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Start Over Author "Song, Haobin" Journal dalton transactions: an international journal of inorganic chemistry

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1. Versatile halogenation via a CNHC^Csp3 palladacycle intermediate.

Author

Teng, Qiaoqiao, Liu, Ziwei, Song, Haobin, Liu, Jiayu, Zhao, Yaru, Jiang, Weihua, Huynh, Han Vinh, and Meng, Qi

Subjects
*HALOGENATION, *PROTON transfer reactions, *LIGANDS (Chemistry), *ELECTRONS, *CHARITABLE giving
Abstract

Stable cyclopalladated complexes containing an (sp3)C–Pd bond were synthesized via α-CH2 deprotonation and palladation of N-alkyl groups of carbene ligands bearing electron-withdrawing substituents. The strong electron donating strengths of the resulting CNHC^Csp3 chelators were experimentally identified, and the palladacycle underwent template-directed, versatile C-halogenation with X2. [ABSTRACT FROM AUTHOR]

Published
2023
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