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Let S be the polynomial ring on the space of non-square generic matrices or the space of odd-sized skew-symmetric matrices, and let I be the determinantal ideal of maximal minors or Pf the ideal of sub-maximal Pfaffians, respectively. Using desingularizations and representation theory of the general linear group we expand upon work of Raicu–Weyman–Witt [Adv. Math. 250 (2014), pp. 596–610] to determine the S-module structures of Ext^j_S(S/I^t, S) and Ext^j_S(S/Pf^t, S), from which we get the degrees of generators of these Ext modules. As a consequence, via graded local duality we answer a question of Wenliang Zhang [J. Pure Appl. Algebra 225 (2021), Paper No. 106789] on the socle degrees of local cohomology modules of the form H^j_\mathfrak {m}(S/I^t). [ABSTRACT FROM AUTHOR]