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Abstract The sustainability of the water-energy-food (WEF) nexus is a significant challenge faced by developing countries, especially China. Evaluating the sustainability status of China's water-energy-food, and improving its sustainable use, may provide good physical conditions to support China's future development. This paper applied the Pressure, State, and Response (PSR) model to select evaluation indexes. A combination weighting method was used to combine two objective weighting methods to determine index weights. The study constructed the classical field, the limited field, and the matter-element to be evaluated. This allowed the establishment of an improved matter-element extension model to evaluate the sustainability of the water-energy-food nexus; the model was then used to quantitatively evaluate the sustainability of China's water-energy-food nexus. The simulation results indicated that in 2005, the sustainability of China's water-energy-food was at a relatively low efficiency rank. By 2015, the sustainability of China's water-energy-food had reached a general efficiency rank. The results suggested that the sustainability of China's water-energy-food system significantly improved between 2005 and 2015; however, the improved sustainability remained at a general status (The general status means that the sustainability of water-energy-food nexus in China can meet the basic development needs, but it is far from the optimal state and needs further adjustment and improvement). Thus, China should improve its current utilization patterns for the three resources and consider them as a whole. This would help realize synergistic resource use and enhance their sustainability. Highlights • The sustainability of WEF nexus is a severe challenge faced by developing country. • An improved matter-element extension model to evaluate sustainability of WEF nexus. • The sustainability of China's WEF system significantly improved from 2005 to 2015. • China should improve its utilization patterns for the WEF and consider it as whole. [ABSTRACT FROM AUTHOR]