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In this paper, we prove sharp isoperimetric inequalities for lower order eigenvalues of Neumann Laplacian on bounded domains in both compact and noncompact rank-1 symmetric spaces. Our results generalize the work of Wang and Xia for bounded domains in the hyperbolic space (Xia and Wang in Math Ann 385(1–2):863–879, 2023), and Szegö–Weinberger inequalities in rank-1 symmetric spaces obtained by Aithal and Santhanam (Trans Am Math Soc 348(10):3955–3965, 1996). [ABSTRACT FROM AUTHOR]