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This paper proposes a hyperspectral imaging technique for capturing radiative images at a high temporal–spatial resolution, for the purpose of spectrally visualizing the instantaneous combustion behaviors of single coal particles. We initially use a hyperspectral imaging device to record the combustion processes of two types of single pulverized coal particles on a McKenna flat-flame burner. From the snapshot images captured by the device, we observe the combustion processes, ignition characteristics, flame morphologies, and sizes of the two single coal particles. The observations indicate that the two single coal particles undergo volatile release/combustion and char ignition/oxidation during the luminous combustion process; moreover, both particles exhibit homogeneous ignition characteristics under the experimental conditions. Furthermore, based on the spectral radiative intensity images obtained via the device, the soot temperature and volume fraction images of the two single coal particles in the envelope flame are obtained at different burning times. Thereafter, the influences of the combustion behaviors and soot formation mechanisms on the distribution rules of the soot temperature and concentration at different combustion periods are discussed. Finally, the temperature and apparent spectral emissivity values of the two single char particles during the char oxidation process are also calculated to analyze their combustion behaviors. The results show that the temperature changes within a relatively narrow range with respect to the burning time during the oxidation stage, whereas the spectral emissivity continues to increase with the oxidation of chars and subsequently decreases. [ABSTRACT FROM AUTHOR]