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The synthesis of Laser-Induced Graphene (LIG) through the laser ablation process of carbon-containing materials is a rapid and scalable process which enables the production of graphene in a cost-effective manner. In recent years, metal oxide – graphene composite electrodes have gained a lot of importance due to their use in various Energy Storage Devices (ESDs). In our investigation, we manufacture composite electrodes of manganese dioxide (MnO 2) and LIG through a hydrothermal process and use it as electrodes in Flexible Supercapacitors. This method deviates from traditional procedures as it eliminates the requirement for binders in creating composite electrodes, given that MnO 2 can be directly deposited onto the LIG electrodes. The assembled all-Flexible Supercapacitor (FSC), featuring unique LIG-MnO 2 composite electrodes, showcased a remarkable areal capacitance of 66.5 mF cm−2 at 5 mV s−1 scan rate. The device also exhibited a very high areal energy density (2.3 mWh cm−2) and power density (19.7 mW cm−2) at 0.2 mA cm−2 current density. Also, 82 % capacitance retention was observed at the end of 2000 cycles and the device also exhibited a good flexibility during bending tests, as evidenced by an 80 % capacitance retention after 100 bending cycles. [ABSTRACT FROM AUTHOR]