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• Embodied and operational carbon tradeoffs in building envelopes are studied. • Envelope variables include wall assemblies, WWRs, glazing and shading. • Energy decarbonization models are used to determine the 30-year operational carbon. • Results show the importance of a total carbon approach to envelope design. • Over or under insulation can result in waste of 10–150 kgCO 2 e/m2. The building envelope has a substantial influence on a building's life cycle operational and embodied carbon emissions. Window-to-wall ratios, wall assemblies, shading and glazing types, have been shown to have a significant impact on total emissions. This paper provides building designers, owners, and policy makers with actionable guidance and a prioritization framework for establishing co-optimized lifecycle carbon performance of facade assembly components in a broad spectrum of climate contexts and energy carbon intensities. A large parametric study of building envelopes is conducted using building performance simulation and cradle-to-gate embodied carbon calculations in 6 US cities. The authors derive the total carbon emissions optimization for commercial office and residential space types using standard code-reference models and open-source lifecycle data. Comparisons between optimal total carbon solutions and (i) optimal operational carbon and (ii) minimum required assemblies, show the impact of under and over investing in envelope-related efficiency measures for each climate. Results show how the relationship between embodied and operational carbon is highly localized, that optimal design variables can vary significantly. In low carbon intensity energy grids, over investment in envelope embodied carbon can exceed as 10 kgCO 2 e/m2, while under investment in high carbon intensity grids can be higher than 150 kgCO 2 e/m2. [ABSTRACT FROM AUTHOR]