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Currently, bismuth oxychalcogenide family (Bi 2 O 2 X, X S, Se, Te), led by Bi 2 O 2 Se with unique characteristics, have emerged as promising candidates for high-performance optoelectronic devices. Herein, the novel Bi 2 O 2 S flowers with hierarchical structure have been successfully prepared via a facile hydrothermal method with only 3 h of reaction. The as-prepared Bi 2 O 2 S flower is composed of many ultrathin nanosheets (NSs) with a thickness of about 12–16 nm. And the possible formation mechanism of ultrathin NSs self-assembled Bi 2 O 2 S flowers is further analyzed. In addition, a self-powered infrared photodetector based on Bi 2 O 2 S flowers, which can work without an external power, is designed. Under illumination at 850 nm light, the Bi 2 O 2 S flowers photodetector exhibits well photoresponse switching behaviors, of which the high responsivity, specific detectivity and fast response time reach up to 9.48 mA/W, 9.96 × 1010 Jones and 227.7 ms, respectively. Of particular note, the Bi 2 O 2 S flowers photodetector also possesses the eximious stability. [Display omitted] ● The Bi 2 O 2 S flowers composed of 2D ultrathin nanosheets were prepared on the fluorine-doped tin oxide substrate. ● The Bi 2 O 2 S flowers infrared photodetector exhibits a high responsivity of 9.48 mA/W and detectivity of 9.96 × 1010 Jones. ● The Bi 2 O 2 S flowers infrared photodetector possesses eximious stability, and can operated without an external power source. [ABSTRACT FROM AUTHOR]