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In recent years, coal-fired power plants contribute the biggest part of power generation in China. Challenges of energy conservation and emission reduction of the coal-fired power plant encountering with a rapid growth due to the rising proportion of renewable energy generation in total power generation. Energy saving power generation dispatch (ESPGD) based on power units sorting technology is a promising approach to meet the challenge. Therefore, it is crucial to establish a reasonable and feasible multi-index comprehensive evaluation (MICE) framework for assessing the performance of coal-fired power units accessed by the power grid. In this paper, a hierarchical multiple criteria evaluation system was established. Except for the typical economic and environmental indices, the evaluation system considering operational flexibility and power quality indices either. A hybrid comprehensive evaluation model was proposed to assess the unit operational performance. The model is an integration of grey relational analysis (GRA) with analytic hierarchy process (AHP) and a novel entropy-based method (abbreviate as BECC) which integrates bootstrap method and correlation coefficient (CC) into entropy principle to get the objective weight of indices. Then a case study on seven typical 600 megawatts coal-fired power units was carried out to illustrate the proposed evaluation model, and a weight sensitivity analysis was developed in addition. The results of the case study shows that unit 4 has the power generating priority over the rest ones, and unit 2 ranks last, with the lowest grey relational degree. The weight sensitivity analysis shows that the environmental factor has the biggest sensitivity coefficient. And the validation analysis of the developed BECC weight method shows that it is feasible for the MICE model, and it is stable with an ignorable uncertainty caused by the stochastic factor in the bootstrapping process. The elaborate analysis of the result reveals that it is feasible to rank power units with the proposed evaluation model. Furthermore, it is beneficial to synthesize the updated multiple criteria in optimizing the power generating priority of coal-fired power units. [ABSTRACT FROM AUTHOR]