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Despite offsetting global mean surface temperature, various studies demonstrated that Stratospheric Aerosol Injection (SAI) could influence the recovery of stratospheric ozone and have important impacts on stratospheric and tropospheric circulation, thereby potentially playing an important role in modulating regional and seasonal climate variability. However, so far most of the assessments of such an approach have come from climate model simulations in which SO2 is injected only in a single location or a set of locations. Here we use CESM2-WACCM6 SAI simulations under a comprehensive set of SAI strategies achieving the same global mean surface temperature with different locations and/or timing of injections: an equatorial injection, an annual injection of equal amounts of SO2 at 15N and 15S, an annual injection of equal amounts of SO2 at 30N and 30S, and a polar strategy injecting SO2 at 60N and 60S only in spring in each hemisphere. We demonstrate that despite achieving the same global mean surface temperature, the different strategies result in contrastingly different impacts on stratospheric temperatures and circulation, thereby leading to different impacts on Northern Hemispheric polar vortex and, thus, winter mid- and high latitude surface climate, as well as leading to important differences in the future evolution of stratospheric ozone throughout the globe. Overall, the results contribute to an increased understanding of the underlying physical processes as well as lay ground for identifying an optimal SAI strategy that could form a basis of a future multi-model assessment., The 28th IUGG General Assembly (IUGG2023) (Berlin 2023)

The Geoengineering Model Intercomparison Project (GeoMIP) is a coordinating framework, started in 2010, that includes a series of standardized climate model experiments aimed at understanding the physical processes and projected impacts of solar geoengineering (also known as “climate intervention”). Numerous experiments have been conducted, and several more have been proposed as “testbed” experiments, spanning a variety of geoengineering techniques aimed at modifying the planetary radiation budget: stratospheric aerosol injection, marine cloud brightening, surface albedo modification, cirrus cloud thinning and sunshade mirrors. To date, over 125 studies have been published that used results from GeoMIP simulations.Here we provide an introduction to GeoMIP and its experiments. We discuss the knowledge that GeoMIP has contributed to the field of geoengineering research and climate scienc: what have we learned in terms of inter-model differences, robustness of the projected outcomes for specific methods and future areas of model development that would for the future. We also offer multiple examples of cases where GeoMIP experiments were fundamental for international assessments.We provide a critical assessment of GeoMIP with an eye toward future priorities in simulation design and analysis. We discuss the next set of experiments we are working on, in light of future Climate Model Intercomparison Project scenarios and activities, highlighting areas of collaborations with other international projects and intercomparisons. We outline a series of criteria that should guide the development of future GeoMIP experiments and make them relevant to its participants and the broader community, centered around plausibility, policy relevance, scientific relevance and reproducibility., The 28th IUGG General Assembly (IUGG2023) (Berlin 2023)

We have derived values of the ultraviolet index (UVI) at solar noon using the Tropospheric Ultraviolet Model (TUV) driven by ozone, temperature and aerosol fields from climate simulations of the first phase of the Chemistry-Climate Model Initiative (CCMI-1). Since clouds remain one of the largest uncertainties in climate projections, we simulated only the clear-sky UVI. We compared the modelled UVI climatologies against present-day climatological values of UVI derived from both satellite data (the OMI-Aura OMUVBd product) and ground-based measurements (from the NDACC network). Depending on the region, relative differences between the UVI obtained from CCMI/TUV calculations and the ground-based measurements ranged between −5.9 % and 10.6 %. We then calculated the UVI evolution throughout the 21st century for the four Representative Concentration Pathways (RCPs 2.6, 4.5, 6.0 and 8.5). Compared to 1960s values, we found an average increase in the UVI in 2100 (of 2 %–4 %) in the tropical belt (30∘ N–30∘ S). For the mid-latitudes, we observed a 1.8 % to 3.4 % increase in the Southern Hemisphere for RCPs 2.6, 4.5 and 6.0 and found a 2.3 % decrease in RCP 8.5. Higher increases in UVI are projected in the Northern Hemisphere except for RCP 8.5. At high latitudes, ozone recovery is well identified and induces a complete return of mean UVI levels to 1960 values for RCP 8.5 in the Southern Hemisphere. In the Northern Hemisphere, UVI levels in 2100 are higher by 0.5 % to 5.5 % for RCPs 2.6, 4.5 and 6.0 and they are lower by 7.9 % for RCP 8.5. We analysed the impacts of greenhouse gases (GHGs) and ozone-depleting substances (ODSs) on UVI from 1960 by comparing CCMI sensitivity simulations (1960–2100) with fixed GHGs or ODSs at their respective 1960 levels. As expected with ODS fixed at their 1960 levels, there is no large decrease in ozone levels and consequently no sudden increase in UVI levels. With fixed GHG, we observed a delayed return of ozone to 1960 values, with a corresponding pattern of change observed on UVI, and looking at the UVI difference between 2090s values and 1960s values, we found an 8 % increase in the tropical belt during the summer of each hemisphere. Finally we show that, while in the Southern Hemisphere the UVI is mainly driven by total ozone column, in the Northern Hemisphere both total ozone column and aerosol optical depth drive UVI levels, with aerosol optical depth having twice as much influence on the UVI as total ozone column does. ISSN:1680-7375 ISSN:1680-7367

An accurate estimate of global hydroxyl radical (OH) abundance is important for projections of air quality, climate, and stratospheric ozone recovery. As the atmospheric mixing ratios of methyl chloroform (CH₃CCl₃) (MCF), the commonly used OH reference gas, approaches zero, it is important to find alternative approaches to infer atmospheric OH abundance and variability. The lack of global bottom‐up emission inventories is the primary obstacle in choosing a MCF alternative. We illustrate that global emissions of long‐lived trace gases can be inferred from their observed mixing ratio differences between the Northern Hemisphere (NH) and Southern Hemisphere (SH), given realistic estimates of their NH‐SH exchange time, the emission partitioning between the two hemispheres, and the NH versus SH OH abundance ratio. Using the observed long‐term trend and emissions derived from the measured hemispheric gradient, the combination of HFC‐32 (CH₂F₂), HFC‐134a (CH₂FCF₃, HFC‐152a (CH₃CHF₂), and HCFC‐22 (CHClF₂), instead of a single gas, will be useful as a MCF alternative to infer global and hemispheric OH abundance and trace gas lifetimes. The primary assumption on which this multispecies approach relies is that the OH lifetimes can be estimated by scaling the thermal reaction rates of a reference gas at 272 K on global and hemispheric scales. Thus, the derived hemispheric and global OH estimates are forced to reconcile the observed trends and gradient for all four compounds simultaneously. However, currently, observations of these gases from the surface networks do not provide more accurate OH abundance estimate than that from MCF.