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International audience; We report on structured light-induced femtosecond direct laser writing (DLW) under tight focusing in non-commercial silver-containing zinc phosphate glass, which leads to original patterns of fluorescent silver clusters. These fluorescence topologies show unique features of frustrated diffusion of charged species, giving rise to distorted silver cluster spatial distributions. Fluorescence and second harmonic generation correlative microscopy demonstrate the realization of structured light-induced direct laser poling, resulting from a laser-induced permanent and stable electric field buried inside the modified glass. Thus, structured light-induced DLW remarkably enables both linear and nonlinear patterning. This work highlights the interest of optical phase engineering to obtain nontrivial beam profiles and subsequent photo-induced patterns that cannot be reached under Gaussian beam irradiation.

We demonstrate the first (to our knowledge) quasi-three-level conical refraction laser operating at 2 μm, with 1.6 W of output power at 2074 nm, using a holmium-doped KY(WO4)2 crystal. A maximum slope efficiency of 52% has been achieved, along the optic axis with respect to the absorbed pump power. Furthermore, lasing operation around the optic axis has been performed. In this case, a maximum output power of 3 W has been reached, with a slope efficiency better than 70%, which are the best performances ever reported on this material.

We demonstrate simultaneous measurement of the real and the imaginary parts of third-order susceptibilities by use of a collinear pump-probe technique. This technique allows for good results and simple implementation. The signal analysis is based on the particular oscillatory signature versus the pump-probe delay allowed by the collinear configuration. Results are compared with interferometric measurements of a SF59 (Schott) glass sample.