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Vortex-induced vibration (VIV) is a process that wind energy converts to the mechanical energy of the bluff body. Enhancing VIV to harvest wind energy is a promising method to power wireless sensor nodes in the Internet of Things. In this work, a VIV-driven square cylinder triboelectric nanogenerator (SC-TENG) is proposed to harvest broadband wind energy. The vibration characteristic and output performance are studied experimentally to investigate the effect of the natural frequency by using five different springs in a wide range of stiffnesses ( 27   N / m < K < 90   N / m ). The square cylinder is limited to transverse oscillation and experiments were conducted in the Reynolds regime ( 3.93 × 10 3 – 3.25 × 10 4 ). The results demonstrate the strong dependency of VIV on natural frequency and lock-in observed in a broad range of spring stiffness. Moreover, the amplitude ratio and range of lock-in region increase by decreasing spring stiffness. On the other hand, the SC-TENG with higher spring stiffness can result in higher output under high wind velocities. These observations suggest employing an adjustable natural frequency system to have optimum energy harvesting in VIV-based SC-TENG in an expanded range of operations. [ABSTRACT FROM AUTHOR]