10 results on '"Luca Perfetti"'
Search Results
2. Significant Reduction of Electronic Correlations upon Isovalent Ru Substitution ofBaFe2As2
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Véronique Brouet, Dorothée Colson, B. Mansart, François Bertran, Amina Taleb-Ibrahimi, A. Forget, Jérôme Faure, F. Rullier-Albenque, Markus Aichhorn, Luca Perfetti, Marino Marsi, Silke Biermann, and P. Le Fèvre
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Superconductivity ,Materials science ,Condensed matter physics ,Magnetism ,General Physics and Astronomy ,Angle-resolved photoemission spectroscopy ,Fermi surface ,02 engineering and technology ,Electronic structure ,Electron ,021001 nanoscience & nanotechnology ,01 natural sciences ,Hall effect ,0103 physical sciences ,Strongly correlated material ,010306 general physics ,0210 nano-technology - Abstract
We investigate $\mathrm{Ba}({\mathrm{Fe}}_{0.65}{\mathrm{Ru}}_{0.35}{)}_{2}{\mathrm{As}}_{2}$, a compound in which superconductivity appears at the expense of magnetism, by transport measurements and angle resolved photoemission spectroscopy. By resolving the different Fermi surface pockets and deducing from their volumes the number of hole and electron carriers, we show that Ru induces neither hole nor electron doping. However, the Fermi surface pockets are about twice larger than in ${\mathrm{BaFe}}_{2}{\mathrm{As}}_{2}$. A change of sign of the Hall coefficient with decreasing temperature evidences the contribution of both carriers to the transport. Fermi velocities increase significantly with respect to ${\mathrm{BaFe}}_{2}{\mathrm{As}}_{2}$, suggesting a reduction of correlation effects.
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- 2010
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3. Ultrafast Electron Relaxation in SuperconductingBi2Sr2CaCu2O8+δby Time-Resolved Photoelectron Spectroscopy
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Uwe Bovensiepen, Panagiotis A. Loukakos, Luca Perfetti, Martin Wolf, M. Lisowski, and Hiroshi Eisaki
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Superconductivity ,Materials science ,Thermalisation ,X-ray photoelectron spectroscopy ,Phonon ,Condensed Matter::Superconductivity ,Doping ,General Physics and Astronomy ,Electronic structure ,Electron ,Atomic physics ,Omega - Abstract
Time-resolved photoelectron spectroscopy is employed to study the dynamics of photoexcited electrons in optimally doped Bi{2}Sr{2}CaCu{2}O{8+delta} (Bi-2212). Hot electrons thermalize in less than 50 fs and dissipate their energy on two distinct time scales (110 fs and 2 ps). These are attributed to the generation and subsequent decay of nonequilibrium phonons, respectively. We conclude that 20% of the total lattice modes dominate the coupling strength and estimate the second momentum of the Eliashberg coupling function lambdaOmega{0}{2}=360+/-30 meV{2}. For the typical phonon energy of copper-oxygen bonds (Omega{0} approximately 40-70 meV), this results in an average electron-phonon coupling lambda
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- 2007
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4. Time Evolution of the Electronic Structure of1T−TaS2through the Insulator-Metal Transition
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Uwe Bovensiepen, Martin Wolf, Pablo S. Cornaglia, Antoine Georges, Helmuth Berger, Panagiotis A. Loukakos, Silke Biermann, Luca Perfetti, and M. Lisowski
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Physics ,Electronic correlation ,Condensed matter physics ,Mott insulator ,Excited state ,Femtosecond ,Time evolution ,General Physics and Astronomy ,Condensed Matter::Strongly Correlated Electrons ,Electronic structure ,Metal–insulator transition ,Excitation - Abstract
Femtosecond time-resolved photoemission is used to investigate the time evolution of electronic structure in the Mott insulator 1T-TaS2. A collapse of the electronic gap is observed within 100 femtoseconds after optical excitation. The photoemission spectra and the spectral function calculated by dynamical mean field theory show that this insulator-metal transition is driven solely by hot electrons. A coherently excited lattice displacement results in a periodic shift of the spectra lasting for 20 ps without perturbing the insulating phase. This capability to disentangle electronic and phononic excitations opens new directions to study electron correlation in solids.
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- 2006
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5. Strongly Coupled Optical Phonons in the Ultrafast Dynamics of the Electronic Energy and Current Relaxation in Graphite
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Christian Frischkorn, F. Schapper, Tobias Kampfrath, Luca Perfetti, and Martin Wolf
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Materials science ,Condensed matter physics ,Ambipolar diffusion ,Phonon ,Terahertz radiation ,business.industry ,General Physics and Astronomy ,Electron ,Terahertz spectroscopy and technology ,Photoexcitation ,Condensed Matter::Materials Science ,Optics ,Excited state ,Charge carrier ,business - Abstract
Ultrafast charge carrier dynamics in graphite has been investigated by time-resolved terahertz spectroscopy. Analysis of the transient dielectric function and model calculations show that more than 90% of the initially deposited excitation energy is transferred to a few strongly coupled lattice vibrations within 500 fs. These hot optical phonons also substantially contribute to the striking increase of the Drude relaxation rate observed during the first picosecond after photoexcitation. The subsequent cooling of the hot phonons yields a lifetime estimate of 7 ps for these modes. Graphite has attracted continuous attention in research over the past decades [1]. Recently, a strong ambipolar electric field effect was found in thin films of this semimetal, thereby demonstrating its potential for future electronics [2]. Moreover, graphite is closely related to carbon nanotubes, which are the focus of nanotechnology research [3]. The latest experimental and theoretical efforts revealed that optical phonons in graphite strongly interact with the electrons [4,5]. These strongly coupled optical phonons (SCOPs) have high quantum energies of up to 0.2 eV and can be excited only by electrons of elevated energy. The scattering of electrons by SCOPsis believed to increase the dc resistivity of carbon nanotubes when high electric fields are applied [3]. In view of possible applications in electronics, further investigations are required on how SCOPs influence the transport and energy relaxation of electrons. Time-resolved terahertz spectroscopy (TRTS) is a promising experimental approach to this question. Avisible pump pulse excites charge carriers in the sample and thus enables them to generate optical phonons. A subsequent terahertz (THz) pulse probes the low-energy response of the system
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- 2005
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6. Ultrafast dynamics of delocalized and localized electrons in carbon nanotubes
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Patrick Desjardins, Richard Martel, Luca Perfetti, Carla M. Aguirre, Christian Frischkorn, F. Schapper, Tobias Kampfrath, Tobias Hertel, A. Hagen, and Martin Wolf
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Materials science ,Exciton ,Physics::Optics ,General Physics and Astronomy ,Nanotechnology ,Carbon nanotube ,Electron ,Molecular physics ,law.invention ,Carbon nanotube quantum dot ,Optical properties of carbon nanotubes ,Condensed Matter::Materials Science ,Delocalized electron ,law ,Charge carrier ,Absorption (electromagnetic radiation) - Abstract
We report on the dynamics of the dielectric function of single-wall carbon nanotubes in the 10--30 THz frequency range after ultrafast laser excitation. The absence of a distinct free-carrier response is attributed to the photogeneration of strongly bound excitons in the tubes with large energy gaps. We find a feature of enhanced transmission caused by the blocking of optical transitions in small-gap tubes. The rapid decay of a featureless background with pronounced dichroism is associated with the increased absorption of spatially localized charge carriers before thermalization is completed.
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- 2005
7. Mott phase at the surface of 1T-TaSe2 observed by scanning tunneling microscopy
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Stefano, Colonna, Fabio, Ronci, Antonio, Cricenti, Luca, Perfetti, Helmuth, Berger, and Marco, Grioni
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In this Letter we report the observation, by scanning tunneling microscopy, of a Mott metal to insulator transition at the surface of 1T-TaSe2. Our spectroscopic data compare considerably well with previous angle-resolved photoemission spectroscopy measurements and confirm the presence of a large hysteresis related to a first order process. The local character of the tunneling spectroscopy technique allows a direct visualization of the surface symmetry and provides spectroscopic measurements on the defect-free region of the sample. It follows that the electronic localization is driven purely by the enhancement of the charge density wave amplitude which drives a bandwidth controlled metal-insulator transition.
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- 2004
8. Low Energy Electronic Excitations in the Layered Cuprates Studied by CopperL3Resonant Inelastic X-Ray Scattering
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Marco Grioni, Giacomo Claudio Ghiringhelli, Alberto Tagliaferri, E. Annese, Luca Perfetti, Claudia Dallera, Helmuth Berger, N. B. Brookes, and Lucio Braicovich
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Physics ,Condensed matter physics ,Scattering ,Energy level splitting ,General Physics and Astronomy ,Electronic structure ,Inelastic scattering ,Resonant inelastic X-ray scattering ,symbols.namesake ,Photon polarization ,symbols ,Condensed Matter::Strongly Correlated Electrons ,Cuprate ,Raman scattering - Abstract
We have measured the resonant inelastic x-ray scattering (RIXS) spectra at the Cu L3 edge in a variety of cuprates. Exploiting a considerably improved energy resolution (0.8 eV) we recorded significant dependencies on the sample composition and orientation, on the scattering geometry, and on the incident photon polarization. The RIXS final states correspond to two families of electronic excitations, having local (dd excitations) and nonlocal (charge-transfer) character. The dd energy splitting can be estimated with a simple crystal field model. The RIXS at the L3 edge demonstrates here a great potential, thanks to the resonance strength and to the large 2p spin-orbit splitting.
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- 2004
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9. Spectroscopic Signatures of a Bandwidth-Controlled Mott Transition at the Surface of1T−TaSe2
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S. Biermann, Y. Tomm, Marco Grioni, Serge Florens, Helmuth Berger, Hartmut Höchst, Slobodan Mitrovic, Luca Perfetti, and Antoine Georges
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Condensed Matter::Quantum Gases ,Physics ,Condensed matter physics ,Hubbard model ,Spectral weight ,Photoemission spectroscopy ,Bandwidth (signal processing) ,General Physics and Astronomy ,Fermi surface ,02 engineering and technology ,021001 nanoscience & nanotechnology ,7. Clean energy ,01 natural sciences ,Mott transition ,0103 physical sciences ,Quasiparticle ,Condensed Matter::Strongly Correlated Electrons ,Spectral function ,010306 general physics ,0210 nano-technology - Abstract
High-resolution angle-resolved photoemission data show that a metal-insulator Mott transition occurs at the surface of the quasi-two-dimensional compound 1T-TaSe2. The transition is driven by the narrowing of the Ta 5d band induced by a temperature-dependent modulation of the atomic positions. A dynamical mean-field theory calculation of the spectral function of the half-filled Hubbard model captures the main qualitative feature of the data, namely, the rapid transfer of spectral weight from the observed quasiparticle peak at the Fermi surface to the Hubbard bands, as the correlation gap opens up.
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- 2003
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10. Spectroscopic Indications of Polaronic Carriers in the Quasi-One-Dimensional Conductor(TaSe4)2I
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Leonardo Degiorgi, Giorgio Margaritondo, Johannes Voit, Hartmut Höchst, A. Reginelli, Marco Grioni, Helmuth Berger, and Luca Perfetti
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Physics ,Condensed matter physics ,Condensed Matter::Superconductivity ,Quasiparticle ,General Physics and Astronomy ,Condensed Matter::Strongly Correlated Electrons ,Angle-resolved photoemission spectroscopy ,Fermi liquid theory ,Electronic structure ,Metal–insulator transition ,Adiabatic process ,Polaron ,Pseudogap - Abstract
Angle-resolved photoemission (ARPES) on the quasi-one-dimensional conductor (TaSe4)(2)I shows a hidden Fermi-surface crossing in its metallic state and the opening of a Peierls gap at low temperatures, The underlying quasiparticles have vanishing spectral weight and extremely short coherence lengths. They are interpreted as polarons in the strong-coupling adiabatic Lin-Lit, and almost all their ARPES weight is incoherent. These observations suggest a scenario where the long-standing contradictions between ARPES and other experiments on Peierls materials could be resolved.
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- 2001
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