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To enhance the performance of rigid coaxial rotors across both hovering and high-speed cruising conditions, this study develops a novel aerodynamic optimization method that differentiates between the upper and lower rotors. Utilizing the lifting line and reformulated viscous vortex particle method (rVPM), this approach models the complex wake fields of coaxial rotors and accurately assesses the aerodynamic loads on the blades. The optimization of geometric properties such as planform configuration and nonlinear twist is conducted through an innovative solver that integrates simulated annealing with the Nelder–Mead algorithm, ensuring both rapid and comprehensive optimization results. Comparative analyses demonstrate that these tailored geometric adjustments significantly enhance efficiency in both operational states, surpassing traditional methods. This research provides a strategic framework for addressing the varied aerodynamic challenges presented by different flight states in coaxial rotor design.