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1. Direct amide synthesis from either alcohols or aldehydes with amines: activity of Ru(II) hydride and Ru(0) complexes

Author

Muthaiah, Senthilkumar, Ghosh, Subhash Chandra, Joo-Eun Jee, Cheng Chen, Jian Zhang, and Soon Hyeok Hong

Subjects
Ruthenium -- Chemical properties, Ruthenium -- Structure, Amides -- Chemical properties, Amides -- Structure, Aldehydes -- Chemical properties, Aldehydes -- Structure, Acetonitrile -- Chemical properties, Acetonitrile -- Structure, Biological sciences, Chemistry
Abstract

An in situ generated catalyst were developed from readily available Ru[H.sub.2][(P[Ph.sub.3]).sub.4], an N-heterocyclic carbene (NHC) precursor, NaH, and acetonitrile. The prepared catalyst exhibited high activity for the amide synthesis directly from either alcohols or aldehydes with amines.

Published
2010

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