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Circulating current can be decomposed into double line-frequency positive-, negative- and zero-sequence components under unbalanced voltage conditions. First, in order to decrease peak/rms value of arm current, double line-frequency circulating current should be eliminated. Second, ac-side current that consists of positive- and negative-sequence components under unbalanced voltage conditions should be regulated to track the reference signal. Furthermore, fundamental frequency circulating current caused by asymmetry of the upper and lower arm should be also removed. To effectively control ac-side current and eliminate all circulating currents, an arm current control strategy based on a decoupler and proportional-integral controller plus the vector proportional integral (VPI) controller is proposed in this paper. The proposed control strategy works well under balanced and unbalanced voltage conditions as well as asymmetry of the upper and lower arm. In addition, this paper proposes a design procedure for the VPI controller to reduce the uncertainty of this process. A three-phase modular multilevel converter simulation model is set up on PSCAD/EMTDC to verify the effectiveness of the proposed control strategy.