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This study aims to investigate solar radiation pressure acting on the spherical geodetic satellites, Ajisai, LAGEOS-1, and LAGEOS-2. The solar radiation pressure coefficients ( C R ) are derived in two independent ways: (a) through precise orbit determination (POD) using satellite laser ranging (SLR) data, and (b) through modeling using the optical properties of the satellite surface material. The average C R value of Ajisai (1.039), as calculated from the time series of C R POD estimates every 15 days, is consistently smaller than those of LAGEOS-1 (1.140) and LAGEOS-2 (1.103). This difference can be explained by the fact that the surface of Ajisai is mostly covered by mirrors. The Ajisai C R values estimated by POD show remarkable semi-annual variation, which disagrees with the results of a previous study (Sengoku et al., 1995) predicting that the C R of Ajisai varies almost annually. We attribute this semi-annual variation to two physical reasons: the non-spherical additional cross-sectional area due to the “attached fitting ring” and the low reflectivity of the surface material in the polar regions. Furthermore, the solar radiation pressure acting on Ajisai varies annually in a direction perpendicular to the sun-satellite vector. Finally, the two independent C R values of Ajisai agree more when we assume a total solar irradiance of 1361 W/m2, whereas the value 1367 W/m2 has been commonly used in POD.