Search

Holmium-166 is a high-energy β

In the framework of an international BIPM comparison (Bureau International des Poids et Mesures), the activity standardization of

In National Metrology Institutes like LNE-LNHB, renewal and improvement of the instrumentation is an important task. Nowadays, the current trend is to adopt digital boards, which present numerous advantages over the standard electronics. The feasibility of an on-line fulfillment of nuclear-instrumentation functionalities using a commercial FPGA-based (Field-Programmable Gate Array) board has been validated in the case of TDCR primary measurements (Triple to Double Coincidence Ratio method based on liquid scintillation). The new applications presented in this paper have been included to allow either an on-line processing of the information or a raw-data acquisition for an off-line treatment. Developed as a complementary tool for TDCR counting, a time-to-digital converter specifically designed for this technique has been added. In addition, the description is given of a spectrometry channel based on the connection between conventional shaping amplifiers and the analog-to-digital converter (ADC) input available on the same digital board. First results are presented in the case of α- and γ-counting related to, respectively, the defined solid angle and well-type NaI(Tl) primary activity techniques. The combination of two different channels (liquid scintillation and γ-spectrometry) implementing the live-time anticoincidence processing is also described for the application of the 4πβ–γ coincidence method. The need for an optimized coupling between the analog chain and the ADC stage is emphasized. The straight processing of the signals delivered by the preamplifier connected to a HPGe detector is also presented along with the first development of digital filtering.

The Publisher regrets that this article is an accidental duplication of an article that has already been published, doi:10.1016/j.apradiso.2010.01.040. The duplicate article has therefore been withdrawn.

In this paper we present a prototype of a new class of detectors, metallic magnetic calorimeters operating at cryogenic temperatures, which we are developing for absolute activity measurement of low-energy-emitting radionuclides. We explain the detection principle and give a detailed description of the realisation of the prototype, containing an (55)Fe source inside the detector absorber. The analysis of first data taken with this detector is presented and the result of activity measurement compared with liquid scintillation counting. Some ways for reducing the uncertainty that can be achieved with this new technique are proposed.

(67)Ga is an interesting radionuclide as it is widely used in nuclear medicine. The meta-stable level related to the 93.3keV gamma-transition represents the main difficulty when using the coincidence method to standardize this radionuclide. The 4pi(LS)beta-gamma anti-coincidence system implemented at LNHB is based on the use of electronic modules specifically designed for radioactivity metrology. On the contrary to classical coincidence systems, activity measurements of (67)Ga are carried out as for prompt beta-gamma emitters; indeed, when using a live-timed anti-coincidence system with extendable dead times, the problem due to the excess of counting generated by the meta-stable level is avoided. Considering that the standardization of (67)Ga does not depend on the decay scheme parameters (except for the half-life), the measurement of the gamma-emission intensities has been performed. The standardization of this radionuclide was also a good opportunity for a new participation of our laboratory in the SIR of (67)Ga (International Reference System); the result obtained with the 4pi(LS)beta-gamma anti-coincidence system is compared with those submitted by other National Metrology Institutes (NMIs). The non-extendable dead times used in most of the participations could be one of the causes responsible for the abnormal dispersion of the results. The optimization of the standard solution of (67)Ga for the radioactive source preparation is also discussed.

Applications such as environment monitoring implying alpha emitters activity measurement associated with isotope identification, require high-energy resolution detectors. Conventional silicon detectors are inexpensive therefore widely used, although intrinsically limited in energy resolution. Thermal detection principle of cryogenic detectors introduces a breakthrough in alpha particle measurement. For the first time, spectra with 5.5 keV FWHM energy resolution have been obtained for several external alpha emitting sources using a copper–germanium bolometer specially developed for alpha spectrometry.

This article is an overview of the capabilities of a 4 pi(LS)beta-gamma coincidence counting system based on a liquid scintillation detector in the beta-channel. Equipped with a three-photomultiplier apparatus designed for the triple to double coincidence ratio (TDCR) method, the 4 pi(LS)beta-gamma coincidence system developed at LNHB combines the two techniques. The 4 pi(LS)beta-gamma counting setup records the different types of scintillation events between photomultipliers (double and triple coincidences) and the associated gamma-spectra according to a bi-dimensional configuration. When measuring the activity of a (54)Mn solution, the extrapolation method is carried out by defocusing the photomultipliers; this procedure allows the measurement of gamma-ray sensitivity of the scintillation cocktail in the 835 keV energy region. In addition, in the framework of a (65)Zn standardization, 4 pi(LS)beta-gamma measurements are compared with standard 4 pi(PC)beta-gamma anticoincidence counting using a proportional counter in the beta-channel.

Cryogenic detectors offer remarkably better energy resolutions than those achievable with conventional semiconductor or scintillation detectors. With the additional asset of a detection efficiency close to unity for low-energy X-ray photons and electrons, these detectors have the potential to perform X-ray, gamma and electron spectroscopy of a hitherto unknown quality, in particular at low energies. Two types of cryogenic detectors are described and the results of prototype detectors are presented.

Half-life measurements have been carried out at LNHB for 88Y using a 4pi gamma-ionisation chamber and for 89Sr using a proportional counter. The determined half-life values and associated standard uncertainties are 106.63 +/- 0.05 d for 88Y and 50.65 +/- 0.05 d for 89Sr, being consistent with relevant values reported in literature. Based on the present results and relevant literature values revised recommended half-life values and associated standard uncertainties are proposed, viz. 106.626 +/- 0.021 d for 88Y and 50.57 +/- 0.03 d for 89Sr.

Microcalorimeters (or bolometers) operated at temperatures below 100 mK allow individual counting of photons and electrons with a very low energy detection threshold. The physics is based on the pulse temperature increase of the target (or absorber) of the detector due to the complete absorption of both electrons and photons. Since this target can be constructed with a perfect 4-pi geometry, a bolometer offers potentially a new method for absolute activity measurements of radionuclides emitting low-energy radiation. In this paper we present our first results of a feasibility study of activity standardization of a 55Fe solution with a prototype 4-pi bolometer.

In the field of radioactivity measurement, there is a constant need for highly specialized electronic modules such as ADCs, amplifiers, discriminators, dead-time modules, etc. But sometimes it is almost impossible to find on the market the modules having the performances corresponding to our needs. The purpose of the module presented here, called MTR2 (Module de Temps-mort Reconductible), is to process, in terms of pulse height discrimination and dead-time corrections, the pulses delivered by the detectors used in counting systems. This dead-time, of the extendible type, is triggered by both the positive and negative parts of the incoming pulse and the dead-time corrections are made according to the live-time method. This module, which has been developed and tested at LPRI, can be used alone in simple counting channels or in more complex systems such as coincidence systems. The philosophy governing the choice and the implementation of this type of dead-time as well as the system used for the dead-time corrections is presented. The electronic scheme and the performances are also presented. This module is available in the NIM standard.