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Nonlinear metasurfaces provide a promising platform for integrated nonlinear photonic devices owing to their unprecedented capability of nonlinear wavefront manipulation. However, the previously reported second‐harmonic (SH) metasurfaces are mainly based on the nonlinear Pancharatnam–Berry phase modulation. While this method is quite convenient and robust, it shows limitations of modulation efficiency and the difficulty in extending to multidimensional combined modulations. Here, the resonant nonlinear synthetic metasurface is proposed and experimentally demonstrated for independent phase and amplitude modulations of the SH beam. A high SH modulation efficiency of 75% (with a theoretical limit of 90%) is achieved in the polarization‐dependent SH metalens. Moreover, SH holographic imaging with phase and amplitude (at 2 and 4 levels) combined modulation is realized experimentally. Compared with the pure‐phase modulation, the signal‐to‐noise ratios are increased by 2 and 3 times when 2‐ and 4‐level amplitude controls are introduced. This is not only an important step in the improvement and innovation of holographic display technology, but also paves a distinct avenue toward multifunctional, higher efficiency, and ultracompact nonlinear optical devices. [ABSTRACT FROM AUTHOR]

Here we report on the hybrid nanostructures where a single ZnS nanobelt was half-covered with an aluminum (Al) film, which is an ideal platform for studying the second-harmonic generation (SHG) enhancement effects of the Al coating. It was fabricated by the lift-off process and allowed for the accurate comparison of the SHG intensity between the Al-covered and the same bare ZnS nanobelt under consistent test conditions. The results indicate that the Al coating in the hybrid nanostructures not only confines the pumping laser in the ZnS effectively, but also concentrates the emitted SHG signal greatly, increasing the signal collection efficiency. By the combination of these two effects, ∼60 times enhancement of the SHG intensity is achieved at the optimized geometry size (width and thickness) of the ZnS nanobelts. The Al-based hybrid nanostructures open up new possibilities for low-cost, highly efficient and directional coherent nanolight sources at short wavelengths. [ABSTRACT FROM AUTHOR]