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Three-dimensional phase field simulations of coupled γ/γ ′ microstructural evolution and plastic deformation in single crystal Ni-Al are carried out at micrometer scales. Coherent γ/γ ′ microstructures and plastic deformation in γ-channels are described using a single, consistent methodology based on Khachaturyan's phase field microelasticity approach to coherent precipitates and dislocations. In particular, a new set of phase fields is introduced to characterize local density of dislocations from individual active slip systems. To increase the length scale of the phase field simulations, the Kim–Kim–Suzuki (KKS) treatment of γ/γ ′ interfaces was adopted. The rafting kinetics, precipitate-matrix inversion process and the corresponding creep deformation are characterized with respect to parameters such as applied stress and lattice misfit. The simulation results on γ ′-rafting kinetics and morphological evolution of the γ/γ ′ microstructures are compared with available experiment. The model can be used to ...