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1. Spontaneous exciton dissociation enables spin state interconversion in delayed fluorescence organic semiconductors

Author

Alexander J. Gillett, Claire Tonnelé, Giacomo Londi, Gaetano Ricci, Manon Catherin, Darcy M. L. Unson, David Casanova, Frédéric Castet, Yoann Olivier, Weimin M. Chen, Elena Zaborova, Emrys W. Evans, Bluebell H. Drummond, Patrick J. Conaghan, Lin-Song Cui, Neil C. Greenham, Yuttapoom Puttisong, Frédéric Fages, David Beljonne, and Richard H. Friend

Subjects
Science
Abstract

A low singlet-triplet energy gap, necessary for delayed fluorescence organic semiconductors, results in a small radiative rate that limits performance in OLEDs. Here, the authors show that it is possible to reconcile these conflicting requirements in materials that can access both high oscillator strength intramolecular excitations and intermolecular charge transfer states.

Published
2021
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