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2. First identification and thermodynamic characterization of the ternary U(VI) species, U[O.sub.2]([O.sub.2])[(C[O.sub.3]).sub.2.sup.4-], in U[O.sub.2]-[H.sub.2][O.sub.2]-[K.sub.2]C[O.sub.3] solutions

Author

Goff, George S., Brodnax, Lia F., Cisneros, Michael R., Peper, Shane M., Field, Stephanie E., Scott, Brian L., and Runde, Wolfgang H.

Subjects
Ligands -- Analysis, Coordination compounds -- Chemical properties, Carbonates -- Chemical properties, Chemistry
Abstract

The spectroscopic characterization and thermodynamic stability of the mixed-ligand complex, U[O.sub.2]([O.sub.2])[(C[O.sub.3]).sub.2.sup.4-], is described in both solution and solid state. The studies have shown that the stable solution species is U[O.sub.2]([O.sub.2])[(C[O.sub.3]).sub.2.sup.4-], which has a formation constant that is relative to the tris-carbonato complex.

Published
2008

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