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A random laser carrying the scattering information on a biological host is a promising tool for the characterization of biophysical properties. In this work, random lasing from label-free living cells is proposed to achieve rapid cytometry of apoptosis. Random lasing is achieved by adding biocompatible gain medium to a confocal dish containing cells under optically pumped conditions. The random lasing characteristics are distinct at different stages of cell apoptosis after drug treatment. By analyzing the power Fourier transform results of the random lasing spectra, the percentage of apoptotic cells could be distinguished within two seconds, which is more than an order of magnitude faster than traditional flow cytometry. These results provide a label-free approach for rapid cytometry of apoptosis, which is advantageous for further research of random lasers in the biological field.

An all-optical tunable whispering gallery mode (WGM) laser pumped by a laser diode is proposed. The laser is fabricated by filling a silica capillary with a light-emitting conjugated polymer solution. Based on the thermo-optic effect of the hydroxyl groups in the polymer and capillary, the effective refractive index of the WGM cavity changes by the auxiliary irradiation of the laser, and the wavelength of the WGM mode shifts correspondingly. The emission wavelength was continuously tuned over 13 nm with the irradiation power intensity changing from 0 to 22.41 W cm

Multiferroic materials have great potential in non-volatile devices for low-power and ultra-high density information storage, owing to their unique characteristic of coexisting ferroelectric and ferromagnetic orders. The effective manipulation of their intrinsic anisotropy makes it promising to control multiple degrees of the storage “medium”. Here, we have discovered intriguing in-plane electrical and magnetic anisotropies in van der Waals (vdW) multiferroic CuCrP2S6. The uniaxial anisotropies of current rectifications, magnetic properties and magnon modes are demonstrated and manipulated by electric direction/polarity, temperature variation and magnetic field. More important, we have discovered the spin-flop transition corresponding to specific resonance modes, and determined the anisotropy parameters by consistent model fittings and theoretical calculations. Our work provides in-depth investigation and quantitative analysis of electrical and magnetic anisotropies with the same easy axis in vdW multiferroics, which will stimulate potential device applications of artificial bionic synapses, multi-terminal spintronic chips and magnetoelectric devices.

In situ self-assembly of semiconducting emitters into multilayer cracks is a significant solution-processing method to fabricate organic high- Q lasers. However, it is still difficult to realize from conventional conjugated polymers. Herein, we create the molecular super-hindrance-etching technology, based on the π-functional nanopolymer PG-Cz, to modulate multilayer cracks applied in organic single-component random lasers. Massive interface cracks are formed by promoting interchain disentanglement with the super-steric hindrance effect of π-interrupted main chains, and multilayer morphologies with photonic-crystal-like ordering are also generated simultaneously during the drop-casting method. Meanwhile, the enhancement of quantum yields on micrometer-thick films ( Φ = 40% to 50%) ensures high-efficient and ultrastable deep-blue emission. Furthermore, a deep-blue random lasing is achieved with narrow linewidths ~0.08 nm and high-quality factors Q ≈ 5,500 to 6,200. These findings will offer promising pathways of organic π-nanopolymers for the simplification of solution processes applied in lasing devices and wearable photonics.

Multiferroic materials have great potential in non-volatile devices for low-power and ultra-high density information storage, owing to their unique characteristic of coexisting ferroelectric and ferromagnetic orders. The effective manipulation of their intrinsic anisotropy makes it promising to control the multiple degrees of freedom of the storage "medium". Here, we have discovered intriguing electrical and magnetic anisotropies within the intralayer of CuCrP2S6, a promising van der Waals multiferroic material. The in-plane uniaxial anisotropies of the current rectifications, magnetic properties and magnon modes are demonstrated and manipulated by electric direction/polarity, temperature variation and magnetic field. More important, we have observed spin-flop transition corresponding to specific magnon modes, and it is well supported by theoretical calculations. Our work provides the first observation of electrical and magnetic anisotropies with same easy axis in van der Waals multiferroics, which will stimulate novel device applications of artificial bionic synapses, multi-terminal spintronic chips and magnetoelectric devices.

Single mode lasers, particularly red-green-blue (RGB) colors, have attracted wide attention due to their potential applications in the photonic field. Here, we realize the RGB single mode lasing in a hybrid two-dimension and three-dimension (2D–3D) hybrid microcavity (μ-cavity) with a low threshold. The hybrid 2D–3D μ-cavity consists of a polymer fiber and a microsphere. Typical RGB polymer film consisting gain materials are cladded on a fiber. To achieve single mode lasing, the polymer fiber therein serves as an excellent gain cavity to provide multiple lasing modes while the microsphere acts as a loss channel to suppress most of the lasing modes. Mode switching can be realized by adjusting the pump position. It can be attributed to the change of coupled efficiency between gain μ-cavity and loss μ-cavity. Our work will provide a platform for the rational design of nanophotonic devices and on-chip communication.

Drop-based microcavity lasers emerged as a promising tool in modern physics investigation and chemical detection owing to their cost-effective fabrication, high luminescence, and sensitive molecule sensing. However, it is of great challenge to achieve highly directional emission along with high quality (Q) factors via traditional droplet self-assembly behavior of the gain medium on a planar substrate. In this work, a single-mode microcavity laser with directional far-field emission is first proposed via droplet self-assembly 3D-curved microcavities, and simultaneously, acetic acid (AcOH) gas sensing is realized. Trichromatic single-mode lasing in 3D-curved microcavities with distinct organic polymer droplets is constructed on silica fibers via a self-assembly procedure. By regulating the curvature of the substrate, mode selection and directional emission of the lasing action are realized. The measured Q-factor of the proposed anisotropic 3D-curved active microcavity is ∼20k. Furthermore, on account of the sensitive responsiveness of liquid organic polymers, single-mode laser sensors can be realized by measuring the shift of their lasing modes on exposure to organic vapor. Benefiting from chemical reaction with rhodamine 6G, the AcOH gas sensor displays a short response time. These results may open new insights into drop-based quasi-3D-anisotropic whispering-gallery-mode microcavities to improve the development of lab-in-a-droplet, ranging from a tuneable microcavity laser to a chemical gas sensor.

Single-mode plasmonic lasing has great potential for use in photonic and sensing applications. In this work, single-mode lasing is realized using a plasmonic-enhanced woven microfiber that shows ultrahigh sensitivity to the ambient environment. This plasmonic-enhanced microfiber is fabricated by spraying Ag nanospheres onto rhodamine 6G-doped polymer microfibers. Single-mode laser emission with an ultranarrow linewidth (0.1 nm) and a low threshold (18.8 kW/mm2) is achieved in the microfiber using the effects of mode selection and plasmonic enhancement provided by the Ag nanospheres. A large wavelength shift in the single-mode lasing is observed when the proposed laser is used as a sensor and exposed to a humid or acidic environment. The wavelength shift is attributed to refractive index variations in the microfiber caused by either moisture absorption or chemical reactions. In humidity sensing, the laser's sensitivity is as high as 826.6 pm/% relative humidity (RH) and the detection limit is 0.051% RH. An innovative strategy for acetic acid gas sensing is proposed that uses the chemical reaction with rhodamine 6G, and its minimum response time is 5 min. Because of the microfiber's excellent fabric compatibility, a wearable sensor is fabricated by weaving the plasmonic-enhanced microfiber into clothes, and this sensor demonstrates extreme bending stability. The results reported here provide a novel approach to the design and fabrication of ultrasensitive wearable sensors for multifunctional sensing applications.

Light-emitting fabric can facilitate the innovation of wearable display applications. Electronic and luminescent textiles capable of communicating, sensing, and supplying energy have been achieved. However, a facile strategy for fabricating large-area flexible lasing textiles has not yet been reported. In this work, we propose a gravity-assisted rotatory drawing method for fabricating flexible lasing microfibers, which can be woven into multicolor lasing textiles. By regulating the doped dyes and solution viscosity, we achieve the mass manufacturing of lasing microfibers with different emission colors and modes and further weave them into full-color textiles with a wide color gamut, approximately 79.1% larger than that of standard RGB space. For application, we print nanoparticle patterns on the lasing textile and encode it with programmable lasing signal distribution, which can supply an anticounterfeiting label for efficient authentication. This work unifies the fabrication and application of lasing textiles, and we expect that this will provide a new platform for flexible lasing devices.

Chaotic cryptography as an important means for digital image encryption has become a great cryptographic project in the current information age. As a novel microcavity laser, a random laser (RL) has a natural advantage for a chaotic system, relying on its spectral randomness. Nevertheless, this encrypted image generally suffers from outline exposition when an unsuitable key from a single RL spectrum is employed. Herein, to realize reliable dual chaotic encryption, an internally integrated hybrid microcavity in random and whispering-gallery-mode (WGM) is reported. Within this coupled microcavity, the rhodamine-6G-doped inner-wall of the fiber serves as the gain medium and the optical cavities for WGM lasing; an RL mode is enabled by scattered particles and the gain medium (Rh6G). Interestingly, the smooth inner wall of the fiber with a high-quality (

Microlasers hold great promise for the development of photonics and optoelectronics. At present, tunable microcavity lasers, especially regarding in situ dynamic tuning, are still the focus of research. In this study, we combined a 0.7Pb(Mg1/3Nb2/3)O3-0.3PbTiO3 (PMN-PT) piezoelectric crystal with a Poly [9,9-dioctylfluorenyl-2,7-diyl] (PFO) microring cavity to realize a high-quality, electrically tunable, whispering-gallery-mode (WGM) laser. The dependence of the laser properties on the diameter of the microrings, including the laser spectrum and quality (Q) value, was investigated. It was found that with an increase in microring diameter, the laser emission redshifted, and the Q value increased. In addition, the device effectively achieved a blueshift under an applied electric field, and the wavelength tuning range was 0.71 nm. This work provides a method for in situ dynamic spectral modulation of microcavity lasers, and is expected to provide inspiration for the application of integrated photonics technology.

An ultrathin-film microring laser was fabricated using inkjet printing and a simple lift-off technique. Whispering-gallery-mode lasing was observed under optically pumped conditions in the film. The freestanding laser can be transferred to arbitrary surfaces for multifunctional applications, such as acoustic and relative humidity sensing. Using the first eigenmode of a membrane vibration, an acoustic sensor with a 0.15 Pa limit of detection was demonstrated via laser bandwidth broadening. A relative humidity sensor with a 1.1% limit of detection via wavelength shifts was demonstrated by placing the device on an optical fiber facet. These cost-effective, transferrable, multifunctional laser sensors will have many additional applications.

Because of its limited light field mode and high Q value, the whispering-gallery-mode (WGM) cavity has been widely studied. In this study, we propose a simple, rapid, low-cost and no-manufacturing technology method that we call the drip-coating method to obtain an irregular cavity with arbitrary boundaries. By using polyvinyl alcohol (PVA) solution doped with rhodamine 6G, the irregular cavity with arbitrary boundaries was drip-coated on a high-reflection mirror, forming a WGM laser. The sample was pumped with a 532 nm pulsed laser, and the single-mode WGM and multi-WGM lasing were obtained. All WGMs are the vertical oscillation modes, which originate from both the total internal reflection of the PVA/air interface and vertical reflection of the PVA/mirror interface. The other boundaries of the cavity were not involved in the reflection and could have any shape. The mechanism of producing single-mode lasing is due to the action of the loss-gain cavity. Multi-WGM lasing is attributed to at least two groups of different WGMs existing in an irregular cavity. This can be confirmed by using a microsphere model and intensity correlation method. These results may provide an alternative for the design of WGM lasers.

Topological Weyl semimetals have attracted considerable interest because they manifest underlying physics and device potential in spintronics. Large anomalous Hall effect (AHE) in non-collinear antiferromagnets (AFMs) represents a striking Weyl phase, which is associated with Bloch-band topological features. In this work, we report robust AHE and Lifshitz transition in high-quality Weyl semimetal Mn3Ge thin film, comprising stacked Kagome lattice and chiral antiferromagnetism. We successfully achieved giant AHE in our Mn3Ge film, with a strong Berry curvature enhanced by the Weyl phase. The enormous coercive field HC in our AHE curve at 5 K reached an unprecedented 5.3 T among hexagonal Mn3X systems. Our results provide direct experimental evidence of an electronic topological transition in the chiral AFMs. The temperature was demonstrated to play an efficient role in tuning the carrier concentration, which could be quantitatively determined by the two-band model. The electronic band structure crosses the Fermi energy level and leads to the reversal of carrier type around 50 K. The results not only offer new functionality for effectively modulating the Fermi level location in topological Weyl semimetals but also present a promising route of manipulating the carrier concentration in antiferromagnetic spintronic devices.

Surface-enhanced Raman scattering (SERS) is a molecule-specific ultra-sensitive spectroscopic technique. With the development of portable Raman equipment, it has become possible to apply the SERS technique for rapid on-site detection. Therefore, the search for materials with excellent surface plasmon resonance (SPR) activity and high stability has become an important research focus in recent years. In this study, we successfully prepared plasmonic nanostructures with a large number of SERS “hotspots” using alloy nanoparticles (NPs) with tunable gold–silver mole ratios. These structures were composed of numerous narrow gapped gold–silver alloy NPs with diameters ranging from 10 to 100 nm. SERS property evaluation showed that the prepared alloy SERS substrates had good uniformity, and the performance of the substrates rapidly improved as the Ag content increased. Gold-stabilized Au–Ag alloy SERS substrates combine the high performance of the Ag SERS substrate and the excellent stability of Au. In addition, the wavelength of the SPR can be tuned by adjusting the mole ratio of Au and Ag to satisfy different excitation wavelengths. Thus, the Au–Ag alloy SERS substrates we prepared show good comprehensive performance. The lowest concentration of rhodamine 6G that can be homogeneously detected by the prepared Au1Ag8 alloy substrate is 5 × 10−12 M, and the enhancement factor is 5.1 × 108. Finite-difference time-domain (FDTD) theoretical calculations further confirmed our experimental results and theoretically demonstrated the unique properties of the Au–Ag alloy SERS substrates.

Hybrid lead halide perovskites have made great strides in next-generation photovoltaic and optoelectronic devices. Random lasers based on perovskite materials have been intensively investigated, but the miniaturization of perovskite random lasers has not been achieved up to now. Here, we report the fabrication of perovskite random lasers based on perovskite films deposited on the optical fiber facets using a dip-coating method. Under optical pumping conditions, random lasing was observed with minimum threshold energy of 32.3 μJ/cm2 at ~550 nm; also, the lasing threshold decreased with increasing diameter of the optical fiber. The results show that the random lasing emission originates from the scattering between the perovskite crystal grains, and the decreased threshold is attributed to the increased active area of the perovskite film. The directionality of perovskite random lasers indicates that the divergence angle of the laser beam is less than 60°. We also demonstrate that the perovskite random laser on the fiber facet can prevent speckle formation and improve image quality. These results may promote the applications of random lasers in compact sources and integrated optoelectronic devices.

Molecular carbon imides, especially extended perylene diimides (PDIs) have been the best wide-band-gap nonfullerene acceptors. Despite their excellent photothermal/chemical stability, flexible reaction sites, and unique photoelectronic properties, there is still a lack of fundamental understanding of their molecular characteristics as a third component. Here, generations of PDIs with distinctive molecular architecture, are deliberately screened out as the third component to PM6:Y6. Only a rylene-fullerene hybrid, S-Fuller-PMI, surprisingly boosts the fill factor (FF) of ternary organic solar cells (OSCs) to 0.77 from 0.72 for PM6:Y6 binary ones, and therefore the power conversion efficiency (PCE) of ternary cells is enhanced from 15.3% to 16.2%. Compared with highly-flexible rylene dimer and rigid multimer, S-Fuller-PMI exhibits higher electron mobility, favorable surface tension, and, therefore tailored compatibility with Y6. These formed Y6:S-Fuller-PMI alloys play as a morphological controller to improve charge separation and transport process. Simultaneously, the suppressed photothermal-induced traps, along with inherent enlarged entropy effect, endow the ternary OSCs still with ≈70% of initial PCE even after 500 h continuous illumination, whereas only 53% is left in their binary counterparts. These results provide new insight into the molecular design principle for distinctive molecular carbon imides as the third component for efficient and durable PM6:Y6-based OSCs.

Humidity sensing plays an important role in the professional field and our daily life, such as chemical preparation process, environmental monitoring, and food storage. Herein, a wearable humidity sensor is designed based on a flexible plasmonic random laser. The random laser-based humidity sensor is fabricated by transferring an ultrathin light-emitting polymer membrane doped with silver nanoparticles onto the humidity-sensitive PEDOT:PSS film. Under optical pumping, random lasing with low-threshold is achieved, assisted by the strong plasmonic feedback of the silver nanoparticles. The random laser-based humidity sensor exhibits a good linear response with a coefficient of 0.997. Comparing with the emission intensity at initial relative humidity (RH) (34.8%), the peak intensity increases 5.5 times at an RH value of 93.5%. This phenomenon mainly results from the ambient humidity-sensitive relative refractive index difference between polymer membrane and PEDOT:PSS film. The random laser-based humidity sensor is flexible and nontoxic, which can be transplanted easily to achieve wearable laser devices.

This article assembles a distributed feedback (DFB) cavity on the sidewalls of the optical fiber by using very simple fabrication techniques including two-beam interference lithography and dip-coating. The DFB laser structure comprises graduated gratings on the optical fiber sidewalls which are covered with a layer of colloidal quantum dots. Directional DFB lasing is observed from the fiber facet due to the coupling effect between the grating and the optical fiber. The directional lasing from the optical fiber facet exhibits a small solid divergence angle as compared to the conventional laser. It can be attributed to the two-dimensional light confinement in the fiber waveguide. An analytical approach based on the Bragg condition and the coupled-wave theory was developed to explain the characteristics of the laser device. The intensity of the output coupled laser is tuned by the coupling coefficient, which is determined by the angle between the grating vector and the fiber axis. These results afford opportunities to integrate different DFB lasers on the same optical fiber sidewall, achieving multi-wavelength self-aligned DFB lasers for a directional emission. The proposed technique may provide an alternative to integrating DFB lasers for applications in networking, optical sensing, and power delivery.

The orbital angular momentum (OAM) of the structure light is viewed as a candidate for enhancing the capacity of information processing. Microring has advantages in realizing the compact lasers required for on-chip applications. However, as the clockwise and counterclockwise whispering gallery modes (WGM) appear simultaneously, the emitted light from the normal microring does not possess net OAM. Here, we propose an OAM laser based on the standing-wave WGMs containing clockwise and counterclockwise WGM components. Due to the inhomogeneous intensity distribution of the standing-wave WGM, the single-mode lasing for the OAM light can be realized. Besides, the OAM of the emitted light can be designed on demand. The principle and properties of the proposed laser are demonstrated by numerical simulations. This work paves the way for exploring a single-mode OAM laser based on the plasmonic standing-wave WGMs at the microscale, which can be served as a basic building block for on-chip optical devices.

Recently, wearable sensor technology has drawn attention to many health-related appliances due to its varied existing optical, electrical, and mechanical applications. Similarly, we have designed a simple and cheap lift-off fabrication technique for the realization of large-area biocompatible random lasers to customize wearable sensors. A large-area random microcavity comprises a matrix element polymethyl methacrylate (PMMA) in which rhodamine B (RhB, which acts as a gain medium) and gold nanorods (Au NRs, which offer plasmonic feedback) are incorporated via a spin-coating technique. In regards to the respective random lasing device residing on a heterogenous film (area &gt, 100 cm2), upon optical excitation, coherent random lasing with a narrow linewidth (~0.4 nm) at a low threshold (~23 μJ/cm2 per pulse) was successfully attained. Here, we maneuvered the mechanical flexibility of the device to modify the spacing between the feedback agents (Au NRs), which tuned the average wavelength from 612.6 to 624 nm under bending while being a recoverable process. Moreover, the flexible film can potentially be used on human skin such as the finger to serve as a motion and relative-humidity sensor. This work demonstrates a designable and simple method to fabricate a large-area biocompatible random laser for wearable sensing.

One of the most attractive characteristics of diluted ferromagnetic semiconductors is the possibility to modulate their electronic and ferromagnetic properties, coupled by itinerant holes through various means. A prominent example is the modification of Curie temperature and magnetic anisotropy by ion implantation and pulsed laser melting in III–V diluted magnetic semiconductors. In this study, to the best of our knowledge, we performed, for the first time, the co-doping of (In,Mn)As diluted magnetic semiconductors by Al by co-implantation subsequently combined with a pulsed laser annealing technique. Additionally, the structural and magnetic properties were systematically investigated by gradually raising the Al implantation fluence. Unexpectedly, under a well-preserved epitaxial structure, all samples presented weaken Curie temperature, magnetization, as well as uniaxial magnetic anisotropies when more aluminum was involved. Such a phenomenon is probably due to enhanced carrier localization introduced by Al or the suppression of substitutional Mn atoms.

A full-color whispering-gallery mode (WGM) laser has been fabricated by partitioning different light-emitting polymers in a nested microcavity. Red-green-blue WGM lasing with a high quality factor above 104 and a narrow linewidth of 0.025 nm emits from nested capillaries when excited with a nanosecond laser. The full-color WGM lasing shows a low excitation threshold for the nested microcavities, which can avoid fluorescence resonant energy transfer. We also achieve wavelength tunable lasing upon altering the different polymers in the nested microcavities. The work demonstrates a simple method to fabricate a full-color WGM laser and its potential applications in compact lighting devices and white laser sources.

Among the efforts to improve the performances of microlasers, optimization of the gain properties and cavity parameters of these lasers has attracted significant attention recently. Distributed feedback lasers, as one of the most promising candidate technologies for electrically pumped microlasers, can be combined with dual-gratings. This combination provides additional freedom for the design of the laser cavity. Here, a holographic dual-grating is designed to improve the distributed feedback laser performance. The holographic dual-grating laser consists of a colloidal quantum dot film with two parallel gratings, comprising first-order (210 nm) and second-order (420 nm) gratings that can be fabricated easily using a combination of spin coating and interference lithography. The feedback and the output from the cavity are controlled using the first-order grating and the second-order grating, respectively. Through careful design and analysis of the dual-grating, a balance is achieved between the feedback and the cavity output such that the lasing threshold based on the dual-grating is nearly half the threshold of conventional distributed feedback lasers. Additionally, the holographic dual-grating laser shows a high level of stability because of the high stability of the colloidal quantum dots against photobleaching.

Fibonacci-spaced defect resonators were analytically investigated by cavity coupling, which exhibited a series of well-defined optical modes in fractals. The analytic model can be used to predict the output performance of microcavity lasers based on Fibonacci-spaced defect resonators, such as the mode number, resonant frequency, and Q factor. All results obtained by the analytical solution are in good consistency with that obtained by the finite-difference time-domain method. The simulation result shows that the Q factor of the resonant modes would increase dramatically with the appearance of narrower optical modes. The proposed theoretical model can be used to inversely design high performance polymer lasers based on the Fibonacci-spaced defect resonators.

Considerable research efforts have been devoted to the investigation of distributed feedback (DFB) organic lasing in photonic crystals in recent decades. It is still a big challenge to realize DFB lasing in complex photonic crystals. This review discusses the recent progress on the DFB organic laser based on one-, two-, and three-dimensional photonic crystals. The photophysics of gain materials and the fabrication of laser cavities are also introduced. At last, future development trends of the lasers are prospected.

Here we report the contribution of self-absorption to excitonic luminescence in an ultrathin-walled ZnO semiconductor microtube cavity. The trapping structure regulates the X-band and near-band edge emission via various excitation-detection geometries. The self-absorption in the microcavity results in a high concentration of exciton ~3.65 × 1016 cm−3 and boosts the amplified spontaneous emission. The enhancement ratio for the UV band emissions can be up to 40 folds, higher than using localized surface plasmon resonance via Ag nanoparticles. The coefficient of self-absorption by the light-trapping microtube structure is therefore determined to be 6.1. The present work opens up new opportunities to enhance the photons collection and interaction with excitons in wide-band-gap semiconductor for on-chip wavelength-tunable UV-luminescence devices in optoelectronic applications.

Herein, a quantum dot random laser was achieved using a silicon nanowire array. The silicon nanowire array was grown by a metal-assisted chemical etching method. A colloidal quantum dot solution was spin-coated on silicon nanowires to form the random laser. The performance of the random laser was controlled by the resistivity of silicon wafers and the length of silicon nanowires. A transition from incoherent random lasing to coherent random lasing was obtained by increasing the resistivity of the silicon wafers. The random lasing threshold increased with an increase in the length of the silicon nanowires. These results may be useful to explore high-performance silicon-based random lasers.

A hybrid membrane is employed as a high-order plasmonic distributed feedback (DFB) cavity to reduce the lasing threshold of polymer lasers. The hybrid membrane consists of an anodic aluminum oxide (AAO) membrane, a 25 nm thick silver layer and a free-standing polymer membrane. The AAO membrane is fabricated by a low-cost, single chemical etching method. Then, a layer of silver with a thickness of 25 nm is sputtered on the surface of the AAO. Subsequently, a polymer membrane is directly attached to the silver-plated AAO membrane, forming an AAO/silver/polymer hybrid membrane. Under optical pumping conditions, low-threshold, three-order DFB lasing is observed. The proposed laser device exhibited a dual-threshold characteristic because of the evolution from amplified spontaneous emission to DFB lasing. And a significant shift from omnidirectional emission to directional emission lasing can be observed while the pump energy density is beyond the second threshold. Furthermore, the plasmonic enhancement sourced from silver corrugation reveals important improvement effects to the DFB lasing of AAO/silver/polymer hybrid membrane for decreasing threshold, narrowing full width at half maximum (FWHM), and an increasing Q factor. This work may promote the design and production of low-cost and large-area high-order plasmonic DFB polymer lasers.

Miniaturized lasing with dynamic manipulation is critical to the performance of compact and versatile photonic devices. However, it is still a challenge to manipulate the whispering gallery mode lasing modes dynamically. Here, we design the quasi-three-dimensional coupled cavity by a micromanipulation technique. The coupled cavity consists of two intersection polymer microfibers. The mode selection mechanism is demonstrated experimentally and theoretically in the coupled microfiber cavity. Dynamic manipulation from multiple modes to single-mode lasing is achieved by controlling the coupling strength, which can be quantitatively controlled by changing the coupling angle or the coupling distance. Our work provides a flexible alternative for the lasing mode modulation in the on-chip photonic integration.

Spintronics and molecular chemistry have achieved remarkable achievements separately. Their combination can apply the superiority of molecular diversity to intervene or manipulate the spin-related properties. It inevitably brings in a new type of functional devices with a molecular interface, which has become an emerging field in information storage and processing. Normally, spin polarization has to be realized by magnetic materials as manipulated by magnetic fields. Recently, chiral-induced spin selectivity (CISS) was discovered surprisingly that non-magnetic chiral molecules can generate spin polarization through their structural chirality. Here, the recent progress of integrating the strengths of molecular chemistry and spintronics is reviewed by introducing the experimental results, theoretical models, and device performances of the CISS effect. Compared to normal ferromagnetic metals, CISS originating from a chiral structure has great advantages of high spin polarization, excellent interface, simple preparation process, and low cost. It has the potential to obtain high efficiency of spin injection into metals and semiconductors, getting rid of magnetic fields and ferromagnetic electrodes. The physical mechanisms, unique advantages, and device performances of CISS are sequentially clarified, revealing important issues to current scientific research and industrial applications. This mini-review points out a key technology of information storage for future spintronic devices without magnetic components.

We present a hybrid cavity designed to manipulate lasing modes, consisting of a metal-dielectric core–shell hybrid microcavity fabricated using a simple brush-coating method. Single and multiple modes can be obtained in the proposed laser device by the trade-off between loss and gain. Moreover, we achieve electrically tunable whispering-gallery-mode lasing by employing the thermo-optic effect in the hybrid microcavity. The lasing peak of the modes can be electrically tuned by quantitative control of Joule heating. We measure a tuning rate of 15.3 pm/J for all the lasing peaks.

Lasing properties of the two-dimensional (2D) distributed feedback (DFB) lasers can be engineered by replacing either the gain medium or periodic structures necessary for the feedback mechanism. Quasicrystals are the intermediate class between the periodic and random structures. They have high rotational symmetry and more favorable for the generation of photonic bandgap as compared to periodic structures. In our experiment, we designed a pentagonal prism for the holographic lithography to construct a long-range 10-fold rotational symmetry, which exhibits 2D quasiperiodic structures. A solution-processable colloidal quantum dots (CQDs) was spin-coated on the resultant 2D quasicrystals. An analytical model based on the cavity mode coupling effect was developed to predict the output performance of the 2D DFB CQDs photonic quasicrystals laser. The respective optically pumped 2D photonic quasicrystal samples exhibit multi-wavelength lasing emission in different directions due to long-range rotational symmetry. The five DFB lasing spots are symmetrically distributed in the 2D space, the center of the lasing spots is similar to a star shape. The derived analytical model predictions are in line with the experimental results.

Hall-effect in semiconductors has wide applications for magnetic field sensing. Yet, a standard Hall sensor retains two problems: its linearity is affected by the non-uniformity of the current distribution; the sensitivity is bias-dependent, with linearity decreasing with increasing bias current. In order to improve the performance, we here propose a novel structure which realizes bias-free, photo-induced Hall sensors. The system consists of a semi-transparent metal Pt and a semiconductor Si or GaAs to form a Schottky contact. We systematically compared the photo-induced Schottky behaviors and Hall effects without net current flowing, depending on various magnetic fields, light intensities and wavelengths of Pt/GaAs and Pt/Si junctions. The electrical characteristics of the Schottky photo-diodes were fitted to obtain the barrier height as a function of light intensity. We show that the open-circuit Hall voltage of Pt/GaAs junction is orders of magnitude lower than that of Pt/Si, and the barrier height of GaAs is smaller. It should be attributed to the surface states in GaAs which block the carrier drifting. This work not only realizes the physical investigations of photo-induced Hall effects in Pt/GaAs and Pt/Si Schottky junctions, but also opens a new pathway for bias-free magnetic sensing with high linearity and sensitivity comparing to commercial Hall-sensors.

Topological Weyl semimetals have attracted considerable interest because they manifest underlying physics and device potential in spintronics. Large anomalous Hall effect (AHE) in non-collinear antiferromagnets (AFMs) represents a striking Weyl phase, which is associated with Bloch-band topological features. In this work, we report robust AHE and Lifshitz transition in high-quality Weyl semimetal Mn3Ge thin film, comprising stacked Kagome lattice and chiral antiferromagnetism. We successfully achieved giant AHE in our Mn3Ge film, with a strong Berry curvature enhanced by the Weyl phase. The enormous coercive field HC in our AHE curve at 5 K reached an unprecedented 5.3 T among hexagonal Mn3X systems. Our results provide direct experimental evidence of an electronic topological transition in the chiral AFMs. The temperature was demonstrated to play an efficient role in tuning the carrier concentration, which could be quantitatively determined by the two-band model. The electronic band structure crosses the Fermi energy level and leads to the reversal of carrier type around 50 K. The results not only offer new functionality for effectively modulating the Fermi level location in topological Weyl semimetals but also present a promising route of manipulating the carrier concentration in antiferromagnetic spintronic devices.