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This paper investigates the attitude control of rigid spacecraft in the presence of uncertainties, disturbances, and actuator faults. In order to effectively address these challenges and improve the performance of the system, a novel actor-critic neural-network-based fractional-order sliding mode control (ACNNFOSMC) has been developed for spacecraft. The integration of actor-critic neural network, fractional-order theory, and sliding mode control enables dual functionality: the actor-critic neural network serves to approximate the aggregate of uncertain parameters, disturbances, and actuator faults, thereby facilitating their compensation, while the fractional-order sliding mode control mechanism significantly improves the system's tracking precision and overall robustness against uncertainties. Theoretical analyses are presented to analyze the stability of the proposed control framework. Thorough examination via simulation experiments affirms the effectiveness and control precision of attitude of our proposed control strategy, even in complex operational scenarios. [ABSTRACT FROM AUTHOR]