1. Extreme magnetoresistance at high-mobility oxide heterointerfaces with dynamic defect tunability.
- Author
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Christensen, D. V., Steegemans, T. S., D. Pomar, T., Chen, Y. Z., Smith, A., Strocov, V. N., Kalisky, B., and Pryds, N.
- Subjects
MAGNETORESISTANCE ,ENHANCED magnetoresistance ,HETEROJUNCTIONS ,SEMIMETALS ,MAGNETIC fields ,STRENGTH of materials - Abstract
Magnetic field-induced changes in the electrical resistance of materials reveal insights into the fundamental properties governing their electronic and magnetic behavior. Various classes of magnetoresistance have been realized, including giant, colossal, and extraordinary magnetoresistance, each with distinct physical origins. In recent years, extreme magnetoresistance (XMR) has been observed in topological and non-topological materials displaying a non-saturating magnetoresistance reaching 10
3 −108 % in magnetic fields up to 60 T. XMR is often intimately linked to a gapless band structure with steep bands and charge compensation. Here, we show that a linear XMR of 80,000% at 15 T and 2 K emerges at the high-mobility interface between the large band-gap oxides γ-Al2 O3 and SrTiO3 . Despite the chemically and electronically very dissimilar environment, the temperature/field phase diagrams of γ-Al2 O3 /SrTiO3 bear a striking resemblance to XMR semimetals. By comparing magnetotransport, microscopic current imaging, and momentum-resolved band structures, we conclude that the XMR in γ-Al2 O3 /SrTiO3 is not strongly linked to the band structure, but arises from weak disorder enforcing a squeezed guiding center motion of electrons. We also present a dynamic XMR self-enhancement through an autonomous redistribution of quasi-mobile oxygen vacancies. Our findings shed new light on XMR and introduce tunability using dynamic defect engineering. Extreme magnetoresistance is characterized by a large and non-saturating magnetoresistance. Typically, it is observed in materials with compensated bandstructures, however, here, Christensen et al demonstrate a large and non-saturating magnetoresistance in a γAl2O3/SrTiO3 heterostructure, which is related to disorder, rather than the materials bandstructure. [ABSTRACT FROM AUTHOR]- Published
- 2024
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