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Start Over Author "Yang, Fa" Journal nature communications
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5. Bismuthene for highly efficient carbon dioxide electroreduction reaction

Author

Manos Mavrikakis, Roberto Schimmenti, Ping Song, Ahmed O. Elnabawy, Weilin Xu, Shuang Yao, Yang Fa, Yue Lin, Ruiping Deng, Jiawei Wang, Shuyan Song, and Zhangquan Peng

Subjects
Materials science, Science, General Physics and Astronomy, chemistry.chemical_element, 02 engineering and technology, Overpotential, Two-dimensional materials, 010402 general chemistry, Electrocatalyst, 01 natural sciences, Article, General Biochemistry, Genetics and Molecular Biology, Catalysis, Bismuth, chemistry.chemical_compound, Monolayer, Formate, lcsh:Science, Author Correction, Heterogeneous catalysis, Multidisciplinary, General Chemistry, 021001 nanoscience & nanotechnology, 0104 chemical sciences, chemistry, Chemical engineering, Reversible hydrogen electrode, lcsh:Q, Electrocatalysis, 0210 nano-technology, Faraday efficiency
Abstract

Bismuth (Bi) has been known as a highly efficient electrocatalyst for CO2 reduction reaction. Stable free-standing two-dimensional Bi monolayer (Bismuthene) structures have been predicted theoretically, but never realized experimentally. Here, we show the first simple large-scale synthesis of free-standing Bismuthene, to our knowledge, and demonstrate its high electrocatalytic efficiency for formate (HCOO−) formation from CO2 reduction reaction. The catalytic performance is evident by the high Faradaic efficiency (99% at −580 mV vs. Reversible Hydrogen Electrode (RHE)), small onset overpotential (, Stable free-standing two-dimensional Bi monolayer (Bismuthene) structures have been predicted theoretically, but never realized experimentally. Here, the authors show a large-scale synthesis of free-standing Bismuthene and its electrocatalytic activity for CO2 reduction to formate.

Published
2020

6. Author Correction: Bismuthene for highly efficient carbon dioxide electroreduction reaction

Author

Manos Mavrikakis, Roberto Schimmenti, Yue Lin, Ping Song, Ruiping Deng, Shuang Yao, Shuyan Song, Ahmed O. Elnabawy, Yang Fa, Zhangquan Peng, Jiawei Wang, and Weilin Xu

Subjects
chemistry.chemical_compound, Multidisciplinary, Materials science, chemistry, Science, Inorganic chemistry, Carbon dioxide, General Physics and Astronomy, lcsh:Q, General Chemistry, lcsh:Science, General Biochemistry, Genetics and Molecular Biology
Abstract

An amendment to this paper has been published and can be accessed via a link at the top of the paper.

Published
2020

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