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In the practical operation of an electromagnetic pulse (EMP) simulator, the flashover phenomenon on the edge of polypropylene dielectrics dominates the insulation failure mode of a peaking capacitor. To analyze the characteristics of polypropylene film flashover voltage under high-pressure SF6, an experimental platform was established, and the pulse generator could output a pulse with a rise time of approximately 27 ns. The experiments were performed on finger electrodes, and the SF6 pressure was set from 0.1 to 1.0 MPa. The experimental results show that the relationship of flashover voltage and gas pressure could be divided into two regions: in low-pressure regions, the flashover voltage increases with the gas pressure linearly and in high-pressure regions, the growth of flashover voltage gradually slows down and approaches a saturation value. As the gap distance increases, the saturation point of gas pressure decreases, and even when close to 0.4 MPa, with a 9-mm gap distance, this unconventional phenomenon cannot be ignored, particularly in practical EMP simulators. When the high surface resistivity and the charge trap distribution on the polypropylene film are considered, the accumulation and emission of surface charges on the film might be the primary reason for the saturated phenomena. [ABSTRACT FROM AUTHOR]