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To reduce the oxidative degradation of citral and improve its antimildew performance, citral was modified with natural antioxidants such as tea polyphenols, ascorbic acid, and theaflavin in the present study. Additionally, the effects of these natural antioxidants on the citral degradation rate and DPPH radical-scavenging rate, as well as the effectiveness of antioxidant-modified citral in the antimildew treatment of bamboo were investigated. Ascorbic acid, theaflavin, and tea polyphenols improved the antioxidant performance of citral to some extent, and the tea polyphenols exhibited the best antioxidant performance. When the amount of tea polyphenols added to citral reached 1.0%, the oxidative degradation of citral was effectively prevented. Compared with citral, tea-polyphenol-modified citral could reduce the efficacy of the bamboo antimildew treatment against all four mildews and the effectiveness of the antimildew treatment reached 100%. Citral modification with antioxidants reduced the amount of citral required in the treatment, thereby reducing the treatment cost for bamboo mildew.