61 results on '"Minola, M."'
Search Results
2. Dependence of Tc of YBa2Cu3O6.67 on in-plane uniaxial stress
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Barber, M.E., Kim, H.-H., Loew, T., Le Tacon, M., Minola, M., Konczykowski, M., Keimer, B., Mackenzie, A.P., Hicks, C.W., University of St Andrews. School of Physics and Astronomy, and University of St Andrews. Condensed Matter Physics
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MCC ,QC Physics ,TK ,DAS ,QC ,TK Electrical engineering. Electronics Nuclear engineering - Abstract
Funding: We acknowledge the financial support of the Max Planck Society. A.P.M. and C.W.H. acknowledge support from the Deutsche Forschungsgemeinschaft through SFB 1143 (Project ID 247310070). M.K. acknowledges financial support from ANR LABEX Grant No. ANR-10-LABX-0039-PALM. We probe the effect on Tc of in-plane uniaxial stress applied to the high-temperature superconductor YBa2Cu3O6.67. We find a highly anisotropic response. Under compression along the b axis, which reduces the orthorhombicity of the CuO2 planes, Tc is broadly flat for stresses up to at least 1.7 GPa. Under compression along the a axis, Tc decreases steeply. For stresses beyond ≈1 GPa the decrease is quasilinear. We hypothesize that superconductivity is suppressed by competition with uniaxial charge density wave order, which has been found to onset at ≈1 GPa. Publisher PDF
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- 2022
3. Investigations of Graphene on SrTiO3 Single-Crystal using Confocal Raman Spectroscopy
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Shrestha, S., Chang, C. S., Lee, S., Kothalawala, N. L., Kim, D. Y., Minola, M., Kim, J., and Seo, A.
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Condensed Matter - Other Condensed Matter ,Condensed Matter - Materials Science ,Condensed Matter - Strongly Correlated Electrons ,Strongly Correlated Electrons (cond-mat.str-el) ,Materials Science (cond-mat.mtrl-sci) ,FOS: Physical sciences ,Other Condensed Matter (cond-mat.other) - Abstract
Graphene layers placed on SrTiO3 single-crystal substrates were investigated using temperature-dependent confocal Raman spectroscopy. This approach successfully resolved distinct Raman modes of graphene that are often untraceable in conventional measurements due to the strong Raman scattering background of SrTiO3. Information on defects and strain states was obtained for a few graphene/SrTiO3 samples that were synthesized by different techniques. This confocal Raman spectroscopic approach can shed light on the investigation of not only this graphene/SrTiO3 system but also various two-dimensional layered materials whose Raman modes interfere with their substrates., Comment: 6 pages, 3 figures
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- 2022
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4. Charge density waves in YBa$_2$Cu$_3$O$_{6.67}$ probed by resonant x-ray scattering under uniaxial compression
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Kim, H. -H., Lefrançois, E., Kummer, K., Fumagalli, R., Brookes, N. B., Betto, D., Nakata, S., Tortora, M., Porras, J., Loew, T., Barber, M., Braicovich, L., Mackenzie, A. P., Hicks, C. W., Keimer, B., Minola, M., Tacon, M. Le, University of St Andrews. School of Physics and Astronomy, and University of St Andrews. Condensed Matter Physics
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Superconductivity (cond-mat.supr-con) ,MCC ,Condensed Matter - Strongly Correlated Electrons ,QC Physics ,Strongly Correlated Electrons (cond-mat.str-el) ,TK ,Condensed Matter::Superconductivity ,Condensed Matter - Superconductivity ,NDAS ,FOS: Physical sciences ,QC ,TK Electrical engineering. Electronics Nuclear engineering - Abstract
We report a comprehensive Cu L$_3$-edge resonant x-ray scattering study of two- and three-dimensional (2D and 3D) incommensurate charge correlations in single crystals of the underdoped high-temperature superconductor YBa$_2$Cu$_3$O$_{6.67}$ under uniaxial compression up to 1% along the two inequivalent Cu-O-Cu bond directions (a and b) in the CuO$_2$ planes. The pressure response of the 2D charge correlations is symmetric: pressure along a enhances correlations along b, and vice versa. Our results imply that the underlying order parameter is uniaxial. In contrast, 3D long-range charge order is only observed along b in response to compression along a. Spectroscopic resonant x-ray scattering measurements show that the 3D charge order resides exclusively in the CuO$_2$ planes and may thus be generic to the cuprates. We discuss implications of these results for models of electronic nematicity and for the interplay between charge order and superconductivity., Revised version - Accepted for publication in Phys. Rev. Lett
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- 2020
5. Backfolded acoustic phonons as ultrasonic probes in metal-oxide superlattices
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Lyzwa, Fryderyk, Chan, A., Khmaladze, Jarji, Fürsich, K., Keimer, B., Bernhard, Christian, Minola, M., and Mallett, Benjamin P. P.
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Condensed Matter::Materials Science - Abstract
Ultrasonics have been an incisive probe of internal interfaces in a wide variety of systems ranging from stars to solids. For thin-film structures, however, ultrasound is largely ineffective because the signal is dominated by the substrate. Using confocal Raman spectromicroscopy, we show that multiple reflection of sound waves at internal interfaces of a metal-oxide superlattice generates standing waves that are insensitive to the substrate. Such modes had previously been observed only in high-quality superlattices of elemental semiconductors, and their observation in complex metal- oxide heterostructures is testimony to recent progress in this field. We use the high spatial resolution of the Raman microscope to demonstrate the high sensitivity of the mode frequency to atomic-scale thickness variations of the superlattice. Spectroscopy of acoustic standing waves can hence serve as a powerful characterization tool of thin-film structures. In analogy to ultrasound spectroscopy of bulk solids, lineshape analysis of these modes has the potential to yield detailed information about the internal structure of the interfaces as well as the coupling of sound waves to the low- frequency spin, charge, and orbital dynamics in metal-oxide superlattices.
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- 2020
6. Granular superconductivity and charge/orbital order in YBa 2 Cu 3 O 7 /manganite trilayers
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Khmaladze, Jarji, Sarkar, Subhrangsu, Soulier, Mathias, Lyzwa, Fryderyk, Prada, R. de Andres, Perret, Edith, Mallett, Benjamin P. P., Minola, M., Keimer, B., and Bernhard, Christian
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Condensed Matter::Materials Science ,Condensed Matter::Superconductivity ,Condensed Matter::Strongly Correlated Electrons - Abstract
We studied how the electronic, superconducting, and magnetic properties of YBa2Cu3O7/Nd1−x(Ca1−ySry )xMnO3 multilayers depend on the tolerance factor and the hole doping of the manganite. In particular, we investigated the granular superconducting state and the related magnetic-field-driven insulator-to- superconductor transition that was previously discovered in corresponding multilayers with Pr0.5La0.2Ca0.3MnO3 [B. P. P. Mallett et al., Phys. Rev. B 94, 180503(R) (2016)]. We found that this granular uperconducting state occurs only when the manganite layer is in a charge/orbital ordered and CE-type antiferromagnetic state (Mn-CO/OO). The coupling mechanism underlying this intriguing proximity effect seems to involve the domain boundaries of the Mn-CO/OO and/or the charge disordered regions of the manganite layer that become more numerous as the hole doping is reduced below x = 0.5.
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- 2019
7. Raman scattering from current-stabilized nonequilibrium phases in Ca$_2$RuO$_4$
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F��rsich, K., Bertinshaw, J., Butler, P., Krautloher, M., Minola, M., and Keimer, B.
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Condensed Matter - Strongly Correlated Electrons ,Strongly Correlated Electrons (cond-mat.str-el) ,FOS: Physical sciences ,Condensed Matter::Strongly Correlated Electrons - Abstract
We used Raman light scattering to study the current-stabilized nonequilibrium semimetallic and metallic phases in Ca$_2$RuO$_4$. By determining the local temperature through careful analysis of the Stokes and anti-Stokes intensities, we find that Joule heating can be completely avoided by supplying sufficient cooling power in a helium-flow cryostat, and that the current induces the semimetallic state without inducing any significant heating. We further investigate the current-induced semimetallic state as a function of temperature and current. We confirm the absence of long-range antiferromagnetic order and identify a substantial Fano broadening of several phonons, which suggests coupling to charge and orbital fluctuations. Our results demonstrate that the semimetallic state is a genuine effect of the applied electrical current and that the current-induced phases have characteristics distinct from the equilibrium ones., accepted for publication as a Rapid Communication in Physical Review B
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- 2019
8. Polarization resolved Cu $L_3$-edge resonant inelastic x-ray scattering of orbital and spin excitations in NdBa$_{2}$Cu$_{3}$O$_{7-\delta}$
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Fumagalli, R., Braicovich, L., Minola, M., Peng, Y. Y., Kummer, K., Betto, D., Rossi, M., Lefrançois, E., Morawe, C., Salluzzo, M., Suzuki, H., Yakhou, F., Tacon, M. Le, Keimer, B., Brookes, N. B., Sala, M. Moretti, and Ghiringhelli, G.
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Condensed Matter - Strongly Correlated Electrons ,Condensed Matter::Superconductivity ,Condensed Matter - Superconductivity ,Condensed Matter::Strongly Correlated Electrons - Abstract
High resolution resonant inelastic x-ray scattering (RIXS) has proven particularly effective in the determination of crystal field and spin excitations in cuprates. Its strength lies in the large Cu $L_{3}$ resonance and in the fact that the scattering cross section follows quite closely the single-ion model predictions, both in the insulating parent compounds and in the superconducting doped materials. However, the spectra become increasingly broader with (hole) doping, hence resolving and assigning spectral features has proven challenging even with the highest energy resolution experimentally achievable. Here we have overcome this limitation by measuring the complete polarization dependence of the RIXS spectra as function of momentum transfer and doping in thin films of NdBa$_{2}$Cu$_{3}$O$_{7-\delta}$. Besides confirming the previous assignment of $dd$ and spin excitations (magnon, bimagnon) in the antiferromagnetic insulating parent compound, we unequivocally single out the actual spin-flip contribution at all dopings. We also demonstrate that the softening of $dd$ excitations is mainly attributed to the shift of the $xy$ peak to lower energy loss. These results provide a definitive assessment of the RIXS spectra of cuprates and demonstrate that RIXS measurements with full polarization control are practically feasible and highly informative., Comment: 14 pages, 10 figures
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- 2019
9. Compressive-strain induced enhancement of exchange interactions and short-range magnetic order in Sr$_2$IrO$_4$ investigated by Raman spectroscopy
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Seo, A., Stavropoulos, P. P., Kim, H. -H., Fürsich, K., Souri, M., Connell, J. G., Gretarsson, H., Minola, M., Kee, H. Y., and Keimer, B.
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Superconductivity (cond-mat.supr-con) ,Condensed Matter - Strongly Correlated Electrons ,Condensed Matter - Materials Science ,Condensed Matter::Materials Science ,Condensed Matter - Mesoscale and Nanoscale Physics ,Strongly Correlated Electrons (cond-mat.str-el) ,Condensed Matter - Superconductivity ,Mesoscale and Nanoscale Physics (cond-mat.mes-hall) ,Materials Science (cond-mat.mtrl-sci) ,FOS: Physical sciences ,Condensed Matter::Strongly Correlated Electrons - Abstract
We have carried out Raman spectroscopy experiments to investigate two-magnon excitations in epitaxial thin films of the quasi-two-dimensional antiferromagnetic Mott insulator Sr$_2$IrO$_4$ under in-plane misfit strain. With in-plane biaxial compression, the energy of the two-magnon peak increases, and the peak remains observable over a wider temperature range above the N\'eel temperature, indicating strain-induced enhancement of the superexchange interactions between $\it{J}_{eff}$ = 1/2 pseudospins. From density functional theory calculations, we have found an increase of the nearest-neighbor hopping parameter and exchange interaction with increasing biaxial compressive strain, in agreement with the experimental observations. Our experimental and theoretical results provide perspectives for systematic, theory-guided strain control of the primary exchange interactions in 5$\it{d}$ transition metal oxides., Comment: 3 figures
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- 2019
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10. Polarization resolved Cu $L_3$-edge resonant inelastic x-ray scattering of orbital and spin excitations in NdBa$_{2}$Cu$_{3}$O$_{7-��}$
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Fumagalli, R., Braicovich, L., Minola, M., Peng, Y. Y., Kummer, K., Betto, D., Rossi, M., Lefran��ois, E., Morawe, C., Salluzzo, M., Suzuki, H., Yakhou, F., Tacon, M. Le, Keimer, B., Brookes, N. B., Sala, M. Moretti, and Ghiringhelli, G.
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Superconductivity (cond-mat.supr-con) ,Strongly Correlated Electrons (cond-mat.str-el) ,Condensed Matter::Superconductivity ,FOS: Physical sciences ,Condensed Matter::Strongly Correlated Electrons - Abstract
High resolution resonant inelastic x-ray scattering (RIXS) has proven particularly effective in the determination of crystal field and spin excitations in cuprates. Its strength lies in the large Cu $L_{3}$ resonance and in the fact that the scattering cross section follows quite closely the single-ion model predictions, both in the insulating parent compounds and in the superconducting doped materials. However, the spectra become increasingly broader with (hole) doping, hence resolving and assigning spectral features has proven challenging even with the highest energy resolution experimentally achievable. Here we have overcome this limitation by measuring the complete polarization dependence of the RIXS spectra as function of momentum transfer and doping in thin films of NdBa$_{2}$Cu$_{3}$O$_{7-��}$. Besides confirming the previous assignment of $dd$ and spin excitations (magnon, bimagnon) in the antiferromagnetic insulating parent compound, we unequivocally single out the actual spin-flip contribution at all dopings. We also demonstrate that the softening of $dd$ excitations is mainly attributed to the shift of the $xy$ peak to lower energy loss. These results provide a definitive assessment of the RIXS spectra of cuprates and demonstrate that RIXS measurements with full polarization control are practically feasible and highly informative., 14 pages, 10 figures
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- 2019
- Full Text
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11. Electronic and vibrational signatures of ruthenium vacancies in Sr$_2$RuO$_4$ thin films
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Kim, Gideok, Suyolcu, Y. Eren, Herrero-Martin, J., Putzky, D., Nair, H. P., Ruf, J. P., Schreiber, N. J., Dietl, C., Christiani, G., Logvenov, G., Minola, M., van Aken, P. A., Shen, K. M., Schlom, D. G., and Keimer, B.
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Superconductivity (cond-mat.supr-con) ,Condensed Matter - Materials Science ,Condensed Matter - Strongly Correlated Electrons ,Strongly Correlated Electrons (cond-mat.str-el) ,Condensed Matter - Superconductivity ,Materials Science (cond-mat.mtrl-sci) ,FOS: Physical sciences - Abstract
The synthesis of stoichiometric Sr$_2$RuO$_4$ thin films has been a challenge because of the high volatility of ruthenium oxide precursors, which gives rise to ruthenium vacancies in the films. Ru vacancies greatly affect the transport properties and electronic phase behavior of Sr$_2$RuO$_4$, but their direct detection is difficult due to their atomic dimensions and low concentration. We applied polarized X-ray absorption spectroscopy at the oxygen K-edge and confocal Raman spectroscopy to Sr$_2$RuO$_4$ thin films synthesized under different conditions. The results show that these methods can serve as sensitive probes of the electronic and vibrational properties of Ru vacancies, respectively. The intensities of the vacancy-related spectroscopic features extracted from these measurements are well correlated with the transport properties of the films. The methodology introduced here can thus help to understand and control the stoichiometry and transport properties in films of Sr$_2$RuO$_4$ and other ruthenates.
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- 2019
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12. Polarization-resolved Cu L3-edge resonant inelastic X-ray scattering of orbital and spin excitations in NdBa2Cu3 O7-δ
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Fumagalli, R., Braicovich, L., Minola, M., Peng, Y. Y., Kummer, K., Betto, D., Rossi, M., Lefrancois, E., Morawe, C., Salluzzo, M., Suzuki, H., Yakhou, F., Le Tacon, M., Keimer, B., Brookes, N. B., Sala, M. M., and Ghiringhelli, G.
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- 2019
13. Backfolded acoustic phonons in metal-oxide superlattices
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Lyzwa, F., Chan, A., Khmaladze, J., Fürsich, K., Keimer, B., Bernhard, C., Minola, M., and Mallett, B. P. P.
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Superconductivity (cond-mat.supr-con) ,Condensed Matter - Materials Science ,Condensed Matter - Strongly Correlated Electrons ,Condensed Matter::Materials Science ,Strongly Correlated Electrons (cond-mat.str-el) ,Condensed Matter - Superconductivity ,Condensed Matter::Superconductivity ,Materials Science (cond-mat.mtrl-sci) ,FOS: Physical sciences ,Condensed Matter::Mesoscopic Systems and Quantum Hall Effect - Abstract
We report the observation of low-frequency modes in the Raman spectra of thin-film superlattices of the high-temperature superconductor YBa$ _{2} $Cu$ _{3} $O$ _{7-\delta} $ and various manganite perovskites. Our study shows that these modes are caused by the backfolding of acoustic phonons due to the additional periodicity introduced by the superlattice. Such modes were previously only observed for ultra-pure semiconductor superlattices. They can be used to determine the bilayer thickness of the superlattice and its speed of sound. Moreover, we use the spatial resolution of Raman microscopy to map the film thickness inhomogeneity across a sample, making these modes a useful tool to characterize thin-film superlattices., Comment: 5 pages, 4 figures
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- 2019
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14. Stabilization of three-dimensional charge order in YBa2Cu3O6+x via epitaxial growth
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Bluschke, M, Frano, A, Schierle, E, Putzky, D, Ghorbani, F, Ortiz, R, Suzuki, H, Christiani, G, Logvenov, G, Weschke, E, Birgeneau, RJ, da Silva Neto, EH, Minola, M, Blanco-Canosa, S, and Keimer, B
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Condensed Matter::Superconductivity - Abstract
© 2018, The Author(s). Incommensurate charge order (CO) has been identified as the leading competitor of high-temperature superconductivity in all major families of layered copper oxides, but the perplexing variety of CO states in different cuprates has confounded investigations of its impact on the transport and thermodynamic properties. The three-dimensional (3D) CO observed in YBa2Cu3O6+x in high magnetic fields is of particular interest, because quantum transport measurements have revealed detailed information about the corresponding Fermi surface. Here we use resonant X-ray scattering to demonstrate 3D-CO in underdoped YBa2Cu3O6+x films grown epitaxially on SrTiO3 in the absence of magnetic fields. The resonance profiles indicate that Cu sites in the charge-reservoir layers participate in the CO state, and thus efficiently transmit CO correlations between adjacent CuO2 bilayer units. The results offer fresh perspectives for experiments elucidating the influence of 3D-CO on the electronic properties of cuprates without the need to apply high magnetic fields.
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- 2018
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15. Coupled Cu and Mn charge and orbital orders in YBa₂Cu₃O₇/Nd 0.65 (Ca 1-y Sr y ) 0.35 MnO₃ multilayers
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Perret, Edith, Monney, Claude, Johnston, S., Khmaladze, Jarji, Lyzwa, Fryderyk, Gaina, Roxana, Dantz, M., Pelliciari, Jonathan, Piamonteze, C., Mallett, B.P.P., Minola, M., Keimer, B., Schmitt, Thorsten, and Bernhard, Christian
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The observation of a charge density wave in the underdoped cuprate high Tc superconductors (Cu-CDW) raised a debate about its relationship with superconductivity. In bulk YBa2Cu3O7−δ the Cu-CDW is incipient and mainly pinned by defects. Nevertheless, a large magnetic field can induce a true long-range Cu- CDW order as it suppresses superconductivity. An enhanced Cu-CDW order was also observed in YBa2Cu3O7/La2/3Ca1/3MnO3 multilayers. Here, we show that the magnitude of the Cu-CDW in YBa2Cu3O7−δ / Nd0.65(Ca1-ySry)0.35MnO3 multilayers can be varied by adjusting the strength of the manganite charge and orbital order via the Sr content (tolerance factor). Furthermore, we resolve the reconstruction of the crystal field levels of the interfacial Cu ions that are also affected by the manganite charge and orbital order. This tuneable interfacial coupling and Cu- CDW in YBa2Cu3O7−δ can be used for studying the relationship between the Cu- CDW and superconductivity and, possibly, for inducing new intertwined quantum states.
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- 2018
16. Light-Induced Metastable State in Charge-Ordered YBa$_2$Cu$_3$O$_{6+x}$
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Gretarsson, H., Souliou, S. M., Jeong, S., Porras, J., Loew, T., Bluschke, M., Minola, M., Keimer, B., and Tacon, M. Le
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Superconductivity (cond-mat.supr-con) ,Condensed Matter - Superconductivity ,FOS: Physical sciences - Abstract
We report temporal changes in Raman-scattering spectra of detwinned YBa$_2$Cu$_3$O$_{6+x}$ single crystals under exposure to red laser light polarized along the crystallographic $a$-axis. A recent publication by Bakr et al. (Phys. Rev. B 88 214517 (2013)) identified new Raman-active modes that appear upon cooling below $T \sim 200$ K, and attributed these modes to charge ordering phenomena observed in x-ray scattering and nuclear magnetic resonance experiments on the same materials. Here we report that the intensities of these modes depend not only on temperature and oxygen content, but also on the cumulative photon dose absorbed by the YBa$_2$Cu$_3$O$_{6+x}$ samples. The light-induced changes in the Raman spectra exhibit a stretched-exponential time dependence, with a characteristic time that increases strongly upon cooling. They also depend strongly on doping and are most pronounced for $x \sim 0.6$. In fully illuminated samples, the mode intensities exhibit a monotonic temperature dependence indicative of a second-order phase transition. The findings indicate a metastable state generated by light-induced rearrangement of the oxygen dopants. We hypothesize that the new Raman phonons are associated with a three-dimensional charge-ordered state induced by light illumination, analogous to a state that was recently observed by resonant x-ray scattering in oxygen-disordered YBa$_2$Cu$_3$O$_{6+x}$ films., 8 pages and 5 figures. Manuscript to be published in Physical Review B
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- 2018
17. Dispersion, damping, and intensity of spin excitations in the single-layer (Bi,Pb)$_{2}$(Sr,La)$_{2}$CuO$_{6+\delta}$ cuprate superconductor family
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Peng, Y. Y., Huang, E. W., Fumagalli, R., Minola, M., Wang, Y., Sun, X., Ding, Y., Kummer, K., Zhou, X. J., Brookes, N. B., Moritz, B., Braicovich, L., Devereaux, T. P., and Ghiringhelli, G.
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Condensed Matter::Superconductivity ,Condensed Matter - Superconductivity ,Condensed Matter::Strongly Correlated Electrons - Abstract
Using Cu-$L_3$ edge resonant inelastic x-ray scattering (RIXS) we measured the dispersion and damping of spin excitations (magnons and paramagnons) in the high-$T_\mathrm{c}$ superconductor (Bi,Pb)$_{2}$(Sr,La)$_{2}$CuO$_{6+\delta}$ (Bi2201), for a large doping range across the phase diagram ($0.03\lesssim p\lesssim0.21$). Selected measurements with full polarization analysis unambiguously demonstrate the spin-flip character of these excitations, even in the overdoped sample. We find that the undamped frequencies increase slightly with doping for all accessible momenta, while the damping grows rapidly, faster in the (0,0)$\rightarrow$(0.5,0.5) nodal direction than in the (0,0)$\rightarrow$(0.5,0) antinodal direction. We compare the experimental results to numerically exact determinant quantum Monte Carlo (DQMC) calculations that provide the spin dynamical structure factor $S(\textbf{Q},\omega)$ of the three-band Hubbard model. The theory reproduces well the momentum and doping dependence of the dispersions and spectral weights of magnetic excitations. These results provide compelling evidence that paramagnons, although increasingly damped, persist across the superconducting dome of the cuprate phase diagram; this implies that long range antiferromagnetic correlations are quickly washed away, while short range magnetic interactions are little affected by doping., Comment: 11 pages, 9 figures
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- 2018
18. Dispersion, damping, and intensity of spin excitations in the single-layer (Bi,Pb)$_{2}$(Sr,La)$_{2}$CuO$_{6+��}$ cuprate superconductor family
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Peng, Y. Y., Huang, E. W., Fumagalli, R., Minola, M., Wang, Y., Sun, X., Ding, Y., Kummer, K., Zhou, X. J., Brookes, N. B., Moritz, B., Braicovich, L., Devereaux, T. P., and Ghiringhelli, G.
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Superconductivity (cond-mat.supr-con) ,Condensed Matter::Superconductivity ,FOS: Physical sciences ,Condensed Matter::Strongly Correlated Electrons - Abstract
Using Cu-$L_3$ edge resonant inelastic x-ray scattering (RIXS) we measured the dispersion and damping of spin excitations (magnons and paramagnons) in the high-$T_\mathrm{c}$ superconductor (Bi,Pb)$_{2}$(Sr,La)$_{2}$CuO$_{6+��}$ (Bi2201), for a large doping range across the phase diagram ($0.03\lesssim p\lesssim0.21$). Selected measurements with full polarization analysis unambiguously demonstrate the spin-flip character of these excitations, even in the overdoped sample. We find that the undamped frequencies increase slightly with doping for all accessible momenta, while the damping grows rapidly, faster in the (0,0)$\rightarrow$(0.5,0.5) nodal direction than in the (0,0)$\rightarrow$(0.5,0) antinodal direction. We compare the experimental results to numerically exact determinant quantum Monte Carlo (DQMC) calculations that provide the spin dynamical structure factor $S(\textbf{Q},��)$ of the three-band Hubbard model. The theory reproduces well the momentum and doping dependence of the dispersions and spectral weights of magnetic excitations. These results provide compelling evidence that paramagnons, although increasingly damped, persist across the superconducting dome of the cuprate phase diagram; this implies that long range antiferromagnetic correlations are quickly washed away, while short range magnetic interactions are little affected by doping., 11 pages, 9 figures
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- 2018
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19. Coupling between dynamic magnetic and charge-order correlations in the cuprate superconductor Nd$_{2-x}$Ce$_{x}$CuO$_4$
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Neto, E. H. da Silva, Minola, M., Yu, B., Tabis, W., Bluschke, M., Unruh, D., Suzuki, H., Li, Y., Yu, G., Betto, D., Kummer, K., Yakhou, F., Brookes, N. B., Tacon, M. Le, Greven, M., Keimer, B., and Damascelli, A.
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Superconductivity (cond-mat.supr-con) ,Condensed Matter - Strongly Correlated Electrons ,Strongly Correlated Electrons (cond-mat.str-el) ,Condensed Matter - Superconductivity ,Condensed Matter::Superconductivity ,FOS: Physical sciences ,Condensed Matter::Strongly Correlated Electrons - Abstract
Charge order has now been observed in several cuprate high-temperature superconductors. We report a resonant inelastic x-ray scattering experiment on the electron-doped cuprate Nd$_{2-x}$Ce$_{x}$CuO$_4$ that demonstrates the existence of dynamic correlations at the charge order wave vector. Upon cooling we observe a softening in the electronic response, which has been predicted to occur for a d-wave charge order in electron-doped cuprates. At low temperatures, the energy range of these excitations coincides with that of the dispersive magnetic modes known as paramagnons. Furthermore, measurements where the polarization of the scattered photon is resolved indicate that the dynamic response at the charge order wave vector primarily involves spin-flip excitations. Overall, our findings indicate a coupling between dynamic magnetic and charge-order correlations in the cuprates., Comment: Supplementary information available upon request
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- 2018
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20. Coincident onset of charge density wave order at a quantum critical point in underdoped YBCO
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Jang, H., Lee, W. -S., Song, S., Nojiri, H., Matsuzawa, S., Yasumura, H., Huang, H., Liu, Y. -J., Porras, J., Minola, M., Keimer, B., Hastings, J., Zhu, D., Devereaux, T. P., Shen, Z. -X., Kao, C. -C., and Lee, J. -S.
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Superconductivity (cond-mat.supr-con) ,Condensed Matter - Superconductivity ,Condensed Matter::Superconductivity ,FOS: Physical sciences ,Condensed Matter::Strongly Correlated Electrons - Abstract
The recently demonstrated x-ray scattering approach using a free electron laser with a high field pulsed magnet has opened new opportunities to explore the charge density wave (CDW) order in cuprate high temperature superconductors. Using this approach, we substantially degrade the superconductivity with magnetic fields up to 33 T to investigate the onset of CDW order in YBa$_2$Cu$_3$O$_x$ at low temperatures near a putative quantum critical point (QCP) at $p_1\sim $ 0.08 holes per Cu. We find no CDW can be detected in a sample with a doping concentration less than $p_1$. Our results indicate that the onset of the CDW ground state lies inside the zero-field superconducting dome, and broken translational symmetry is associated with the putative QCP at $p_1$, Comment: 4 figures
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- 2018
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21. Coupling between dynamic magnetic and charge order correlations in the cuprate superconductor Nd2 xCexCuO4
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Da Silva Neto, E., Minola, M., Yu, B., Tabis, W., Bluschke, M., Unruh, D., Suzuki, H., Li, Y., Yu, G., Betto, D., Kummer, K., Yakhou, F., Brookes, N., Le Tacon, M., Greven, M., Keimer, B., and Damascelli, A.
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charge order ,stripes ,cuprates ,Strongly correlated systems - Abstract
Charge order has now been observed in several cuprate high temperature superconductors. We report a resonant inelastic x ray scattering experiment on the electron doped cuprate Nd2 amp; 8722;xCexCuO4 that demonstrates the existence of dynamic correlations at the charge order wave vector. Upon cooling we observe a softening in the electronic response, which has been predicted to occur for a d wave charge order in electron doped cuprates. At low temperatures, the energy range of these excitations coincides with that of the dispersive magnetic modes known as paramagnons. Furthermore, measurements where the polarization of the scattered photon is resolved indicate that the dynamic response at the charge order wave vector primarily involves spin flip excitations. Overall, our findings indicate a coupling between dynamic magnetic and charge order correlations in the cuprates
- Published
- 2018
22. Raman scattering study of vibrational and magnetic excitations in Sr$_{2-x}$La$_x$IrO$_4$
- Author
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Gretarsson, H., Sauceda, J., Sung, N. H., H��ppner, M., Minola, M., Kim, B. J., Keimer, B., and Tacon, M. Le
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Condensed Matter::Materials Science ,Condensed Matter - Strongly Correlated Electrons ,Strongly Correlated Electrons (cond-mat.str-el) ,Condensed Matter::Superconductivity ,FOS: Physical sciences ,Condensed Matter::Strongly Correlated Electrons - Abstract
We have measured the doping and temperature dependence of lattice vibrations and magnetic excitations in the prototypical doped spin-orbit Mott insulator Sr$_{2-x}$La$_x$IrO$_4$ (x=0, 0.015, and 0.10). Our findings show that the pseudospin-lattice coupling -- responsible for the renormalization of several low energy phonon modes -- is preserved even when long-range magnetic order is suppressed by doping. In our most highly doped sample, the single magnon (Gamma-point) excitation disappears while the two-magnon mode softens and becomes heavily damped. Doping induced electron-phonon coupling is also observed in a higher energy phonon mode. We observe two different electron-phonon interaction channels, which provide evidence of the coexistence of fluctuating magnetic moments and mobile carriers in doped iridates., 9 pages, 9 figures
- Published
- 2017
23. Re-entrant charge order in overdoped (Bi,Pb)$_{2.12}$Sr$_{1.88}$CuO$_{6+��}$ outside the pseudogap regime
- Author
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Peng, Y. Y., Fumagalli, R., Ding, Y., Minola, M., Caprara, S., Betto, D., De Luca, G. M., Kummer, K., Lefran��ois, E., Salluzzo, M., Suzuki, H., Tacon, M. Le, Zhou, X. J., Brookes, N. B., Keimer, B., Braicovich, L., Grilli, M., and Ghiringhelli, G.
- Subjects
Superconductivity (cond-mat.supr-con) ,Condensed Matter::Superconductivity ,FOS: Physical sciences ,Condensed Matter::Strongly Correlated Electrons - Abstract
Charge modulations are considered as a leading competitor of high-temperature superconductivity in the underdoped cuprates, and their relationship to Fermi surface reconstructions and to the pseudogap state is an important subject of current research. Overdoped cuprates, on the other hand, are widely regarded as conventional Fermi liquids without collective electronic order. For the overdoped (Bi,Pb)2.12Sr1.88CuO6+�� (Bi2201) high-temperature superconductor, here we report resonant x-ray scattering measurements revealing incommensurate charge order reflections, with correlation lengths of 40-60 lattice units, that persist up to at least 250K. Charge order is markedly more robust in the overdoped than underdoped regime but the incommensurate wave vectors follow a common trend; moreover it coexists with a single, unreconstructed Fermi surface, without pseudogap or nesting features, as determined from angle-resolved photoemission spectroscopy. This re-entrant charge order is reproduced by model calculations that consider a strong van Hove singularity within a Fermi liquid framework., 11 pages, 5 figures
- Published
- 2017
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24. Crossover from Collective to Incoherent Spin Excitations in Superconducting Cuprates Probed by Detuned Resonant Inelastic X-ray Scattering
- Author
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Minola, M., Lu, Y., Peng, Y. Y., Dellea, G., Gretarsson, H., Haverkort, M. W., Ding, Y., Sun, X., Zhou, X. J., Peets, D. C., Chauviere, L., Dosanjh, P., Bonn, D. A., Liang, R., Damascelli, A., Brookes, N. B., Yakhou, F., Pelliciari, J., Dantz, M., Lu, X., Schmitt, T., Braicovich, L., Ghiringhelli, G., Keimer, B., and Tacon, M. Le
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Physics ,Quantum phase transition ,Superconductivity ,Condensed matter physics ,Hubbard model ,Scattering ,Condensed Matter - Superconductivity ,superconductivity ,General Physics and Astronomy ,FOS: Physical sciences ,02 engineering and technology ,Photon energy ,021001 nanoscience & nanotechnology ,01 natural sciences ,Resonant inelastic X-ray scattering ,Superconductivity (cond-mat.supr-con) ,Physics and Astronomy (all) ,Condensed Matter::Superconductivity ,0103 physical sciences ,Cuprate ,Condensed Matter::Strongly Correlated Electrons ,Atomic physics ,010306 general physics ,0210 nano-technology ,Spin-½ - Abstract
Spin excitations in the overdoped high temperature superconductors Tl$_2$Ba$_2$CuO$_{6+\delta}$ and (Bi,Pb)$_2$(Sr,La)$_{2}$CuO$_{6+\delta}$ were investigated by resonant inelastic x-ray scattering (RIXS) as functions of doping and detuning of the incoming photon energy above the Cu-$L_3$ absorption peak. The RIXS spectra at optimal doping are dominated by a paramagnon feature with peak energy independent of photon energy, similar to prior results on underdoped cuprates. Beyond optimal doping, the RIXS data indicate a sharp crossover to a regime with a strong contribution from incoherent particle/hole excitations whose maximum shows a fluorescence-like shift upon detuning. The spectra of both compound families are closely similar, and their salient features are reproduced by exact-diagonalization calculations of the single-band Hubbard model on a finite cluster. The results are discussed in the light of recent transport experiments indicating a quantum phase transition near optimal doping., Comment: 6 pages, 3 figures, accepted in Physical Review Letters
- Published
- 2017
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- View/download PDF
25. Prevention of serious vascular events by aspirin amongst patients with peripheral arterial disease: randomized, double-blind trial
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Fabris, F., Pilger, E., Pabst, E., Kostner, G., Wautrecht, J. C., Baitsch, G., Breddin, K., Diehm, C., Podhaisky, H., Taute, B. M., Diamantoupolos, E. J., Aimar, T., Alari, G., Albano, S., Altamura, N., Arosio, E., Bortolon, M., Caccia, R., Carotta, M., Carzaniga, G., Catalano, M., Contini, P., Difolca, A., Dore, M., Falaschi, F., Franchini, B., Frare, C., Frascisco, M., Giansante, C., Giona, E., Giubbolini, M., Lucarelli, F., Marchitelli, E., Marcialis, M. R., Martignoni, A., Melillo, E., Minola, M., Monetti, D., Nenci, G., Paolicelli, M., Pasqualini, L., Perilli, E., Pettina, G., Poli, L., Radicchia, S., Rossi, M., Scandale, G., Scondotto, G., Sergi, D., Setacci, C., Spada, S., Todini, A. R., Vaudo, G., Verlato, F., Visona, A., Zannoni, M., Bielawiec, M., Jawien, A., Meissner, A., Michalak, J., Nizankowski, R., Wandzilak, M., Avram, J. A., Avram, R., Hancu, N., Marian, A., Marian, I., Murariu, M., Negrisanu, G., Olinic, D., Olinic, N., Trambitas, R., Veresiu, I., Victoria, I., Kozak, M., Mavri, A., Bahi, J. S., Bahi, P. S., Brunkwall, J., and Gallino, A.
- Subjects
Male ,medicine.medical_specialty ,Settore MED/09 - Medicina Interna ,Placebo ,law.invention ,Double-Blind Method ,Randomized controlled trial ,Ischemia ,law ,Internal medicine ,Internal Medicine ,medicine ,Humans ,Myocardial infarction ,Stroke ,Aged ,Angiology ,Peripheral Vascular Diseases ,Leg ,Aspirin ,Vascular disease ,business.industry ,Antioxidant vitamins ,Peripheral arterial disease ,Prevention ,medicine.disease ,Surgery ,Clinical trial ,Treatment Outcome ,Female ,business ,Platelet Aggregation Inhibitors ,medicine.drug - Abstract
OBJECTIVE: To assess the prophylactic efficacy of aspirin and a high-dose antioxidant vitamin combination in patients with peripheral arterial disease (PAD) in terms of reduction of the risk of a first vascular event (myocardial infarction, stroke, vascular death) and critical limb ischaemia. DESIGN: Randomized, placebo-controlled, double-blind clinical trial with 2 x 2 factorial design. SETTING: Thirty-seven European angiology/vascular medicine units. SUBJECTS: A total of 366 outpatients with stage I-II PAD documented by angiography or ultrasound, with ankle/brachial index
- Published
- 2007
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26. Origin of interface magnetism in BiMnO3/SrTiO3 and LaAlO3/SrTiO3 heterostructures
- Author
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Salluzzo, M., Gariglio, S., Stornaiuolo, D., Sessi, V., Rusponi, S., Piamonteze, C., De Luca, G. M., Minola, M., Marré, D., Gadaleta, A., Brune, H., Nolting, F., Brookes, N. B., Ghiringhelli, G., Salluzzo, M., Gariglio, S., Stornaiuolo, D., Sessi, V., Rusponi, S., Piamonteze, C., De Luca, G. M., Minola, M., Marre, D., Gadaleta, A., Brune, H., Nolting, F., Brookes, N. B., and Ghiringhelli, G.
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Condensed Matter::Materials Science ,Condensed Matter - Strongly Correlated Electrons ,Condensed Matter - Materials Science ,Strongly Correlated Electrons (cond-mat.str-el) ,Materials Science (cond-mat.mtrl-sci) ,FOS: Physical sciences ,ddc:500.2 - Abstract
Possible ferromagnetism induced in otherwise non-magnetic materials has been motivating intense research in complex oxide heterostructures. Here we show that a confined magnetism is realized at the interface between SrTiO3 and two insulating polar oxides, BiMnO3 and LaAlO3. By using polarization dependent x-ray absorption spectroscopy, we find that in both cases the magnetic order is stabilized by a negative exchange interaction between the electrons transferred to the interface and local magnetic moments. These local magnetic moments are associated to Ti3+ ions at the interface itself for LaAlO3/SrTiO3 and to Mn3+ ions in the overlayer for BiMnO3/SrTiO3. In LaAlO3/SrTiO3 the induced magnetic moments are quenched by annealing in oxygen, suggesting a decisive role of oxygen vacancies in the stabilization of interfacial magnetism., 5 pages, 4 figures
- Published
- 2013
27. Magnetic excitations and phonons simultaneously studied by resonant inelastic x-ray scattering in optimally doped Bi$_{1.5}$Pb$_{0.55}$Sr$_{1.6}$La$_{0.4}$CuO$_{6+\delta}$
- Author
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Peng, Y. Y., Hashimoto, M., Sala, M. Moretti, Amorese, A., Brookes, N. B., Dellea, G., Lee, W. -S., Minola, M., Schmitt, T., Yoshida, Y., Zhou, K. -J., Eisaki, H., Devereaux, T. P., Shen, Z. -X., Braicovich, L., and Ghiringhelli, G.
- Subjects
Condensed Matter::Superconductivity ,Condensed Matter - Superconductivity ,Condensed Matter::Strongly Correlated Electrons - Abstract
Magnetic excitations in the optimally doped high-$T_\mathrm{c}$ superconductor Bi$_{1.5}$Pb$_{0.55}$Sr$_{1.6}$La$_{0.4}$CuO$_{6+\delta}$ (OP-Bi2201, $T_\mathrm{c}\simeq 34$ K) are investigated by Cu $L_3$ edge resonant inelastic x-ray scattering (RIXS), below and above the pseudogap opening temperature. At both temperatures the broad spectral distribution disperses along the (1,0) direction up to $\sim$350~meV at zone boundary, similarly to other hole-doped cuprates. However, above $\sim$0.22 reciprocal lattice units, we observe a concurrent intensity decrease for magnetic excitations and quasi-elastic signals with weak temperature dependence. This anomaly seems to indicate a coupling between magnetic, lattice and charge modes in this compound. We also compare the magnetic excitation spectra near the anti-nodal zone boundary in the single layer OP-Bi2201 and in the bi-layer optimally doped Bi$_{1.5}$Pb$_{0.6}$Sr$_{1.54}$CaCu$_2$O$_{8+\delta}$ (OP-Bi2212, $T_\mathrm{c}\simeq96$ K). The strong similarities in the paramagnon dispersion and in their energy at zone boundary indicate that the strength of the super-exchange interaction and the short-range magnetic correlation cannot be directly related to $T_\mathrm{c}$, not even within the same family of cuprates.
- Published
- 2015
28. Recent Reactivation of a Miocene Fold-and-Thrust Belt (Northern Apennines, Italy). Implications for the Petroleum System
- Author
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PICOTTI, VINCENZO, CAPOZZI, ROSSELLA, OPPO, DAVIDE, PONZA, ALESSIO, Minola M., Terazzi F., Picotti V., Capozzi R., Minola M., Terazzi F., Oppo D., and Ponza A.
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PETROLEUM SYSTEM ,Northern Apennine - Published
- 2011
29. Momentum and polarization dependence of single-magnon spectral weight for Cu L3 -edge resonant inelastic x-ray scattering from layered cuprates
- Author
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Braicovich L., Moretti Sala M., Ament L. J. P., Bisogni V., Minola M., Balestrino G., Di Castro D., De Luca G. M., Salluzzo M., Ghiringhelli G., Van Den Brink J., Braicovich, L., Moretti Sala, M., Ament, L. J. P., Bisogni, V., Minola, M., Balestrino, G., Di Castro, D., De Luca, G. M., Salluzzo, M., Ghiringhelli, G., and Van Den Brink, J.
- Published
- 2010
30. Resonant X-ray Scattering Study of Charge Density Wave Correlations in YBa$_2$Cu$_3$O$_{6+x}$
- Author
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Blanco-Canosa, S., Frano, A., Schierle, E., Porras, J., Loew, T., Minola, M., Bluschke, M., Weschke, E., Keimer, B., and Tacon, M. Le
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Superconductivity (cond-mat.supr-con) ,Condensed Matter - Strongly Correlated Electrons ,Strongly Correlated Electrons (cond-mat.str-el) ,Condensed Matter - Superconductivity ,Condensed Matter::Superconductivity ,FOS: Physical sciences ,Condensed Matter::Strongly Correlated Electrons - Abstract
We report the results a comprehensive study of charge density wave (CDW) correlations in untwinned YBCO6+x single crystals with 0.4 0.09) an enhancement of the signal when an external magnetic field up to 6 T is applied in the superconducting state. For samples with p~0.08, where prior work has revealed a field-enhancement of incommensurate magnetic order, the RXS signal is field-independent. This supports a previously suggested scenario in which incommensurate charge and spin orders compete against each other, in addition to individually competing against. We discuss the relationship of these results to stripe order 214, the pseudogap phenomenon, superconducting fluctuations, and quantum oscillations., Comment: revised version. To appear in Phys. Rev. B
- Published
- 2014
- Full Text
- View/download PDF
31. Orbital occupancies and the putative jeff=1/2 ground state in Ba2IrO4: A combined oxygen K-edge XAS and RIXS study
- Author
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Sala, M. Moretti, Rossi, M., Boseggia, S., Akimitsu, J., Brookes, N. B., Isobe, M., Minola, M., Okabe, H., Ronnow, H. M., Simonelli, L., McMorrow, D. F., and Monaco, G.
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Condensed Matter - Strongly Correlated Electrons ,Strongly Correlated Electrons (cond-mat.str-el) ,MPBH ,FOS: Physical sciences ,Condensed Matter::Strongly Correlated Electrons - Abstract
The nature of the electronic groundstate of Ba2IrO4 has been addressed using soft X-ray absorption and inelastic scattering techniques in the vicinity of the oxygen K edge. From the polarization and angular dependence of XAS we deduce an approximately equal superposition of xy, yz and zx Ir4+ 5d orbitals. By combining the measured orbital occupancies, with the value of the spin-orbit coupling provided by RIXS, we estimate the crystal field splitting associated with the tetragonal distortion of the IrO6 octahedra to be small, \Delta=50(50) meV. We thus conclude definitively that Ba2IrO4 is a close realization of a spin-orbit Mott insulator with a jeff = 1/2 groundstate, thereby overcoming ambiguities in this assignment associated with the interpretation of X-ray resonant scattering experiments., Comment: 5 pages, 5 figures
- Published
- 2014
32. Connection between charge-density-wave order and charge transport in the cuprate superconductors
- Author
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Tabis, W., Li, Y., Tacon, M. Le, Braicovich, L, Kreyssig, A., Minola, M., Dellea, G., Weschke, E., Veit, M. J., Ramazanoglu, M., Goldman, A. I., Schmitt, T., Ghiringhelli, G., Barišić, N., Chan, M. K., Dorow, C. J., Yu, G., Zhao, X., Keimer, B., and Greven, M.
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Superconductivity (cond-mat.supr-con) ,Condensed Matter - Superconductivity ,Condensed Matter::Superconductivity ,FOS: Physical sciences ,Condensed Matter::Strongly Correlated Electrons - Abstract
Charge-density-wave (CDW) correlations within the quintessential CuO$_2$ planes have been argued to either cause [1] or compete with [2] the superconductivity in the cuprates, and they might furthermore drive the Fermi-surface reconstruction in high magnetic fields implied by quantum oscillation (QO) experiments for YBa$_2$Cu$_3$O$_{6+{\delta}}$ (YBCO) [3] and HgBa$_2$CuO$_{4+{\delta}}$ (Hg1201) [4]. Consequently, the observation of bulk CDW order in YBCO was a significant development [5,6,7]. Hg1201 features particularly high structural symmetry and recently has been demonstrated to exhibit Fermi-liquid charge transport in the relevant temperature-doping range of the phase diagram, whereas for YBCO and other cuprates this underlying property of the CuO$_2$ planes is partially or fully masked [8-10]. It therefore is imperative to establish if the pristine transport behavior of Hg1201 is compatible with CDW order. Here we investigate Hg1201 ($T_c$ = 72 K) via bulk Cu L-edge resonant X-ray scattering. We indeed observe CDW correlations in the absence of a magnetic field, although the correlations and competition with superconductivity are weaker than in YBCO. Interestingly, at the measured hole-doping level, both the short-range CDW and Fermi-liquid transport appear below the same temperature of about 200 K. Our result points to a unifying picture in which the CDW formation is preceded at the higher pseudogap temperature by $q$ = 0 magnetic order [11,12] and the build-up of significant dynamic antiferromagnetic correlations [13]. Furthermore, the smaller CDW modulation wave vector observed for Hg1201 is consistent with the larger electron pocket implied by both QO [4] and Hall-effect [14] measurements, which suggests that CDW correlations are indeed responsible for the low-temperature QO phenomenon.
- Published
- 2014
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33. Measurement of the effect of lattice strain on magnetic interactions and orbital splitting in CaCuO_{2} using resonant inelastic x-ray scattering
- Author
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Minola, M, Hozoi, L, DI CASTRO, D, Felici, R, Moretti Sala, M, Tebano, A, Balestrino, G, Ghiringhelli, G, Van Den Brink, J, and Braicovich, L
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Settore FIS/03 - Fisica della Materia - Published
- 2013
34. Magnetic excitations in stripe-ordered La_{1.875}Ba_{0.125}CuO_{4} studied using resonant inelastic x-ray scattering
- Author
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Dean, M. P. M., Dellea, G., Minola, M., Wilkins, S. B., Konik, R. M., Gu, G. D., Tacon, M. Le, Brookes, N. B., Yakhou-Harris, F., Kummer, K., Hill, J. P., Braicovich, L., and Ghiringhelli, G.
- Subjects
Superconductivity (cond-mat.supr-con) ,Condensed Matter - Materials Science ,Condensed Matter - Strongly Correlated Electrons ,Strongly Correlated Electrons (cond-mat.str-el) ,Condensed Matter - Superconductivity ,Materials Science (cond-mat.mtrl-sci) ,FOS: Physical sciences - Abstract
The charge and spin correlations in La$_{1.875}$Ba$_{0.125}$CuO$_4$ (LBCO 1/8) are studied using Cu $L_3$ edge resonant inelastic x-ray scattering (RIXS). The static charge order (CO) is observed at a wavevector of $(0.24,0)$ and its charge nature confirmed by measuring the dependence of this peak on the incident x-ray polarization. The paramagnon excitation in LBCO 1/8 is then measured as it disperses through the CO wavevector. Within the experimental uncertainty no changes are observed in the paramagnon due to the static CO, and the paramagnon seems to be similar to that measured in other cuprates, which have no static CO. Given that the stripe correlation modulates both the charge and spin degrees of freedom, it is likely that subtle changes do occur in the paramagnon due to CO. Consequently, we propose that future RIXS measurements, realized with higher energy resolution and sensitivity, should be performed to test for these effects., 5 pages, 4 figures
- Published
- 2013
35. Momentum-dependent charge correlations in YBa$_2$Cu$_3$O$_{6+\delta}$ superconductors probed by resonant x-ray scattering: Evidence for three competing phases
- Author
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Blanco-Canosa, S., Frano, A., Loew, T., Lu, Y., Porras, J., Ghiringhelli, G., Minola, M., Mazzoli, C., Braicovich, L., Schierle, E., Weschke, E., Tacon, M. Le, and Keimer, B.
- Subjects
Condensed Matter - Strongly Correlated Electrons ,Condensed Matter::Superconductivity ,Condensed Matter - Superconductivity ,Condensed Matter::Strongly Correlated Electrons - Abstract
We have used resonant x-ray scattering to determine the momentum dependent charge correlations in YBa$_2$Cu$_3$O$_{6.55}$ samples with highly ordered chain arrays of oxygen acceptors (ortho-II structure). The results reveal nearly critical, biaxial charge density wave (CDW) correlations at in-plane wave vectors (0.315, 0) and (0, 0.325). The corresponding scattering intensity exhibits a strong uniaxial anisotropy. The CDW amplitude and correlation length are enhanced as superconductivity is weakened by an external magnetic field. Analogous experiments were carried out on a YBa$_2$Cu$_3$O$_{6.6}$ crystal with a dilute concentration of spinless (Zn) impurities, which had earlier been shown to nucleate incommensurate magnetic order. Compared to pristine crystals with the same doping level, the CDW amplitude and correlation length were found to be strongly reduced. These results indicate a three-phase competition between spin-modulated, charge-modulated, and superconducting states in underdoped YBa$_2$Cu$_3$O$_{6+\delta}$., Comment: 6 pages, 3 figures revised version, to appear in Phys. Rev. Lett
- Published
- 2012
36. Occurrence of a high-temperature superconducting phase in (CaCuO 2 ) n /(SrTiO 3 ) m superlattices
- Author
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Di Castro, D., Salvato, M., Tebano, A., Innocenti, D., Aruta, C., Prellier, Wilfrid, Lebedev, O., Ottaviani, I., Brookes, N., Minola, M., Moretti Sala, M., Mazzoli, C., Medaglia, P., Ghiringhelli, G., Braicovich, L., Cirillo, M., Balestrino, G., Università degli Studi di Roma Tor Vergata [Roma], Dipartimento di Scienze Fisiche [Naples], University of Naples Federico II = Università degli studi di Napoli Federico II, Laboratoire de cristallographie et sciences des matériaux (CRISMAT), Université de Caen Normandie (UNICAEN), Normandie Université (NU)-Normandie Université (NU)-École Nationale Supérieure d'Ingénieurs de Caen (ENSICAEN), Normandie Université (NU)-Institut de Chimie du CNRS (INC)-Centre National de la Recherche Scientifique (CNRS)-Institut de Recherche sur les Matériaux Avancés (IRMA), Normandie Université (NU)-Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Université de Rouen Normandie (UNIROUEN), Normandie Université (NU)-Institut national des sciences appliquées Rouen Normandie (INSA Rouen Normandie), Institut National des Sciences Appliquées (INSA)-Normandie Université (NU)-Institut National des Sciences Appliquées (INSA)-Centre National de la Recherche Scientifique (CNRS)-Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Université de Rouen Normandie (UNIROUEN), Institut National des Sciences Appliquées (INSA)-Normandie Université (NU)-Institut National des Sciences Appliquées (INSA)-Centre National de la Recherche Scientifique (CNRS), European Synchrotron Radiation Facility (ESRF), Politecnico di Milano [Milan] (POLIMI), Max-Planck-Institut für Extraterrestrische Physik (MPE), Università degli studi di Napoli Federico II, École Nationale Supérieure d'Ingénieurs de Caen (ENSICAEN), Normandie Université (NU)-Normandie Université (NU)-Centre National de la Recherche Scientifique (CNRS)-Université de Caen Normandie (UNICAEN), Normandie Université (NU)-Institut de Chimie du CNRS (INC), and CNR/SPIN and Dipartimento di Fisica
- Subjects
[PHYS]Physics [physics] ,[CHIM]Chemical Sciences ,[CHIM.MATE]Chemical Sciences/Material chemistry ,ComputingMilieux_MISCELLANEOUS - Abstract
International audience; We report the occurrence of superconductivity, with maximum Tc=40 K, in superlattices (SLs) based on two insulating oxides, namely CaCuO2 and SrTiO3. In these (CaCuO2)n/(SrTiO3)m SLs, the CuO2 planes belong only to CaCuO2 block, which is an antiferromagnetic insulator. Superconductivity, confined within a few unit cells at the CaCuO2/SrTiO3 interface, shows up only when the SLs are grown in a highly oxidizing atmosphere, because of extra oxygen ions entering at the interfaces. The hole doping is obtained by charge transfer from the interface layers, which thus act as charge reservoir.
- Published
- 2012
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37. Distinct Charge Orders in the Planes and Chains of Ortho-III-Ordered YBa$_2$Cu$_3$O$_{6+\delta}$ Superconductors Identified by Resonant Elastic X-ray Scattering
- Author
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Achkar, A. J., Sutarto, R., Mao, X., He, F., Frano, A., Blanco-Canosa, S., Tacon, M. Le, Ghiringhelli, G., Braicovich, L., Minola, M., Sala, M. Moretti, Mazzoli, C., Liang, Ruixing, Bonn, D. A., Hardy, W. N., Keimer, B., Sawatzky, G. A., and Hawthorn, D. G.
- Subjects
Condensed Matter - Strongly Correlated Electrons ,Condensed Matter::Superconductivity ,Condensed Matter - Superconductivity ,Condensed Matter::Strongly Correlated Electrons - Abstract
Recently, charge density wave (CDW) order in the CuO$_2$ planes of underdoped YBa$_2$Cu$_3$O$_{6+\delta}$ was detected using resonant soft x-ray scattering. An important question remains: is the chain layer responsible for this charge ordering? Here, we explore the energy and polarization dependence of the resonant scattering intensity in a detwinned sample of YBa$_2$Cu$_3$O$_{6.75}$ with ortho-III oxygen ordering in the chain layer. We show that the ortho-III CDW order in the chains is distinct from the CDW order in the planes. The ortho-III structure gives rise to a commensurate superlattice reflection at $Q$=[0.33 0 $L$] whose energy and polarization dependence agrees with expectations for oxygen ordering and a spatial modulation of the Cu valence in the chains. Incommensurate peaks at [0.30 0 $L$] and [0 0.30 $L$] from the CDW order in the planes are shown to be distinct in $Q$ as well as their temperature, energy, and polarization dependence, and are thus unrelated to the structure of the chain layer. Moreover, the energy dependence of the CDW order in the planes is shown to result from a spatial modulation of energies of the Cu 2$p$ to 3$d_{x^2-y^2}$ transition, similar to stripe-ordered 214 cuprates., Comment: 5 pages, 3 figures
- Published
- 2012
38. Role of multiple electronic-valence elements in A-site manganites
- Author
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Orgiani, P., Galdi, Alice, Maritato, Luigi, Aruta, C., Cataudella, V., De Filippis, G., Perroni, A. C., Marigliano Ramaglia, V., Ciancio, Regina, Brookes, N., Minola, M., Moretti Sala, M., and Ghiringhelli, G.
- Published
- 2012
39. Multiple valence Mn-ions as novel approach for doping oxide manganites
- Author
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Orgiani, P., Galdi, Alice, Maritato, Luigi, Aruta, C., Cataudella, V., De Filippis, G., Perroni, A. C., Marigliano Ramaglia, V., Ciancio, Regina, Brookes, N., Minola, M., Moretti Sala, M., and Ghiringhelli, G.
- Published
- 2012
40. Multiple electronic-valence elements in A-site perovskite manganites: a route to high metallicity and an orbital order coexistence
- Author
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Orgiani, P., Aruta, C., Galdi, Alice, Cataudella, V., De Filippis, G., Perroni, C. A., Marigliano Ramaglia, V., Brookes, N. B., Minola, M., Moretti Sala, M., Ghiringhelli, G., and Maritato, Luigi
- Published
- 2012
41. Coexistence of high metallicity and orbital order in A-site manganites
- Author
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Orgiani, P., Galdi, Alice, Maritato, Luigi, Aruta, C., Cataudella, V., De Filippis, G., Perroni, A. C., Marigliano Ramaglia, V., Ciancio, Regina, Brookes, N., Minola, M., Moretti Sala, M., and Ghiringhelli, G.
- Published
- 2012
42. Occurrence of a high-temperature superconducting phase in (CaCuO2)n/(SrTiO3)m superlattices
- Author
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DI CASTRO, D, Salvato, M, Tebano, A, Innocenti, D, Aruta, C, Prellier, W, Lebedev, O, Ottaviani, I, Brookes, N, Minola, M, Sala, M, Mazzoli, C, Medaglia, Pg, Ghiringhelli, G, Braicovich, L, Cirillo, M, and Balestrino, G
- Subjects
Settore FIS/03 - Fisica della Materia - Published
- 2012
43. Momentum-dependent charge correlations in YBa$_2$Cu$_3$O$_{6+��}$ superconductors probed by resonant x-ray scattering: Evidence for three competing phases
- Author
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Blanco-Canosa, S., Frano, A., Loew, T., Lu, Y., Porras, J., Ghiringhelli, G., Minola, M., Mazzoli, C., Braicovich, L., Schierle, E., Weschke, E., Tacon, M. Le, and Keimer, B.
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Superconductivity (cond-mat.supr-con) ,Strongly Correlated Electrons (cond-mat.str-el) ,Condensed Matter::Superconductivity ,FOS: Physical sciences ,Condensed Matter::Strongly Correlated Electrons - Abstract
We have used resonant x-ray scattering to determine the momentum dependent charge correlations in YBa$_2$Cu$_3$O$_{6.55}$ samples with highly ordered chain arrays of oxygen acceptors (ortho-II structure). The results reveal nearly critical, biaxial charge density wave (CDW) correlations at in-plane wave vectors (0.315, 0) and (0, 0.325). The corresponding scattering intensity exhibits a strong uniaxial anisotropy. The CDW amplitude and correlation length are enhanced as superconductivity is weakened by an external magnetic field. Analogous experiments were carried out on a YBa$_2$Cu$_3$O$_{6.6}$ crystal with a dilute concentration of spinless (Zn) impurities, which had earlier been shown to nucleate incommensurate magnetic order. Compared to pristine crystals with the same doping level, the CDW amplitude and correlation length were found to be strongly reduced. These results indicate a three-phase competition between spin-modulated, charge-modulated, and superconducting states in underdoped YBa$_2$Cu$_3$O$_{6+��}$., 6 pages, 3 figures revised version, to appear in Phys. Rev. Lett
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- 2012
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44. High Tc superconductivity in superlattices of insulating oxides
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Di Castro, D., Salvato, M., Tebano, A., Innocenti, D., Aruta, C., Prellier, W., Lebedev, O. I., Ottaviani, I., Brookes, N. B., Minola, M., Sala, M. Moretti, Mazzoli, C., Medaglia, P. G., Ghiringhelli, G., Cirillo, L. Braicovich M., and Balestrino, G.
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Superconductivity (cond-mat.supr-con) ,Condensed Matter::Materials Science ,Condensed Matter - Superconductivity ,Condensed Matter::Superconductivity ,FOS: Physical sciences ,Condensed Matter::Strongly Correlated Electrons ,Physics::Chemical Physics - Abstract
We report the occurrence of superconductivity, with maximum Tc = 40 K, in superlattices (SLs) based on two insulating oxides, namely CaCuO2 and SrTiO3. In these (CaCuO2)n/(SrTiO3)m SLs, the CuO2 planes belong only to CaCuO2 block, which is an antiferromagnetic insulator. Superconductivity, confined within few unit cells at the CaCuO2/SrTiO3 interface, shows up only when the SLs are grown in a highly oxidizing atmosphere, because of extra oxygen ions entering at the interfaces. Evidence is reported that the hole doping of the CuO2 planes is obtained by charge transfer from the interface layers, which act as charge reservoir., Comment: 18 pages, 8 figures
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- 2011
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45. Bimagnon studies in cuprates with Resonant Inelastic X-ray Scattering at the O K edge. I - An assessment on La2CuO4 and a comparison with the excitation at Cu L3 and Cu K edges
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Bisogni, V., Simonelli, L., Ament, L. J. P., Forte, F., Sala, M. Moretti, Minola, M., Huotari, S., Brink, J. van den, Ghiringhelli, G., Brookes, N. B., and Braicovich, L.
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Superconductivity (cond-mat.supr-con) ,Condensed Matter - Strongly Correlated Electrons ,Strongly Correlated Electrons (cond-mat.str-el) ,Condensed Matter - Superconductivity ,FOS: Physical sciences ,Condensed Matter::Strongly Correlated Electrons - Abstract
We assess the capabilities of magnetic Resonant Inelastic X-ray Scattering (RIXS) at the O $K$ edge in undoped cuprates by taking La_{2}CuO_{4} as a benchmark case, based on a series of RIXS measurements that we present here. By combining the experimental results with basic theory we point out the fingerprints of bimagnon in the O $K$ edge RIXS spectra. These are a dominant peak around 450 meV, the almost complete absence of dispersion both with $\pi$ and $\sigma$ polarization and the almost constant intensity vs. the transferred momentum with $\sigma$ polarization. This behavior is quite different from Cu $L_3$ edge RIXS giving a strongly dispersing bimagnon tending to zero at the center of the Brillouin zone. This is clearly shown by RIXS measurements at the Cu $L_3$ edge that we present. The Cu $L_3$ bimagnon spectra and those at Cu $K$ edge - both from the literature and from our data - however, have the same shape. These similarities and differences are understood in terms of different sampling of the bimagnon continuum. This panorama points out the unique possibilities offered by O $K$ RIXS in the study of magnetic excitations in cuprates near the center of the BZ.
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- 2010
46. Momentum and polarization dependence of single-magnon spectral weight for Cu L3 -edge resonant inelastic x-ray scattering from layered cuprates
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Braicovich, L, Moretti Sala, M, Ament, L, Bisogni, V, Minola, M, Balestrino, G, DI CASTRO, D, De Luca, G, Salluzzo, M, Ghiringhelli, G, and van den Brink, J
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LA2CUO4 ,TRANSITION ,PURE ,Settore FIS/03 - Fisica della Materia - Published
- 2010
47. Prevention of serious vascular events by aspirin amongst patients with peripheral arterial disease: a randomized, double-blind trial
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Pilger, E, Pabst, E, Kostner, G, Wautrecht, Jc, Baitsch, G, Breddin, K, Diehm, C, Podhaisky, H, Taute, Bm, Diamantoupolos, Ej, Aimar, T, Alari, G, Albano, S, Altamura, N, Arosio, E, Bortolon, M, Caccia, R, Carotta, M, Carzaniga, G, Catalano, M, Contini, P, Difolca, A, Dore, M, Fabris, F, Falaschi, F, Franchini, B, Frare, C, Frascisco, M, Giansante, C, Giona, E, Giubbolini, M, Lucarelli, F, Marchitelli, E, Marcialis, Mr, Martignoni, A, Melillo, E, Minola, M, Monetti, D, Nenci, G, Paolicelli, M, Pasqualini, Leonella, Perilli, E, Pettina, G, Poli, L, Radicchia, S, Rossi, M, Scandale, G, Scondotto, G, Sergi, D, Setacci, C, Spada, S, Todini, Ar, Vaudo, Gaetano, Verlato, F, Visona, A, Zannoni, M, Bielawiec, M, Jawien, A, Meissner, A, Michalak, J, Nizankowski, R, Wandzilak, M, Avram, Ja, Avram, R, Hancu, N, Marian, A, Marian, I, Murariu, M, Negrisanu, G, Olinic, D, Olinic, N, Trambitas, R, Veresiu, I, Victoria, I, Kozak, M, Mavri, A, Bahi, Js, Bahi, Ps, Brunkwall, J, and Gallino, A.
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- 2007
48. Cateterismo vescicale: appropriatezza dell´uso ed esiti clinici nell´Azienda Sanitaria Ospedaliera 'Maggiore della Caritá' di Novara
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Luparia, M., Bonvini, D., Demarchi, M.L., Lanszweert, A., Minola, M., Renna, M., Sarasino, D., and Panella, M.
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lcsh:Public aspects of medicine ,lcsh:R ,DOAJ:Public Health ,lcsh:Medicine ,lcsh:RA1-1270 ,DOAJ:Health Sciences - Abstract
Obiettivi: valutare le relazioni intercorrenti tra i livelli di appropriatezza di indicazione e di gestione del cateterismo vescicale e lo sviluppo delle IVU.Materiali e metodi: studio descrittivo condotto in una giornata con rilevazione basata su cartelle cliniche ed infermieristiche. Le relazioni intercorrenti tra la cateterizzazione vescicale e l’insorgenza dell’IVU sono stati studiati mediante modelli di regressione logistica in grado di valutare l’appropriatezza del processo assistenziale e per identificare i determinanti dell’esitto. Risultati: nel giorno dell’indagine son risultati ricoverati 166 pazienti, di questi 57 (34,34%; IC 95% 28,06- 40,62%) erano portatori di catetere urinario. In totale sono state analizzate oltre 1200 procedure. La prevalenza di infezioni nosocomiali delle vie urinarie è stata del 12,28% (IC 95% 7,98-16,50%). Tutti i cateterizzati avevano un sistema di drenaggio di tipo chiuso. I modelli di regressione logistica hanno dimostrato un accresciuto rischio di mancato lavaggio delle mani in presenza di un regime di ricovero d’urgenza e in unità operativa chirurgica (p‹0,01), parimenti si è evidenziato un minor livello di controllo del meato urnario in presenza del regime del ricovero d’urgenza in unità operativa chirurgica (p‹0,01).Conclusioni: le raccomandazioni fornite dalla letteratura in relazione all’inserimento e alla gestione del cateterismo vescicale sono solo in parte seguite nella pratica quotidiana. In particolare il lavaggio delle mani, anche se è una procedura semplice e poco costosa risulta comunque poco seguita, soprattutto in regime di urgenze e nelle chirurgie, dove per la tipologia delle prestazioni effettuata, l’aderenza a queste procedure dovrebbe essere massima. Questi comportamenti “scorretti” rendono inefficace l’utilizzo del cateterismo vescicale a ciclo chiuso. Nonostante queste problematicità la frequenza di IVU è nel range di variabilità che analoghi studi nazionali ed internazionali presentano.
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- 2003
49. Analisi dei processi di un ambulatorio per i viaggiatori internazionali
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Demarchi, M.L., Sarasino, D., Luparia, M., Renna, M., Antoniotti, M.C., Moia, E., Minola, M., Panella, M., Dessì, E., Motta, G., and Meloni, A.M.
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lcsh:Public aspects of medicine ,lcsh:R ,DOAJ:Public Health ,lcsh:Medicine ,lcsh:RA1-1270 ,DOAJ:Health Sciences - Abstract
Obiettivi: 1) determinare i costi di gestione dell’ambulatorio del viaggiatore internazionale dell’ASL13 di Novara; 2) predisporre un piano di riorganizzazione dell’ambulatorio. Materiali e metodi: per la determinazione dei costi di gestione dell’ambulatorio è stata applicata la metodologia dell’Activity Based Costing (ABC) che consiste nello scomporre, secondo un criterio gerarchico, le attività che costituiscono un processo, partendo da quelle poste a livello più elevato (macroattività) e giungendo al singolo compito professionale (microattività).In seguito per ogni attività individuata ciascun operatore del servizio indica, in percentuale, il tempo mediamente dedicato a tale attività, al fine di quantificarne il costo. Le attività individuate sono state rappresentate graficamente con la tecnica del Work design secondo cui per ciascun processo sono identificati input, output, risorse utilizzate, nonché eventuali regole e controlli a cui è soggetto.Risultati: lo studio ha coinvolto tutti gli operatori dell’ambulatorio (4 medici, 2 assistenti sanitari e 1 assistente amministrativo).Sono state identificate 180 attività. Il costo annuale complessivo della gestione dell’ambulatorio, attribuibile alle risorse umane, è pari a ¤ 288.934. Complessivamente il costo di alcune attività è risultato particolarmente elevato, in quanto le attività stesse vengono svolte da figure professionali non pertinenti (es. attività amministrative svolte dall’infermiere, attività di pertinenza infermieristica effettuate dal medico).Attraverso la definizione di input, output, controlli e meccanismi, è stato possibile evidenziare sia le macro criticità del processo organizzativo, quali ad esempio la necessità di integrare l’utilizzo di supporti informatizzati per la gestione delle informazioni relative all’utente, sia le micro criticità, come l’esigenza di predisporre materiale informativo anche in lingua straniera. L’analisi ha inoltre rilevato l’assenza di un sistema informativo di feed-back che consentisse il monitoraggio della morbosità delle patologie contratte all’estero, elemento utile in un’ottica di programmazione.Conclusioni: l’ABC, grazie all’individuazione delle criticità, haconsentito di definire un piano per la riorganizzazione dell’ambulatorio, volto all’ottimizzazione delle risorse disponibili garantendo l’erogazione di prestazioni efficaci ed efficienti.
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- 2003
50. Cathodic protection modelling of a cover and uncover steel in seawater environment following by electric signature simulations of a ship
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Minola, M., Roche, V., J-C, Leprêtre, Goeau, C., Chadebec, O., L-L, Rouve, Olivier Pinaud, Nale, M., Electrochimie Interfaciale et Procédés (EIP ), Laboratoire d'Electrochimie et de Physico-chimie des Matériaux et des Interfaces (LEPMI ), Institut polytechnique de Grenoble - Grenoble Institute of Technology (Grenoble INP )-Institut de Chimie du CNRS (INC)-Université Savoie Mont Blanc (USMB [Université de Savoie] [Université de Chambéry])-Centre National de la Recherche Scientifique (CNRS)-Université Grenoble Alpes [2016-2019] (UGA [2016-2019])-Institut polytechnique de Grenoble - Grenoble Institute of Technology (Grenoble INP )-Institut de Chimie du CNRS (INC)-Université Savoie Mont Blanc (USMB [Université de Savoie] [Université de Chambéry])-Centre National de la Recherche Scientifique (CNRS)-Université Grenoble Alpes [2016-2019] (UGA [2016-2019]), Matériaux Interfaces ELectrochimie (MIEL ), DGA TN F, 1) DGA TN F-29200 Brest, Laboratoire de Génie Electrique de Grenoble (G2ELab), Institut polytechnique de Grenoble - Grenoble Institute of Technology (Grenoble INP )-Centre National de la Recherche Scientifique (CNRS)-Université Grenoble Alpes [2016-2019] (UGA [2016-2019]), G2Elab-Modèles, Méthodes et Méthodologies Appliqués au Génie Electrique (G2Elab-MAGE), Laboratoire de Génie Electrique de Grenoble (G2ELab ), Centre National de la Recherche Scientifique (CNRS)-Université Grenoble Alpes (UGA)-Institut polytechnique de Grenoble - Grenoble Institute of Technology (Grenoble INP ), Université Grenoble Alpes (UGA)-Centre National de la Recherche Scientifique (CNRS)-Université Grenoble Alpes (UGA)-Institut polytechnique de Grenoble - Grenoble Institute of Technology (Grenoble INP ), and Université Grenoble Alpes (UGA)
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[SPI.NRJ]Engineering Sciences [physics]/Electric power ,ComputingMilieux_MISCELLANEOUS - Abstract
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