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6. 2021: A Year Starting Full of Hope

Author

Gooding, J. Justin, primary, Camasso, Nicole, additional, Bakker, Eric, additional, Kelley, Shana, additional, Sailor, Michael, additional, Merkx, Maarten, additional, Mao, Lanqun, additional, Clark, Heather, additional, Maboudian, Roya, additional, Masson, Jean-François, additional, deMello, Andrew, additional, Li, Meng, additional, and Liu, Sue Min, additional

Published
2021
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9. Confronting Racism in Chemistry Journals

Author

Burrows, Cynthia J., primary, Huang, Jiaxing, additional, Wang, Shu, additional, Kim, Hyun Jae, additional, Meyer, Gerald J., additional, Schanze, Kirk, additional, Lee, T. Randall, additional, Lutkenhaus, Jodie L., additional, Kaplan, David, additional, Jones, Christopher, additional, Bertozzi, Carolyn, additional, Kiessling, Laura, additional, Mulcahy, Mary Beth, additional, Lindsley, Craig W., additional, Finn, M. G., additional, Blum, Joel D., additional, Kamat, Prashant, additional, Choi, Wonyong, additional, Snyder, Shane, additional, Aldrich, Courtney C., additional, Rowan, Stuart, additional, Liu, Bin, additional, Liotta, Dennis, additional, Weiss, Paul S., additional, Zhang, Deqing, additional, Ganesh, Krishna N., additional, Atwater, Harry A., additional, Gooding, J. Justin, additional, Allen, David T., additional, Voigt, Christopher A., additional, Sweedler, Jonathan, additional, Schepartz, Alanna, additional, Rotello, Vincent, additional, Lecommandoux, Sébastien, additional, Sturla, Shana J., additional, Hammes-Schiffer, Sharon, additional, Buriak, Jillian, additional, Steed, Jonathan W., additional, Wu, Hongwei, additional, Zimmerman, Julie, additional, Brooks, Bryan, additional, Savage, Phillip, additional, Tolman, William, additional, Hofmann, Thomas F., additional, Brennecke, Joan F., additional, Holme, Thomas A., additional, Merz, Kenneth M., additional, Scuseria, Gustavo, additional, Jorgensen, William, additional, Georg, Gunda I., additional, Wang, Shaomeng, additional, Proteau, Philip, additional, Yates, John R., additional, Stang, Peter, additional, Walker, Gilbert C., additional, Hillmyer, Marc, additional, Taylor, Lynne S., additional, Odom, Teri W., additional, Carreira, Erick, additional, Rossen, Kai, additional, Chirik, Paul, additional, Miller, Scott J., additional, Shea, Joan-Emma, additional, McCoy, Anne, additional, Zanni, Martin, additional, Hartland, Gregory, additional, Scholes, Gregory, additional, Loo, Joseph A., additional, Milne, James, additional, Tegen, Sarah B., additional, Kulp, Daniel T., additional, and Laskin, Julia, additional

Published
2020
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11. Remembering NJ

Author

Gooding, J. Justin, primary, Mazur, Antonella, additional, Bakker, Eric, additional, Kelley, Shana, additional, Sailor, Michael, additional, Merkx, Maarten, additional, Mao, Lanqun, additional, Clark, Heather, additional, Maboudian, Roya, additional, and Long, Yitao, additional

Published
2020
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13. Happy 5th Anniversary for ACS Sensors

Author

Gooding, J. Justin, primary, Mazur, Antonella, additional, Bakker, Eric, additional, Kelley, Shana, additional, Tao, Nongjian, additional, Sailor, Michael, additional, Merkx, Maarten, additional, Mao, Lanqun, additional, and Clark, Heather, additional

Published
2020
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23. First Impact Factor for ACS Sensors – 5.711

Author

Gooding, J. Justin, primary, Mazur, Antonella, additional, Merkx, Maarten, additional, Kelley, Shana, additional, Tao, Nongjian, additional, Long, Yi-Tao, additional, Bakker, Eric, additional, and Sailor, Michael, additional

Published
2018
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26. An Exciting Year Ahead for ACS Sensors

Author

Gooding, J. Justin, primary, Mazur, Antonella, additional, Sailor, Michael, additional, Merkx, Maarten, additional, Kelley, Shana, additional, Tao, Nongjian, additional, Long, Yitao, additional, and Bakker, Eric, additional

Published
2018
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31. August 2017: Two Years of Submissions

Author

Gooding, J. Justin, primary, Bakker, Eric, additional, Kelley, Shana, additional, Long, Yitao, additional, Merkx, Maarten, additional, Sailor, Michael, additional, Tao, Nongjian, additional, and Mazur, Antonella, additional

Published
2017
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46. Welcome to ACS Sensors

Author

Gooding, J. Justin, primary, Kelley, Shana O., additional, Bakker, Eric, additional, Long, Yitao, additional, Tao, Nongjian (NJ), additional, and Mazur, Antonella I., additional

Published
2016
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48. Impact of the Coverage of Aptamers on a Nanoparticle on the Binding Equilibrium and Kinetics between Aptamer and Protein.

Author

Chen X, Lisi F, Bakthavathsalam P, Longatte G, Hoque S, Tilley RD, and Gooding JJ

Subjects
Gold, Kinetics, Aptamers, Nucleotide, Biosensing Techniques, Metal Nanoparticles
Abstract

Knowledge of the interaction between aptamer and protein is integral to the design and development of aptamer-based biosensors. Nanoparticles functionalized with aptamers are commonly used in these kinds of sensors. As such, studies into how the number of aptamers on the nanoparticle surface influence both kinetics and thermodynamics of the binding interaction are required. In this study, aptamers specific for interferon gamma (IFN-γ) were immobilized on the surface of gold nanoparticles (AuNPs), and the effect of surface coverage of aptamer on the binding interaction with its target was investigated using fluorescence spectroscopy. The number of aptamers were adjusted from an average of 9.6 to 258 per particle. The binding isotherm between AuNPs-aptamer conjugate and protein was modeled with the Hill-Langmuir equation, and the determined equilibrium dissociation constant ( K ' D ) decreased 10-fold when increasing the coverage of aptamer. The kinetics of the reaction as a function of coverage of aptamer were also investigated, including the association rate constant ( k on ) and the dissociation rate constant ( k off ). The AuNPs-aptamer conjugate with 258 aptamers per particle had the highest k on , while the k off was similar for AuNPs-aptamer conjugates with different surface coverages. Therefore, the surface coverage of aptamers on AuNPs affects both the thermodynamics and the kinetics of the binding. The AuNPs-aptamer conjugate with the highest surface coverage is the most favorable in biosensors considering the limit of detection, sensitivity, and response time of the assay. These findings deepen our understanding of the interaction between aptamer and target protein on the particle surface, which is important to both improve the scientific design and increase the application of aptamer-nanoparticle based biosensor.

Published
2021
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49. Update to Our Reader, Reviewer, and Author Communities-April 2020.

Author

Burrows CJ, Wang S, Kim HJ, Meyer GJ, Schanze K, Lee TR, Lutkenhaus JL, Kaplan D, Jones C, Bertozzi C, Kiessling L, Mulcahy MB, Lindsley CW, Finn MG, Blum JD, Kamat P, Aldrich CC, Rowan S, Bin Liu, Liotta D, Weiss PS, Zhang D, Ganesh KN, Sexton P, Atwater HA, Gooding JJ, Allen DT, Voigt CA, Sweedler J, Schepartz A, Rotello V, Lecommandoux S, Sturla SJ, Hammes-Schiffer S, Buriak J, Steed JW, Wu H, Zimmerman J, Brooks B, Savage P, Tolman W, Hofmann TF, Brennecke JF, Holme TA, Merz KM Jr, Scuseria G, Jorgensen W, Georg GI, Wang S, Proteau P, Yates JR 3rd, Stang P, Walker GC, Hillmyer M, Taylor LS, Odom TW, Carreira E, Rossen K, Chirik P, Miller SJ, McCoy A, Shea JE, Zanni M, Murphy C, Scholes G, and Loo JA

Published
2020
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