seawater. The 87Sr/86Sr isotopic and elemental ratio systems show that the data set of rainwater was mainly distributed between the seawater end-member (~0.70917) and the soil dust end-member (0.7111–0.7115), and the analysis indicate that the effect of anthropogenic inputs could decrease in 2008. Comparisons of the chemical composition of the rainwater in different periods show that all chemical components, except NH4 +, had the lowest concentration levels during the Olympic Game period. The VWM concentrations of major ions in the rainwater decreased significantly during the Olympic period by up to 29% for SO4 2−, 39% for NO3 −, 38% for Ca2+, 51% for Mg2+, 57% for K+, and 44% for Na+, compared with the pre-control period. The concentrations of almost all species decreased during the 2008 Olympics, most likely due to both strict emission controls and favorable meteorological conditions. [Copyright &y& Elsevier]

Abstract: This paper reports findings of a recent field study that characterized the on-road emissions of individual diesel vehicles in and around Beijing, China during November and December of 2009. We successfully sampled 230 individual trucks on 4 major expressways around the city as well as 57 individual buses in the city using refined mobile chasing techniques and fast response instruments. Emission factors (EF) for carbon monoxide (CO), black carbon (BC) and particulate matter with diameters less than 0.5 μm (PM0.5) are derived from the measurements, which are consistent with the results from laboratory dynamometer tests. The PM0.5 number emission factor distributions demonstrate consistent bimodal modes with peaks around 10 nm and 80 nm, while the mass emission factor distributions demonstrate a unimodal maximum around 110 nm for a majority of the trucks. The BC emissions are shown to be highly correlated with the mass emission of particles with 100–250 nm diameters, which are in good agreement with the results from previous studies. A number of important policy implications are discussed based on the results from this study. First, we identified “heavy emitters” in the on-road fleet we encountered, finding that 5% of diesel trucks in this sample are responsible for 50% of total BC emissions, and 20% of the trucks are responsible for 50% CO and PM0.5 number emissions, 60% PM0.5 mass emissions and over 70% of BC emissions. This suggests that emissions control programs should include identifying and removing heavy emitters from the road or improving their emissions. Second, the BC and PM0.5 number emission factors of trucks registered in regions outside Beijing are significantly higher than those of Beijing-registered trucks, suggesting that improving engine and fuel standards in Beijing alone is not sufficient in reducing the traffic-related air pollution in Beijing. Third, the significantly lower emissions from Euro IV and CNG buses compared to the Euro II and Euro III buses support that introducing clean-burning buses is an effective way to reduce the overall vehicle emissions for the pollutants studied. Fourth, our refined chasing method demonstrates a cost-effective approach to characterize the emissions from a large number of on-road diesel vehicles. Further studies with large sample sizes are critical to constructing more accurate mobile emission inventories to represent the on-road vehicle population. [Copyright &y& Elsevier]

Abstract: Air pollutant emission inventory is an important input parameter for chemical transport models (CTMs). Since great uncertainties exist in the emission inventory, further improvements and refinements are required. In this paper, genetic algorithm (GA), a global search and optimization method, was applied to optimize the emission inventory for the Models-3/Community Multiscale Air Quality (CMAQ) model. An emission optimizing system based on GA was developed and embedded to the CMAQ through the design of several core modules, which implemented the basic functions such as emission adjusting, GA population initializing, CMAQ results evaluating and GA operating. Hypothetical and real-data experiments were respectively performed to examine the validity of GA for emission calibrating. GA showed good performance in both experiments and was always able to find the global minimum. The emission optimizing system was then used to calibrate seasonal PM10 emission inventories of Beijing. Results revealed that PM10 emission in Beijing was underestimated in 2002, an average of 62.74% higher adjustment factor should be imposed on the original emission in target months of different seasons. With the calibrated emission inventories, CMAQ model errors were decreased by 6.46% on average in different seasons. It was concluded that GA was a promising search technique in calibrating emission inputs for CTMs. [ABSTRACT FROM AUTHOR]

Abstract: The technical, economical and environmental performances of combined cooling, heating and power (CCHP) system are closely dependent on its design and operation strategy. This paper analyzes the energy flow of CCHP system and deduces the primary energy consumption following the thermal demand of building. Three criteria, primary energy saving (PES), annual total cost saving (ATCS), and carbon dioxide emission reduction (CDER) are selected to evaluate the performance of CCHP system. Based on the energy flow of CCHP system, the capacity and operation of CCHP system are optimized by genetic algorithm (GA) so as to maximize the technical, economical and environmental benefits achieved by CCHP system in comparison to separation production system. A numerical example of gas CCHP system for a hotel building in Beijing is given to ascertain the effectiveness of the optimal method. Furthermore, a sensitivity analysis is presented in order to show how the optimal operation strategy would vary due to the changes of electricity price and gas price. [Copyright &y& Elsevier]

Abstract: Traffic congestion and air pollution were two major challenges for the planners of the 2008 Olympic Games in Beijing. The Beijing municipal government implemented a package of temporary transportation control measures during the event. In this paper, we report the results of a recent research project that investigated the effects of these measures on urban motor vehicle emissions in Beijing. Bottom–up methodology has been used to develop grid-based emission inventories with micro-scale vehicle activities and speed-dependent emission factors. The urban traffic emissions of volatile organic compounds (VOC), carbon monoxide (CO), nitrogen oxides (NOx) and particulate matter with an aerodynamic diameter of 10 μm or less (PM10) during the 2008 Olympics were reduced by 55.5%, 56.8%, 45.7% and 51.6%, respectively, as compared to the grid-based emission inventory before the Olympics. Emission intensity was derived from curbside air quality monitoring at the North 4th Ring Road site, located about 7 km from the National Stadium. Comparison between the emission intensity before and during the 2008 Olympics shows a reduction of 44.5% and 49.0% in daily CO and NOx emission from motor vehicles. The results suggest that reasonable traffic system improvement strategies along with vehicle technology improvements can contribute to controlling total motor vehicle emissions in Beijing after the Olympic Games. [Copyright &y& Elsevier]

Vehicle exhaust emissions have posed a serious threat in recent years to the urban air quality of Beijing. It is necessary to accurately estimate the magnitude and distribution of these emissions in order to reduce the uncertainty of local scale air quality modeling assessment. This paper provides a bottom-up approach by combining vehicle emission factors and vehicle activity data from a travel demand model estimated at the grid level to generate vehicle emissions data for the Beijing urban area in 2005. In that year, vehicular emissions of HC, CO and NOx were respectively 13.33×104, 100.02×104 and 7.55×104 tons. The grid-based emissions were also compared with the vehicular emission inventory developed by macro-scale approach. It shows this bottom-up approach can result in better estimates of the levels and spatial distribution of vehicle emissions than the macro-scale method that relies on more average and aggregated information. [Copyright &y& Elsevier]

In this paper, we report the results and analysis of a recent field campaign in August 2007 investigating the impacts of emissions from transportation on air quality and community concentrations in Beijing, China. We conducted measurements in three different environments, on-road, roadside and ambient. The carbon monoxide, black carbon and ultrafine particle number emission factors for on-road light-duty vehicles are derived to be 95gkg−1-fuel, 0.3gkg−1-fuel and 1.8×1015 particleskg−1-fuel, respectively. The emission factors for on-road heavy-duty vehicles are 50gkg−1-fuel, 1.3gkg−1-fuel and 1.1×1016 particleskg−1-fuel, respectively. The carbon monoxide emission factors from this study agree with those derived from remote sensing and on-board vehicle emission testing systems in China. The on-road black carbon and particle number emission factors for Chinese vehicles are reported for the first time in the literature. Strong traffic impacts can be observed from the concentrations measured in these different environments. Most clear is a reflection of diesel truck traffic activity in black carbon concentrations. The comparison of the particle size distributions measured at the three environments suggests that the traffic is a major source of ultrafine particles. A four-day traffic control experiment conducted by the Beijing Government as a pilot to test the effectiveness of proposed controls was found to be effective in reducing extreme concentrations that occurred at both on-road and ambient environments. [Copyright &y& Elsevier]

This paper presents a novel method for quantification of the total emission of gases from area sources using the mobile mini-DOAS (Differential Optical Absorption Spectroscopy) instrument, a ground based optical remote sensing technique. The presented method has been applied to measure the emission of SO2 and NO2 from the city of Beijing, P.R. China, on a time scale of approximately 2h. The measurements have been performed during two field campaigns, in April and in August 2005. The estimated emission of NO2 is roughly the same during the two field campaigns with an average emission of 189tonsd−1 during April and 174tonsd−1 during August. The estimated emission of SO2 varies greatly between the two periods, with an average emission of 293tonsd−1 during April and 52tonsd−1 during August. [Copyright &y& Elsevier]

Particulate air pollution is a serious problem in Beijing. The annual concentration of particulate matter with aerodynamic diameter less than 10 μm (PM10), ranging from 141 to 166 μg m−3 in 2000–2004, could be very harmful to human health. In this paper, we presented the mortality and morbidity effects of PM10 pollution based on statistical data and the epidemiological exposure–response function. The economic costs to health during the 5 years were estimated to lie between US$1670 and $3655 million annually, accounting for about 6. 55% of Beijing''s gross domestic product each year. The total costs were apportioned into two parts caused by: the local emissions and long-range transported pollution. The contribution from local emissions dominated the total costs, accounting on average for 3. 60% of GDP. However, the contributions from transported pollution cannot be neglected, and the relative percentage to the total costs from the other regions could account for about 45%. An energy policy and effective measures should be proposed to reduce particulate matter, especially PM2. 5 pollution in Beijing to protect public health. The Beijing government also needs to cooperate with the other local governments to reduce high background level of particulate air pollution. [Copyright &y& Elsevier]

Substantial mitigation of air pollutants emissions has been performed since 2013 around Beijing, and changes in the atmospheric characteristics have been expected over the downstream area of Beijing. In this study, both WRF-Chem simulation and on-site measurements were utilized for the Baengnyeong (island) supersite, one of the representative regional background sites located in the Yellow Sea, the entrance area of the long-range transport process in Korea. The changes in the chemical compositions of inorganic aerosols were examined for spring-time during the Chinese emission mitigation period from 2014 to 2016. The measured ratio of ionic species to PM 2.5 at the Baengnyeong supersite showed changes in aerosol inorganic chemical compositions from sulfate in 2014 to nitrate in 2015–2016. The modeling results also showed that nitrate was low in 2014 and significantly increased in 2015 and 2016, and the acidic aerosol condition had also changed toward a more neutralized status in both the simulation and the observations. The WRF-Chem modeling study further indicated that the sulfur was not neutralized in 2014. However, in 2015 and 2016, SO 2 was more sufficiently neutralized as sulfur emissions were substantially reduced in China, while at the same time nitrate had begun to increase in such a 'SO 2 –poor' condition in Beijing area in China, and thus approaching more enhanced neutralization over the Yellow Sea area. The causes of the higher nitrate based on the modeled characteristics of the ammonia-sulfate-nitrate aerosol formation in response to the SO 2 emissions reduction in China are also discussed in this paper. Inorganic composition is changing from sulfate to nitrate, and aerosol acidity is approaching more enhanced neutralization over regional background area in Northeast Asia. Unlabelled Image • Inorganic components were examined over background area during Beijing's emission reduction. • Observations showed significant change in decreased sulfate and opposite trend in nitrate. • Aerosol acidity changed to enhanced nitrate neutralization through the emission reduction period. • More enhanced nitrate was also simulated by WRF-Chem mainly due to Beijing's emission mitigation. [ABSTRACT FROM AUTHOR]