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The scientific interest in radiocesium and plutonium found in the oceans and seas has increased enormously in the past years as a consequence of the Fukushima Dai-ichi Nuclear Power Plant (FDNPP) accident and is expected to be ongoing due to many unresolved questions. Hence, continuous development of new and verification of old analytical methods should be at the top of the list of the community, working on the topic. In this study, we processed and analyzed several seawater samples, collected in different time frames (2011-2015) from the North Pacific Ocean offshore Fukushima, to determine their radiocesium activities, 134Cs/137Cs activity ratios and 240Pu/239Pu isotopic ratios using the sequential scavenging method, gamma spectrometry and accelerator mass spectrometry (AMS). The observed radiocesium levels in seawater (0.07-0.042 Bq L-1) clearly indicated that the investigated region remained impacted by releases from the damaged power plant even after four years after the accident. Regarding plutonium, its successful separation from large volume seawater samples was confirmed by detection of 240Pu by AMS. However, several problems emerged during the analyzes, which we tried to address with the use of additional methods (e.g., measurements of uranium by ICPMS). The efficiencies of the applied methods and other issues are also discussed.

The present work concerns data of three campaigns carried out during the last twenty years in the plain of the Garigliano river surrounding the Garigliano Nuclear Power Plant (GNPP), which is located in Southern Italy and shut down in 1979. Moreover, some data from surveys held in the eighties, across the Chernobyl accident, have been taken in account. The results for the soil samples, in particular for 137Cs and 236U specific activity, were analyzed for their extension in space and in time. Some of the problems related to the classical analysis of environmental radiological data (non-normal distribution of the values, small number of sample points, multiple comparison and presence of values lesser than the minimum detectable activity) have been overcome with the use of Bayesian methods. The scope of the paper is threefold: (1) to introduce the data of the last campaign held in the Garigliano plain; (2) to insert these data in a larger spatio-temporal frame; (3) to show how the Bayesian approach can be applied to radiological environmental surveys, stressing out its advantages over other approaches, using the data of the campaigns. It results that (i) no new contribution there was in the last decades, (ii) specific activity values of the area surrounding the GNPP are consistent with those obtained in other farther areas, (iii) the effective depletion half-life factor for 137Cs is much lower than the half-life of the radionuclide., Comment: 15 pages, 8 figures, presented at the Envira 2019 Conference, to be published in Journal of Environmental Radioactivity (2020)