For many years, it has been recognized that potential organic photovoltaic cells must be integrated into elements requiring high transparency. In most of such elements, sunlight is likely to be incident at large angles. Here it is demonstrated that light transmission can be largely decoupled from harvesting by optically tailoring an infrared shifted nonfullerene acceptor based organic cell architecture. A 9.67% power conversion efficiency at 50° incidence is achieved together with an average visual transmission above 50% at normal incidence. The deconstruction of a 1D nanophotonic structure is implemented to conclude that just two ¿/4 thick layers are essential to reach, for a wide incidence angle range, a higher than 50% efficiency increase relative to the standard configuration reference. In an outdoor measurement of vertically positioned 50% visible transparent cells, it is demonstrated that 9.80% of sunlight energy can be converted into electricity during the course of 1 day. Q.L., L.G., F.B., J.T., and J.M. acknowledge the financial support from the Spanish Ministry of Economy and Competitiveness (MINECO) through the “Severo Ochoa” program for Centres of Excellence in R&D (SEV2015-0522), from Fundació Privada Cellex, from Generalitat de Catalunya through the Impulsa-Llavor (Llav-00073) and CERCA programs, and also acknowledge financial support from MINECO through project MAT2017-89522-R. T.L. and X.Z. thank the NSFC (No. 21734001). F.B. also thanks the CONACyT international grants program.