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We present the first demonstration of an actively Q-switched orthogonally polarized dual-wavelength Nd:YLF/YVO4 Raman laser to our knowledge. The gain competition of the orthogonally polarized dual-wavelength fundamental laser at 1047 and 1053 nm was ultimately avoided by incorporating two Nd:YLF crystals into two laser resonators. By adjusting the gain or loss difference of two resonators, the pulse synchronization of the orthogonally polarized dual-wavelength Raman laser was realized. Benefitting from the efficient thermal stress and energy-transfer upconversion management of Nd:YLF crystal, a maximum dual-wavelength Raman output power of 4.5 W was obtained with M2