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The main goal of this paper is to study pollution during sea breeze days in the Split town center, which is placed near the industrial area with three cement plants and one asbestos cement plant, as well as a harbor with high traffic, and investigate the sources of pollution with SO2 and its relation to atmospheric parameters using stepwise multiple linear regression (MLR). The hourly temperature difference from the time of the sea breeze lull (dT) was considered in evaluating the influence of meteorological parameters on hourly pollutant concentrations. It was found that the wind direction index (WDI) is a significant predictor for the sea breeze, and wind speed, relative humidity, and dT are significant for the land breeze. A very high index of agreement of 0.9 was obtained by the MLR model for the land breeze, and 0.8 for the sea breeze. Low SO2 concentrations are observed at night, and increased values are found between 0800 and 1800 UTC. With WDI being the only predictor during sea breeze, local traffic is found to be the main anthropogenic source of SO2 pollution. [ABSTRACT FROM AUTHOR]