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This study aimed to assess the nutritional status of soybean and wheat and the relationship with grain yield and biometric components after lime and phosphogypsum (GY) reapplication. Treatments consisted of two lime application methods, surface liming and incorporated liming, to different levels of base saturation (BS) (44, 70, and 90%), in addition to surface liming to 70% BS associated with a standard dose (70GY1) or double dose (70GY2) of GY. Treatments were applied in 2012 and reapplied in 2016. The results refer to the 2018/2019 soybean season and the 2019 wheat season. Lime + GY treatment increased leaf area, plant height, leaf dry matter, and stem dry matter in soybean but had no effect on specific leaf area (235.4 cm2 g−1), stem diameter (6.08 mm), number of pods per plant (71.7), grain number per plant (165), or thousand grain weight (117 g). Liming to 90% BS reduced leaf manganese contents in both crops and leaf iron content in soybean. GY application improved the calcium status of both crops and the sulfur status of soybean. However, 70GY2 reduced leaf magnesium contents in soybean and wheat. Soil tillage without lime reduced wheat yield by 12% compared with no-till. Soybean yield correlated positively with leaf nitrogen (0.79), leaf phosphorus (0.91), leaf area (0.62), and thousand grain weight (0.65), whereas wheat yield correlated with leaf phosphorus (0.83), calcium (0.75), and sulfur (0.74). For improved soybean and wheat performance, it is preferable to apply lime and GY to the soil surface (70GY1), permanently maintaining no-till practices. [ABSTRACT FROM AUTHOR]