1. Improving dynamic collision frequencies: Impacts on dynamic structure factors and stopping powers in warm dense matter
- Author
-
Hentschel, T. W., Kononov, A., Olmstead, A., Cangi, A., Baczewski, A. D., and Hansen, S. B.
- Subjects
Matter under extreme conditions ,X-ray Thomson scattering ,Average-atom models ,Density functional theory ,Time-dependent density functional theory ,Collision frequencies ,High-energy density science ,Warm dense matter - Abstract
Simulations and diagnostics of high-energy-density plasmas and warm dense matter rely on models of material response properties, both static and dynamic (frequency-dependent). Here, we systematically investigate variations in dynamic electron–ion collision frequencies ν(ω) in warm dense matter using data from a self-consistent-field average-atom model. We show that including the full quantum density of states, strong collisions, and inelastic collisions lead to significant changes in ν(ω) . These changes result in red shifts and broadening of the plasmon peak in the dynamic structure factor, an effect observable in x-ray Thomson scattering spectra, and modify stopping powers around the Bragg peak. These changes improve the agreement of computationally efficient average-atom models with first-principles time-dependent density functional theory in warm dense aluminum, carbon, and deuterium.
- Published
- 2023