1. High-harmonic generation by nonlinear resonant excitation of surface plasmon modes in metallic nanoparticles
- Author
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Fernando Haas, Jérôme Hurst, Paul-Antoine Hervieux, Giovanni Manfredi, Institut de Physique et Chimie des Matériaux de Strasbourg (IPCMS), Université de Strasbourg (UNISTRA)-Centre National de la Recherche Scientifique (CNRS)-Matériaux et nanosciences d'Alsace, Centre National de la Recherche Scientifique (CNRS)-Institut National de la Santé et de la Recherche Médicale (INSERM)-Université de Haute-Alsace (UHA) Mulhouse - Colmar (Université de Haute-Alsace (UHA))-Université de Strasbourg (UNISTRA)-Centre National de la Recherche Scientifique (CNRS)-Institut National de la Santé et de la Recherche Médicale (INSERM)-Université de Haute-Alsace (UHA) Mulhouse - Colmar (Université de Haute-Alsace (UHA))-Université de Strasbourg (UNISTRA)-Réseau nanophotonique et optique, and Centre National de la Recherche Scientifique (CNRS)-Université de Strasbourg (UNISTRA)-Université de Haute-Alsace (UHA) Mulhouse - Colmar (Université de Haute-Alsace (UHA))-Université de Strasbourg (UNISTRA)
- Subjects
Materials science ,Physics::Optics ,02 engineering and technology ,Effective radiated power ,Sistemas mesoscopicos ,01 natural sciences ,7. Clean energy ,Molecular physics ,law.invention ,Optics ,[PHYS.QPHY]Physics [physics]/Quantum Physics [quant-ph] ,law ,Ionization ,0103 physical sciences ,High harmonic generation ,Geração harmônica óptica ,010306 general physics ,ComputingMilieux_MISCELLANEOUS ,business.industry ,Surface plasmon ,Nanopartículas ,021001 nanoscience & nanotechnology ,Condensed Matter Physics ,Laser ,Electronic, Optical and Magnetic Materials ,Harmonics ,Quasiparticle ,Fotoionizacao ,Plasmas de superfície ,0210 nano-technology ,business ,Excitation - Abstract
The nonlinear electron dynamics in metallic nanoparticles is studied using a hydrodynamic model that incorporates most quantum many-body features, including spill-out and nonlocal effects as well as electron exchange and correlations. We show that, by irradiating the nanoparticle with a chirped laser pulse of modest intensity (autoresonance), it is possible to drive the electron dynamics far into the nonlinear regime, leading to enhanced energy absorption and complete ionization of the nanoparticle on a time scale of the order of 100 fs. The accompanying radiated power spectrum is rich in high-order harmonics.
- Published
- 2014
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