1. Detection of weak emergent broken-symmetries of the kagome antiferromagnet by Raman spectroscopy
- Author
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Jan O. Haerter, Claire Lhuillier, and Olivier Cepas
- Subjects
Physics ,Condensed matter physics ,Condensed Matter Physics ,Electronic, Optical and Magnetic Materials ,Crystal ,symbols.namesake ,symbols ,Antiferromagnetism ,Condensed Matter::Strongly Correlated Electrons ,Valence bond theory ,Coherent anti-Stokes Raman spectroscopy ,Quantum spin liquid ,Ground state ,Raman spectroscopy ,Random phase approximation - Abstract
We show that the magnetic Raman response of a spin liquid is independent of the polarizations of the light for triangular symmetries. In contrast, a ground state that has a broken-symmetry shows characteristic oscillations when the polarizations are rotated. This would allow one to detect weak broken-symmetries and emergent order parameters. We focus on the kagome antiferromagnet wherein no conventional long-range order has been found so far and present the Raman cross section of a spin liquid and a valence bond crystal by using a random phase approximation.
- Published
- 2008
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