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1. Complexes of triamidoamines with the early actinides. Synthetic routes to monomeric compounds of tetravalent uranium and thorium containing halide and amide ligands

Author

Roussel, Paul, Alcock, Nathaniel W., Boaretto, Rita, Kingsley, Andrew J., Munslow, Ian J., Sanders, Christopher J., and Scott, Peter

Subjects
Actinide elements -- Research, Monomers -- Research, Uranium -- Research, Thorium -- Research, Ligands -- Research, Chemistry
Abstract

Research was conducted to tune the steric protection yielded by substituents on the triamidoamine ligands such that the actinide complexes would have symmetric structures but also be reactive enough to be utilized in the exploration of the chemistry of the elements of this form. Using the tert-butyldimethylsilyl ligand obtains this objective. A convenient approach to the system via the preparation of monomeric, tetravalent actinide chlorides, bromides, iodides and amides is described.

Published
1999

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