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Traditional surface polishing methods are no longer able to meet the ultra-precision requirements of the high-tech industry for the inner surface of the pipe, but magnetorheological polishing technology is very suitable due to its advantages of high precision, fast controllability and good deposition stability. However, there is even less investigation on the microforce analysis, chaining mechanism and micromodeling methods of magnetorheological polishing fluid (MRPF), and the polishing mechanism of MRPF has not been explored yet. As a step to completely develop the magnetorheological polishing (MRP) technique, this paper proposed the simulation method of MRPF based on particle dynamics, and the shear stress model of magnetorheological fluid (MRF) is optimized under the action of the magnetic field after performing the chain simulation. On the basis of the optimized shear stress model and the hexagonal close-packed structure of MRF, the holding mechanism of polishing abrasive particles is explored for the MRPF and the corresponding holding models are proposed. Then, the shear yield stress models and material removal model are also established for the inner surface polishing, respectively. Eventually, the above theoretical analysis and related models have been verified though the polishing experiment of the titanium alloy pipe. [ABSTRACT FROM AUTHOR]