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Start Over Author "Touzé, Ewen" Journal chemical communications cambridge england

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1. Electrocatalytic reduction of CO 2 in water by a C -functionalized Ni-cyclam complex grafted onto carbon.

Author

Forget A, Regnacq M, Orain C, Touzé E, Lelong E, Brandily C, Bernard H, Tripier R, and Le Poul N

Abstract

We present here a novel strategy based on the covalent grafting of a C -functionalized Ni-cyclam complex onto glassy carbon to achieve heterogeneous electrocatalytic CO 2 reduction in neutral water at low overpotential (-500 mV vs. NHE), with moderate turnover number (TON = 454), high selectivity (85% CO produced) and good faradaic efficiency (56% CO). Direct comparison with the N -functionalized Ni-cyclam analogue highlights the benefits of this approach in terms of CO 2 electroreduction.

Published
2022
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