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This study develops a quantitative climatology of water vapour exchange between the atmospheric boundary layer (ABL) and free troposphere (FT) over eastern China. The exchange flux is estimated for January, April, July and October over 7 years based on a water vapour budget equation using simulated meteorological data. The spatiotemporal characteristics and occurrence mechanism of ABL–FT water vapour exchange and its relationship with the El Niño–Southern Oscillation (ENSO) are revealed: (1) the vertical exchange flux varies regionally and seasonally, with downward transport to maintain ABL moisture during winter and autumn in the northern region and persistent output to humidify the FT in the southern region, particularly in summer. Additionally, the vertical exchange flux is also topographic dependent. (2) The vertical motion at the ABL top, which is produced by the dynamic forcing of the terrain on synoptic winds, is the dominant mechanism for the water vapour vertical exchange over the long-term average. The evolution of the vertical exchange flux within 1 d scale is driven by the ABL diurnal cycle. (3) The interannual variation of water vapour vertical exchange is correlated with ENSO. A triple antiphase distribution with negative–positive–negative anomalies from north to south exists in La Niña years (and vice versa in El Niño years), which corresponds to the spatial pattern of anomalous precipitation. This phenomenon is mainly due to the alteration of vertical velocity and water vapour content at the ABL top varying with ENSO phases. These results provide new insight into understanding the atmospheric water cycle. [ABSTRACT FROM AUTHOR]

While the impact of the El Niño–Southern Oscillation (ENSO) on the stratospheric circulation has been long recognized, its effects on stratospheric ozone have been less investigated. In particular, the impact on ozone of different ENSO flavors, eastern Pacific (EP) El Niño and central Pacific (CP) El Niño, and the driving mechanisms for the ozone variations have not been investigated to date. This study aims to explore these open questions by examining the anomalies in advective transport, mixing and chemistry associated with different El Niño flavors (EP and CP) and La Niña in the Northern Hemisphere in boreal winter. For this purpose, we use four 60-year ensemble members of the Whole Atmospheric Community Climate Model version 4. The results show a significant ENSO signal on the total column ozone (TCO) during EP El Niño and La Niña events. During EP El Niño events, TCO is significantly reduced in the tropics and enhanced at middle and high latitudes in boreal winter. The opposite response has been found during La Niña. Interestingly, CP El Niño has no significant impact on extratropical TCO, while its signal in the tropics is weaker than for EP El Niño events. The analysis of mechanisms reveals that advection through changes in tropical upwelling is the main driver for ozone variations in the lower tropical stratosphere, with a contribution of chemical processes above 30 hPa. At middle and high latitudes, stratospheric ozone variations related to ENSO result from combined changes in advection by residual circulation downwelling and changes in horizontal mixing linked to Rossby wave breaking and polar vortex anomalies. The impact of CP El Niño on the shallow branch of the residual circulation is small, and no significant impact is found on the deep branch. [ABSTRACT FROM AUTHOR]

We investigate the temporal variations of ground-level ozone and balloon-based ozone profiles at Pohang (36.02 ∘ N, 129.23 ∘ E) in the Korean Peninsula. Satellite measurements and chemical reanalysis products are also intercompared to address their capability of providing consistent information on the temporal and vertical variability of atmospheric ozone. Sub-seasonal variations of the summertime lower-tropospheric ozone exhibit a bimodal pattern related to atmospheric weather patterns modulated by the East Asian monsoon circulation. The peak ozone abundances occur during the pre-summer monsoon with enhanced ozone formation due to favorable meteorological conditions (dry and sunny). Ozone concentrations reach their minimum during the summer monsoon and then re-emerge in autumn before the winter monsoon arrives. Profile measurements indicate that ground-level ozone is vertically mixed up to 400 hPa in summer, while the impact of the summer monsoon on ozone dilution is found up to 600 hPa. Compared to satellite measurements, reanalysis products largely overestimate ozone abundances in both the troposphere and stratosphere and give inconsistent features of temporal variations. Nadir-viewing measurements from the Ozone Monitoring Instrument (OMI) slightly underestimate the boundary layer ozone but represent the bimodal peaks of ozone in the lower troposphere and the interannual changes in the lower-tropospheric ozone in August well, with higher ozone concentrations during strong El Niño events and low ozone concentrations during the 2020 La Niña event. [ABSTRACT FROM AUTHOR]

The tropospheric water vapour data record generated within the ESA Climate Change Initiative Water Vapour project (ESA TCWV-COMBI) is used to evaluate the interannual variability of global climate models (CMIP6 framework under AMIP scenarios) and reanalysis (ECMWF ERA5). The study focuses on the tropical belt, with a separation of oceanic and continental situations. The intercomparison is performed according to the probability density function (PDF) of the total column water vapour (TCWV) defined yearly from the daily scale, as well as its evolution with respect to large-scale overturning circulation. The observational diagnostic relies on the decomposition of the tropical atmosphere into percentile of the PDF and into dynamical regimes defined from the atmospheric vertical velocity. Large variations are observed in the patterns among the data records over tropical land, while oceanic situations show more similarities in both interannual variations and percentile extremes. The signatures of El Niño and La Niña events, driven by sea surface temperatures, are obvious over the oceans. Differences also occur over land for both trends (a strong moistening is observed in the ESA TCWV-COMBI data record, which is absent in CMIP6 models and ERA5) and extreme years. The discrepancies are probably associated with the scene selection applied in the data process. Since the results are sensitive to the scene selection applied in the data process, discrepancies are observed among the datasets. Therefore, the normalization process is employed to analyse the time evolution with respect to the mean state. Other sources of differences, linked to the models and their parametrizations, are highlighted. [ABSTRACT FROM AUTHOR]

We analyzed air samples collected on board a C-130 cargo aircraft over the western North Pacific from May 2012 to March 2020 for atmospheric δ (O 2 / N 2) and CO 2 amount fraction. Observations were corrected for significant artificial fractionation of O 2 and N 2 caused by thermal diffusion during the air sample collection using the simultaneously measured δ (Ar / N 2). The observed seasonal cycles of the δ (O 2 / N 2) and atmospheric potential oxygen (δ (APO)) varied nearly in opposite phase to the cycle of the CO 2 amount fraction at all latitudes and altitudes. Seasonal amplitudes of δ (APO) decreased with latitude from 34 to 25 ∘ N, as well as with increasing altitude from the surface to 6 km by 50 %–70 %, while those of the CO 2 amount fraction decreased by less than 20 %. By comparing the observed values with the simulated δ (APO) and CO 2 amount fraction values generated by an atmospheric transport model, we found that the seasonal δ (APO) cycle in the middle troposphere was modified significantly by a combination of the northern and southern hemispheric seasonal cycles due to the interhemispheric mixing of air. The simulated δ (APO) underestimated the observed interannual variation in δ (APO) significantly, probably due to the interannual variation in the annual mean air–sea O 2 flux. Interannual variation in δ (APO) driven by the net marine biological activities, obtained by subtracting the assumed solubility-driven component of δ (APO) from the total variation, indicated a clear influence on annual net sea–air marine biological O 2 flux during El Niño and net air–sea flux during La Niña. By analyzing the observed secular trends of δ (O 2 / N 2) and the CO 2 amount fraction, global average terrestrial biospheric and oceanic CO 2 uptakes for the period 2012–2019 were estimated to be (1.8±0.9) and (2.8±0.6) Pg a -1 (C equivalents), respectively. [ABSTRACT FROM AUTHOR]

The Amazon experiences fires every year, and the resulting biomass burning aerosols, together with cloud particles, influence the penetration of sunlight through the atmosphere, increasing the ratio of diffuse to direct photosynthetically active radiation (PAR) reaching the vegetation canopy and thereby potentially increasing ecosystem productivity. In this study, we use the NASA Goddard Earth Observing System (GEOS) model with coupled aerosol, cloud, radiation, and ecosystem modules to investigate the impact of Amazon biomass burning aerosols on ecosystem productivity, as well as the role of the Amazon's clouds in tempering this impact. The study focuses on a 7-year period (2010–2016) during which the Amazon experienced a variety of dynamic environments (e.g., La Niña, normal years, and El Niño). The direct radiative impact of biomass burning aerosols on ecosystem productivity – called here the aerosol diffuse radiation fertilization effect – is found to increase Amazonian gross primary production (GPP) by 2.6 % via a 3.8 % increase in diffuse PAR (DFPAR) despite a 5.4 % decrease in direct PAR (DRPAR) on multiyear average during burning seasons. On a monthly basis, this increase in GPP can be as large as 9.9 % (occurring in August 2010). Consequently, the net primary production (NPP) in the Amazon is increased by 1.5 %, or ∼92 TgCyr-1 – equivalent to ∼37 % of the average carbon lost due to Amazon fires over the 7 years considered. Clouds, however, strongly regulate the effectiveness of the aerosol diffuse radiation fertilization effect. The efficiency of this fertilization effect is the highest in cloud-free conditions and linearly decreases with increasing cloud amount until the cloud fraction reaches ∼0.8 , at which point the aerosol-influenced light changes from being a stimulator to an inhibitor of plant growth. Nevertheless, interannual changes in the overall strength of the aerosol diffuse radiation fertilization effect are primarily controlled by the large interannual changes in biomass burning aerosols rather than by changes in cloudiness during the studied period. [ABSTRACT FROM AUTHOR]

Effects of the El Niño–Southern Oscillation (ENSO) on the interannual variability in spring aerosols over East Asia are investigated using the Modern Era Retrospective analysis for Research and Applications Version 2 (MERRA-2) reanalysis aerosol data. Results show that the ENSO has a crucial effect on the spring aerosols over mainland South East Asia, southern China, and the ocean south of Japan. The above-normal (below-normal) aerosols are found over these regions during the ensuing spring of El Niño (La Niña). In contrast to the local aerosol diffusion in winter, the ENSO affects East Asian aerosols in the following spring mainly via the modulation of upstream aerosol generation and transport processes. The underlying physical mechanism is that during the ensuing spring of El Niño (La Niña), the dry (wet) air and reduced (enhanced) precipitation are beneficial for the increase (reduction) in biomass burning activities over northern mainland South East Asia, resulting in more (fewer) carbonaceous aerosol emissions. On the other hand, the anomalous anticyclone (cyclone) over the north-western Pacific (WNP) associated with El Niño (La Niña) enhances (weakens) the low-level south-westerly wind from northern mainland South East Asia to southern Japan, which transports more (less) carbonaceous aerosol downstream. Anomalous precipitation plays a role in reducing aerosols over the source region, but its washout effect over the downstream region is limited. The ENSO's impact on the ensuing spring aerosols is mainly attributed to the eastern Pacific ENSO rather than the central Pacific ENSO. [ABSTRACT FROM AUTHOR]

The connection between the dominant mode of interannual variability in the tropical troposphere, the El Niño–Southern Oscillation (ENSO), and the entry of stratospheric water vapor is analyzed in a set of model simulations archived for the Chemistry-Climate Model Initiative (CCMI) project and for Phase 6 of the Coupled Model Intercomparison Project. While the models agree on the temperature response to ENSO in the tropical troposphere and lower stratosphere, and all models and observations also agree on the zonal structure of the temperature response in the tropical tropopause layer, the only aspect of the entry water vapor response with consensus in both models and observations is that La Niña leads to moistening in winter relative to neutral ENSO. For El Niño and for other seasons, there are significant differences among the models. For example, some models find that the enhanced water vapor for La Niña in the winter of the event reverses in spring and summer, some models find that this moistening persists, and some show a nonlinear response, with both El Niño and La Niña leading to enhanced water vapor in both winter, spring, and summer. A moistening in the spring following El Niño events, the signal focused on in much previous work, is simulated by only half of the models. Focusing on Central Pacific ENSO vs. East Pacific ENSO, or temperatures in the mid-troposphere compared with temperatures near the surface, does not narrow the inter-model discrepancies. Despite this diversity in response, the temperature response near the cold point can explain the response of water vapor when each model is considered separately. While the observational record is too short to fully constrain the response to ENSO, it is clear that most models suffer from biases in the magnitude of the interannual variability of entry water vapor. This bias could be due to biased cold-point temperatures in some models, but others appear to be missing forcing processes that contribute to observed variability near the cold point. [ABSTRACT FROM AUTHOR]

Stratosphere-to-troposphere mass transport to the planetary boundary layer (STT-PBL) peaks over the western United States during boreal spring, when deep stratospheric intrusions are most frequent. The tropopause-level jet structure modulates the frequency and character of intrusions, although the precise relationship between STT-PBL and jet variability has not been extensively investigated. In this study, we demonstrate how the North Pacific jet transition from winter to summer leads to the observed peak in STT-PBL. We show that the transition enhances STT-PBL through an increase in storm track activity which produces highly amplified Rossby waves and more frequent deep stratospheric intrusions over western North America. This dynamic transition coincides with the gradually deepening PBL, further facilitating STT-PBL in spring. We find that La Niña conditions in late winter are associated with an earlier jet transition and enhanced STT-PBL due to deeper and more frequent tropopause folds. An opposite response is found during El Niño conditions. El Niño–Southern Oscillation (ENSO) conditions also influence STT-PBL in late spring or early summer, during which time La Niña conditions are associated with larger and more frequent tropopause folds than both El Niño and ENSO-neutral conditions. These results suggest that knowledge of ENSO state and the North Pacific jet structure in late winter could be leveraged for predicting the strength of STT-PBL in the following months. [ABSTRACT FROM AUTHOR]

The Asian summer monsoon anticyclone (ASMA) has been a topic of intensive research in recent times regarding its variability in dynamics, chemistry and radiation. This work explores the spatial variability and the trends of the ASMA using observational and reanalysis data sets. Our analysis indicates that the spatial extent and magnitude of the ASMA is greater during July and August than in June and September. The decadal variability of the anticyclone is very large at the edges of the anticyclone compared with the core region. Significant decadal variability is observed in the northeastern and southwestern parts of the ASMA with reference to the 1951–1960 period. The strength of the ASMA shows a drastic increase in zonal wind anomalies in terms of temporal variation. Furthermore, our results show that the extent of the anticyclone is greater during the active phase of the monsoon, strong monsoon years, and La Niña events. Significant warming with strong westerlies is observed exactly over the Tibetan Plateau from the surface to the tropopause during the abovementioned periods. Our results support the existence of transport process over the Tibetan Plateau and the Indian region during active, strong monsoon years and during strong La Niña years. Therefore, it is recommended that the different phases of the monsoon be taken into account when interpreting the variability of pollutants and trace gases in the anticyclone. [ABSTRACT FROM AUTHOR]

Spatial differences in the monthly baseline CO2 since 1992 from Mauna Loa (mlo, 19.5 ∘ N, 155.6 ∘ W, 3379 m), Cape Grim (cgo, 40.7 ∘ S, 144.7 ∘ E, 94 m), and South Pole (spo, 90 ∘ S, 2810 m) are examined for consistency between four monitoring networks. For each site pair, a composite based on the average of NOAA, CSIRO, and two independent Scripps Institution of Oceanography (SIO) analysis methods is presented. Averages of the monthly standard deviations are 0.25, 0.23, and 0.16 ppm for mlo–cgo, mlo–spo, and cgo–spo respectively. This high degree of consistency and near-monthly temporal differentiation (compared to CO2 growth rates) provide an opportunity to use the composite differences for verification of global carbon cycle model simulations. Interhemispheric CO2 variation is predominantly imparted by the mlo data. The peaks and dips of the seasonal variation in interhemispheric difference act largely independently. The peaks mainly occur in May, near the peak of Northern Hemisphere (NH) terrestrial photosynthesis/respiration cycle. February–April is when interhemispheric exchange via eddy processes dominates, with increasing contributions from mean transport via the Hadley circulation into boreal summer (May–July). The dips occur in September, when the CO2 partial pressure difference is near zero. The cross-equatorial flux variation is large and sufficient to significantly influence short-term Northern Hemisphere growth rate variations. However, surface–air terrestrial flux anomalies would need to be up to an order of magnitude larger than found to explain the peak and dip CO2 difference variations. Features throughout the composite CO2 difference records are inconsistent in timing and amplitude with air–surface fluxes but are largely consistent with interhemispheric transport variations. These include greater variability prior to 2010 compared to the remarkable stability in annual CO2 interhemispheric difference in the 5-year relatively El Niño-quiet period 2010–2014 (despite a strong La Niña in 2011), and the 2017 recovery in the CO2 interhemispheric gradient from the unprecedented El Niño event in 2015–2016. [ABSTRACT FROM AUTHOR]

Using COSMIC GPS Radio Occultation (RO) observations from January 2007 to December 2016, we retrieved temperature profiles with the height resolution of about 0.1 km in the upper troposphere and lower stratosphere (UTLS). We investigated the distribution of static stability (N2) and the zonal structure of the tropopause inversion layer (TIL) in the tropics, where a large change in the temperature gradient occurs associated with sharp variations in N2. We show the variations in the mean N2 profiles in coordinates relative to the cold-point tropopause (CPT). A very thin (<1 km) layer is found with average maximum N2 in the range of 11.0– 12.0×10-4 s -2. The mean and standard deviation of TIL sharpness, defined as the difference between the maximum N2 (max⁡N2) and minimum N2 (min⁡N2) within ±1 km of the CPT, is (10.5±3.7)×10-4 s -2. The max⁡N2 is typically located within 0.5 km above CPT. We focused on the variation in TIL sharpness in two longitude regions, 90–150 ∘ E (Maritime Continent; MC) and 170–230 ∘ E (Pacific Ocean; PO), with different land–sea distribution. Seasonal variations in TIL sharpness and thickness were related to the deep convective activity represented by low outgoing longwave radiation (OLR) during the Australian and Asian monsoons. The deviation from the mean sharpness (sharpness anomaly) was out of phase with the OLR anomaly in both the MC and PO. The correlation between the sharpness anomaly over the MC and PO and the sea surface temperature (SST) Niño 3.4 index was -0.66 and +0.88 , respectively. During La Niña (SST Niño 3.4 <-0.5 K) in the MC and El Niño (SST Niño 3.4 >+0.5 K) in the PO, warmer SSTs in the MC and PO produce more active deep convection that tends to force the air upward to the tropopause layer and increase the temperature gradient there. The intraseasonal variation in sharpness anomaly during slow and fast episodes of the Madden–Julian Oscillation (MJO) demonstrates that eastward propagation of the positive sharpness anomaly is associated with organized deep convection. Deep convection during MJO will tend to decrease N2 below CPT and increase N2 above CPT, thus enlarging the TIL sharpness. Convective activity in the tropics is a major control on variations in tropopause sharpness at intraseasonal to interannual timescales. [ABSTRACT FROM AUTHOR]