1. Spin-Driven Jahn-Teller Distortion in a Pyrochlore System
- Author
-
Kazuo Ueda and Yasufumi Yamashita
- Subjects
Physics ,Phase transition ,Strongly Correlated Electrons (cond-mat.str-el) ,Condensed matter physics ,Heisenberg model ,Jahn–Teller effect ,Pyrochlore ,FOS: Physical sciences ,General Physics and Astronomy ,engineering.material ,Condensed Matter - Strongly Correlated Electrons ,Condensed Matter::Materials Science ,Tetragonal crystal system ,engineering ,Antiferromagnetism ,Condensed Matter::Strongly Correlated Electrons ,Valence bond theory ,Spin-½ - Abstract
The ground-state properties of the spin-1 antiferromagnetic Heisenberg model on the corner-sharing tetrahedra, pyrochlore lattice, is investigated. By breaking up each spin into a pair of 1/2-spins, the problem is reduced to the equivalent one of the spin-1/2 tetrahedral network in analogy with the valence bond solid state in one dimension. The twofold degeneracy of the spin-singlets of a tetrahedron is lifted by a Jahn-Teller mechanism, leading to a cubic to tetragonal structural transition. It is proposed that the present mechanism is responsible for the phase transition observed in the spin-1 spinel compounds ZnV$_2$O$_4$ and MgV$_2$O$_4$., Comment: 4 pages, 3 eps figures, REVTeX, to appear in Phys. Rev. Lett
- Published
- 2000
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