Search

Development of nanowire photonics requires integration of different nanowire components into highly ordered functional heterostructures. Herein, we report a sequential self-assembly of binary molecular components into branched nanowire heterostructures (BNHs) via lattice-matched epitaxial growth, in which the microribbon backbone of 2,5-Bis(5-tert-butyl-2-benzoxazolyl)thiophene (BBOT) functions as blue-emitting microlaser source to pump the nanowire branches of BODIPY. By constructing Au electrodes on both branch sides and measuring the photocurrent in them, we successfully realize the integration of an organic laser and a power meter in a single device. This work provides a new insight into the integration of 1D organic nanostructures into BNHs for realizing organic multifunctional photonic devices. [ABSTRACT FROM AUTHOR]

Coherent light signals generated at the nanoscale are crucial to the realization of photonic integrated circuits. Self-assembled nanowires from organic dyes can provide both a gain medium and an effective resonant cavity, which have been utilized for fulfilling miniaturized lasers. Excited-state intramolecular proton transfer (ESIPT), a classical molecular photoisomerization process, can be used to build a typical four-level system, which is more favorable for population inversion. Low-power driven lasing in proton-transfer molecular nanowires with an optimized ESIPT energy-level process has been achieved. With high gain and low loss from the ESIPT, the wires can be applied as effective FP-type resonators, which generated single-mode lasing with a very low threshold. The lasing wavelength can be reversibly switched based on a conformation conversion of the excited keto form in the ESIPT process. [ABSTRACT FROM AUTHOR]

Stapelkunde: Zwei verschiedene, aber verwandte Naphthalene bilden, gesteuert durch ihre H ‐ Brückenbindungen und π ‐ π ‐ Stapelung, unterschiedliche Nanostrukturen (siehe Bild). Diese Nanostrukturen wiesen einzigartige Merkmale hinsichtlich photonischer Begrenzung und Lichtweiterleitung auf, was einen Einsatz in nanophotonischen Schaltkreisen nahelegt. [ABSTRACT FROM AUTHOR]