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Sea salt aerosol in the boundary layer below shallow cumulus clouds is remotely observed with a Ka-band cloud radar at the Barbados Cloud Observatory and is detected in 76% of the measurements over 1 year. Carried by convection, sea salt particles with a diameter larger than 500 nm show an upward motion of 0.2 m s−1 below shallow cumulus clouds for a 2-day case study. Caused by an increasing relative humidity with increasing altitude, the sea salt particles become larger as they move closer to the cloud base. By using combined measurements of a Ka-band cloud radar and a Raman lidar, the retrieved equivolumetric diameter of the hygroscopically grown sea salt particles is found to be between 6 and 11 μm with a total number concentration of 20 cm−3 near cloud base. Assuming a fixed shape parameter, a size distribution of sea salt particles under high-relative-humidity conditions below cloud base is estimated and agrees with measurements taken by a dry-deposition sampler and online aerosol observations. The methods outlined in this paper can be used in future studies to get a better understanding of the vertical and temporal sea salt distribution in the boundary layer and sea salt aerosol–cloud interaction processes. [ABSTRACT FROM AUTHOR]

This paper furthers previous investigations into the zenith angular effect of cloud contamination within infrared (IR) window radiance observations commonly used in the retrieval of environmental data records (EDRs). Here analyses were performed of clear-sky forward radiance calculations versus observations obtained under clear to partly cloudy conditions over ocean. The authors utilized high-resolution IR spectra observed by the aircraft-based National Polar-Orbiting Partnership (NPP) Aircraft Sounder Test Bed-Interferometer (NAST-I) during the Joint Airborne Infrared Atmospheric Sounding Interferometer (IASI) Validation Experiment (JAIVEx) and performed forward calculations using collocated dropsondes. An aerosol optical depth EDR product derived from Geostationary Operational Environmental Satellite (GOES) was then applied to detect clouds within NAST-I fields of view (FOVs). To calculate the angular variation of clouds, expressions were derived for estimating cloud aspect ratios from visible imagery where cloud shadow lengths can be estimated relative to cloud horizontal diameters. In agreement with sensitivity calculations, it was found that a small cloud fraction within window radiance observations can have a measurable impact on the angular agreement with clear-sky calculations on the order of 0.1-0.4 K in brightness temperature. It was also found that systematic sun-glint contamination can likewise have an impact on the order of 0.1 K. These results are germane to IR sensor data record (SDR) calibration/validation and EDR retrieval schemes depending upon clear-sky SDRs, as well as radiative transfer modeling involving randomly distributed broken cloud fields. [ABSTRACT FROM AUTHOR]